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This paper investigates the interfacial bonding behavior between high toughness resin concrete with steel wire mesh (HTRCS) and concrete. A total of five sets of fifteen double shear specimens were tested for parameters including concrete strength and material properties of HTRCS composites. The test results showed that the failure mode of DS1 specimens was partial debonding and fracture, and the rest of the specimens were the fracture of HTRCS. The concrete strength and reinforcement ratios of HTRCS composites were positively correlated with interfacial adhesion properties. When the concrete strength was increased from C30 to C40 and C50, the ultimate load increased by 43.4% and 43.2%, respectively. The ultimate load capacity increased by 32.1%, with the reinforcement ratio of HTRCS composites increasing from 1.05% to 1.83%. Moreover, the bonding slip model and the bearing capacity formula for the interface between HTRCS composites and concrete were proposed, and the calculation values were in good agreement with the test values, with an average value of 0.978. [ABSTRACT FROM AUTHOR]