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The molecule N,N′-bis(3-methylphenyl)-N,N′-dyphenylbenzidine (TPD) has been widely used in optoelectronic applications, mainly for its hole-transporting properties, but also for its capability to emit blue light and amplified spontaneous emission, which is important for the development of organic lasers. Here, we report deep-blue-emitting distributed feedback (DFB) lasers based on TPD dispersed in polystyrene (PS), as active media, and dichromated gelatin layers with holographically engraved relief gratings, as laser resonators. The effect of the device architecture (with the resonator located below or on top of the active layer) is investigated with a dye (TPD) that can be doped into PS at higher rates (up to 60 wt%), than with previously used dyes (<5 wt%). This has enabled changing the index contrast between film and resonator, which has an important effect on the laser performance. With regards to thresholds, both architectures behave similarly for TPD concentrations above 20 wt%, while for lower concentrations, top-layer resonator devices show lower values (around half). Remarkably, the operational durability of top-layer resonator devices is larger (in a factor of around 2), independently of the TPD concentration. This is a consequence of the protection offered by the resonator against dye photo-oxidation when the device is illuminated with pulsed UV light. [ABSTRACT FROM AUTHOR]

Amplified Spontaneous Emission is ubiquitous in systems with optical gain and is responsible for many opportunities and shortcomings. Its role in the progression from the simplest form of thermal radiation (single emitter spontaneous emission) all the way to coherent radiation from inverted systems is still an open question. We critically review observations of photon bursts in micro- and nanolasers, in the perspective of currently used measurement techniques, in relation to threshold-related questions for small devices. Corresponding stochastic predictions are analyzed, and contrasted with burst absence in differential models, in light of general phase space properties. A brief discussion on perspectives is offered in the conclusions. [ABSTRACT FROM AUTHOR]

In this study, high-order distributed-feedback (DFB) polymer lasers were comparatively investigated. Their performance relies on multiple lasing directions and their advantages include their high manufacturing tolerances due to the large grating periods. Nine laser cavities were fabricated by spin-coating the gain polymer films onto a grating structure, which was manufactured via interference lithography that operated at the 2nd, 3rd, and 4th DFB orders. Low threshold lasing and high slope efficiency were achieved in high-order DFB polymer lasers due to the large grating groove depth and the large gain layer thickness. A high-order DFB configuration shows possible advantages, including the ability to control the lasing direction and to achieve multiple-wavelength lasers. Furthermore, our investigation demonstrates that the increase in threshold and decrease in slope efficiency with an increase in the feedback order can be limited by controlling the structural parameters. [ABSTRACT FROM AUTHOR]