1. Magneto-structural correlations in a systematically disordered B2 lattice
- Author
-
Jonathan Ehrler, Biplab Sanyal, Jörg Grenzer, Shengqiang Zhou, Roman Böttger, Benedikt Eggert, Heiko Wende, Jürgen Lindner, Jürgen Fassbender, Christoph Leyens, Kay Potzger, and Rantej Bali
- Subjects
phase transitions ,disorder ,ion beam modifications ,magneto-structural effects ,Science ,Physics ,QC1-999 - Abstract
Ferromagnetism in certain B2 ordered alloys such as Fe _60 Al _40 can be switched on, and tuned, via antisite disordering of the atomic arrangement. The disordering is accompanied by a ∼1 % increase in the lattice parameter. Here we performed a systematic disordering of B2 Fe _60 Al _40 thin films, and obtained correlations between the order parameter ( S ), lattice parameter ( a _0 ), and the induced saturation magnetization ( M _s ). As the lattice is gradually disordered, a critical point occurs at 1 − S = 0.6 and a _0 = 2.91 Å, where a sharp increase of the M _s is observed. DFT calculations suggest that below the critical point the system magnetically behaves as it would still be fully ordered, whereas above, it is largely the increase of a _0 in the disordered state that determines the M _s . The insights obtained here can be useful for achieving tailored magnetic properties in alloys through disordering.
- Published
- 2020
- Full Text
- View/download PDF