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Ultra-short pulses in blue region generated from compact and low-cost semiconductor lasers have attracted much attention for a wide variety of applications. Nitride-based vertical-cavity surface-emitting lasers (VCSELs), having intrinsic high material gain and short cavities, favor the generation of ultra-short blue pulses via a simple gain-switching technique. In this study, we fabricated a single-mode InGaN VCSEL consisting of 10-period InGaN/GaN quantum wells (QWs). The output pulses were evaluated accurately with an up-conversion measurement system having time resolution of 0.12 ps. We demonstrated that ultra-short blue pulses, as short as 2.2 ps at 3.4 K and 4.0 ps at room temperature, were generated from the gain-switched InGaN VCSEL via impulsive optical pumping, without any post-processing. The gain-switched pulses we obtained should greatly promote the development of ultra-short blue pulse generation. In addition, this successful assessment demonstrates the up-conversion technique's usefulness for characterizing ultra-short blue pulses from semiconductor lasers. [ABSTRACT FROM AUTHOR]

Short pulses generated from low-cost semiconductor lasers by a simple gain-switching technique have attracted enormous attention because of their potential usage in wide applications. Therein, reducing the durations of gain-switched pulses is a key technical point for promoting their applications. Therefore, understanding the dynamic characteristics of gain-switched pulses is highly desirable. Herein, we used streak camera to investigate the time- and spectral-resolved lasing characteristics of gain-switched pulses from optically pumped InGaN single-mode vertical-cavity surface-emitting lasers. We found that fast initial components with ultra-short durations far below our temporal resolution of 5.5 ps emerged on short-wavelength sides, while the entire pulses were down-chirped, resulting in the simultaneous broadening of the spectrum and pulse width. The measured chirp characteristics were quantitatively explained using a single-mode rate-equation model, combined with carrier-density-dependent gain and index models. The observed universal fast short-wavelength components can be useful in generating even shorter pulses from gain-switched semiconductor lasers. [ABSTRACT FROM AUTHOR]

Firefly bioluminescence has attracted great interest because of its high quantum yield and intriguing modifiable colours. Modifications to the structure of the enzyme luciferase can change the emission colour of firefly bioluminescence, and the mechanism of the colour change has been intensively studied by biochemists, structural biologists, optical physicists, and quantum-chemistry theorists. Here, we report on the quantitative spectra of firefly bioluminescence catalysed by wild-type and four site-directed mutant luciferases. While the mutation caused different emission spectra, the spectra differed only in the intensity of the green component (λmax ∼ 560 nm). In contrast, the orange (λmax ∼ 610 nm) and red (λmax ∼ 650 nm) components present in all the spectra were almost unaffected by the modifications to the luciferases and changes in pH. Our results reveal that the intensity of the green component is the unique factor that is influenced by the luciferase structure and other reaction conditions [ABSTRACT FROM AUTHOR]

Intrinsic radiative lifetime is an essential physical property of low-dimensional excitons that represents their optical transition rate and wavefunction, which directly measures the probability of finding an electron and a hole at the same position in an exciton. However, the conventional method that is used to determine this property via measuring the temperature-dependent photoluminescence (PL) decay time involves uncertainty due to various extrinsic contributions at high temperatures. Here, we propose an alternative method to derive the intrinsic radiative lifetime via temperature-independent measurement of the absorption cross section and transformation using Einstein's A-B-coefficient equations derived for low-dimensional excitons. We experimentally verified our approach for one-dimensional (1D) excitons in high-quality 14 × 6 nm2 quantum wires by comparing it to the conventional approach. Both independent evaluations showed good agreement with each other and with theoretical predictions. This approach opens a promising path to studying low-dimensional exciton physics. [ABSTRACT FROM AUTHOR]