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Thermal conductive polymer composite prepared by 3D printing technology, which has a highly vertically oriented carbon fiber structure.

Considering the significant threat of heat to electronic equipment and the heat dissipation problems existing in powerful systems, thermal management materials are in high demand. In conjunction with the increasing desire of dissipating heat and stabilizing temperature, high thermal conductivity and phase change latent heat are attracting more attention when designing thermal management material. This work proposes a strategy to combine phase change matrix and thermally conductive filler using freeze casting. The highest thermal conductivity reaches 23.1 W m-1 K-1 accompanied by 62 J g-1 phase change latent heat. Meanwhile, replacing ice with organic phase change material in freeze casting can result in an aligned structure. This discovery will pave a novel way for introducing thermal latent heat without abandoning the aligned structure.

Simultaneous achievement of high thermal transportation performance and superior mechanical properties in a same thermal management composite film.

Correction for ‘Ultrahigh thermal conductive polymer composites by the 3D printing induced vertical alignment of carbon fiber’ by Zhenbang Zhang et al., J. Mater. Chem. A, 2023, https://doi.org/10.1039/D3TA01676E.