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This article presents the evaluation of using pulsed-radio frequency (RF) signals as multitone phase standards for modulated measurements at millimeter-wave (mm-Wave) bands, offering an alternative phase calibration choice for nonlinear vector network analyzers (NVNAs). Based on the NVNA measurements of two pulsed-RF signals generated by square-wave-driven mixers, a high correlation between magnitude and phase errors of unideal pulsed-RF signals is discovered, and an empirical method is developed to accurately estimate the phase errors according to magnitude-only measurements. To confirm its robustness and key preconditions for wide-range applications, theoretical support and explanation to the empirical method is revealed, in which the dominant waveform distortion of an applicable pulsed-RF signal can be decomposed into modulated perturbations with Sinc-like envelopes. The validity of the proposed empirical method, as well as its application for mm-Wave NVNA phase calibration, is verified by both experimental measurements and simulation results, where an estimation error (or phase calibration error) less than ±2° is demonstrated that is reachable in practice. [ABSTRACT FROM AUTHOR]