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Receiver function (RF) analysis is an indispensable method that is widely utilized to image the deep structure of the crust and upper mantle. Although the P -wave receiver function (PRF) has the advantages of a higher signal-to-noise ratio and higher resolution than S -wave receiver function, the information about P -to- S converted (Ps) phases from velocity discontinuities of the crust and upper mantle is usually obstructed by multiples from shallower crustal interfaces. Sometimes it is difficult to identify useful information about lithospheric discontinuities. In this paper, we propose a method for suppressing multiples and isolating the Ps phases of RFs. This task is accomplished by exploiting the differences in arrival times resulting from the slowness between the conversion and the multiples that occur at the same interface in the PRFs and by separating them in the Radon domain, which enables removal of crustal and sedimentary multiples. This method can effectively remove multiples and isolate the useful signals of Ps phases contained in the PRFs. We test the method on synthetic PRFs and demonstrate that crustal multiples can be effectively eliminated or suppressed and that the Ps phase of lithospheric discontinuities can be coherently traced. Next, we apply the method to real PRF data collected from the seismic station of the China Array seismic experiment (Phase II and Phase III) in the Ordos block and its adjacent area, and successfully obtain an improved common conversion point stacking image of lithospheric discontinuity structures in the depth domain, particularly for detecting the lithosphere–asthenosphere boundary. [ABSTRACT FROM AUTHOR]