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After the Fukushima nuclear accident, the Japanese government implemented extensive decontamination work in 137Cs contaminated catchments for residents' health and local revitalization. Whether dramatic land use changes in the upstream decontaminated regions affected river suspended sediment (SS) and particulate 137Cs discharge downstream remain unknown because of the poor quantification on land cover changes and long-term river SS dynamics. We here introduce a 6-year concurrent database of the Niida River Basin, a decontaminated catchment, including the first available vector decontamination maps, satellite images in decontaminated regions with a spatial resolution of 10 m, and long-term river monitoring datasets spanning decontamination (2013–2016) and subsequent natural restoration stages (2017–2018). These datasets allow us, for the first time, to directly link the transport dynamics of river SS (particulate 137Cs) to land use changes caused by humans in real-time, which provide fundamental data for better understanding the river response of sediment to land use change. Moreover, the data obtained by interdisciplinary methods offer a template for land use change impact assessment in other river basins. [ABSTRACT FROM AUTHOR]

Radiocesium released from the Fukushima Daiichi nuclear power plant (FDNPP) and deposited in the terrestrial environment has been transported to the sea through rivers. To study the long-term effect of riverine transport on the remediation process near the FDNPP, a monitoring project was initiated by the University of Tsukuba. It was commissioned by the Ministry of Education, Culture, Sports, Science, and Technology, and the Nuclear Regulatory Commission in June 2011, and was taken over by the Fukushima Prefectural Centre for Environmental Creation from April 2015. The activity concentration and monthly flux of radiocesium in a suspended form were measured in the project. This provides valuable measurement data to evaluate the impact of the accidentally released radiocesium on residents and the marine environment. It can also be used as verification data in the development and testing of numerical models to predict future impacts. Measurement(s) Cesium-137 Gamma Radiation • Cesium-134 Gamma Radiation • Latitude • Longitude • grain size • radiocesium flux • radioactivity concentration Technology Type(s) gamma-ray spectroscopy • GPS navigation system • laser diffraction particle size analyzer • Calculation Factor Type(s) geographic location Sample Characteristic - Environment suspended sediment Sample Characteristic - Location Abukuma River • Fukushima Prefecture • Miyagi Prefecture Machine-accessible metadata file describing the reported data: https://doi.org/10.6084/m9.figshare.13055315 [ABSTRACT FROM AUTHOR]

Long-term monitoring revealed that radiocesium (137Cs) deposition that fall from the canopy with litterfall was characterized by forest types, seasonal change, and canopy closure (CC). The sum of autumn and spring 137Cs deposition values divided by the sum of summer and winter tended to have higher values in the cedar forest. The angle of view α when the correlation between the CC size and litterfall amount is strongest, was 5° or less in the young cedar forest, but varied in the hardwood–pine mixed forest. This indicates the spatial distribution of 137Cs deposition has heterogeneity and homogeneity in each forest. [ABSTRACT FROM AUTHOR]

Strontium-90 (90Sr) is the major long-lived radionuclide derived from the Chernobyl accident, and is still being detected in the heavily contaminated catchments of the Chernobyl Exclusion Zone. This study examines the long-term decrease in the dissolved-phase 90Sr concentration and the concentration–discharge (90Sr-Q) relationship in stream water since the accident. We show that the slow decline in 90Sr follows a double-exponential function, and that there is a clear relationship between 90Sr and Q. This study is the first to reveal that the log(90Sr)-log(Q) slope has been gradually decreasing since the accident. This trend persists after decay correction. Thus, it is not caused by the physical decay of 90Sr and environmental diffusion, but implies that the concentration formation processes in stream water have been changing over a long period. We propose a hydrochemical model to explain the time-dependency of the 90Sr-Q relationship. This paper presents a mathematical implementation of the new concept and describes the model assumptions. Our model accurately represents both the long-term 90Sr trend in stream water and the time-dependency of the 90Sr-Q relationship. Although this paper considers a small catchment in Chernobyl, the conceptual model is shown to be applicable to other accidental releases of radionuclides. [ABSTRACT FROM AUTHOR]

Although several studies have assessed the effects of thinning on water quality, including nitrogen (N) exports, few have examined N-saturated plantations. This study assessed the short-term effect of thinning on N exports from a N-saturated plantation forest in northern Kyushu, western Japan, that was thinned (43% of basal area) during January–March 2012. Water levels at the gauging station were continually measured, and stream-water baseflow and stormflow samples were collected before (2011) and after (2013) forest thinning. Annual precipitation before (2469 mm) and after (2418 mm) forest thinning differed little, and annual water discharge after thinning (1641 mm) was similar to that before thinning (1609 mm). However, direct flow during stormflow periods was higher after thinning (260 mm) than before (153 mm). The concentrations of major ions in stream water did not differ before and after thinning. As a result, the high annual dissolved inorganic N (DIN) exports differed little before (35.8 kg N ha−1 a−1) and after (36.5 kg N ha−1 a−1) forest thinning. DIN exports during stormflow periods were slightly higher after (12.2 kg N ha−1 a−1) than before thinning (10.5 kg N ha−1 a−1) and were proportional to the increased direct flow after thinning (561 mm after vs. 470 mm before thinning). We concluded that thinning does not affect annual N exports from the N-saturated plantation forest, but it can increase the proportion of N exported during stormflow periods in proportion to increased water volume of direct flow after thinning. [ABSTRACT FROM AUTHOR]

Purpose: Spectrocolourimetric measurements provide a relatively inexpensive, quick and non-destructive alternative to the analysis of geochemical and organic matter properties. When used in the analysis of sediments and their potential sources, these colour parameters may provide important information on the dominant processes (i.e. erosion) occurring in the Critical Zone. Here, they are used to investigate whether eroded sediment is derived from forest (i.e. natural), cultivated (i.e. anthropogenic) or subsoil sources in order to assess their potential to monitor the effect of decontamination in regions impacted by fallout from the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident. Materials and methods: Fifteen spectrocolourimetric properties (L*, a*, b*, C*, h, x, y, z, L, a, b, u*, v*, u', v') were measured in potential source (n = 37) and sediment (n = 400) samples collected during 13 campaigns from 2011 to 2017 after major flood events in two catchments (total surface area of 450 km2) draining the main FDNPP radioactive pollution plume. Potential sources included topsoil from forest and cultivated sources along with subsoil material originating from landslides, channel banks and the decontamination of cultivated areas. The optimum set of parameters used in the mixed linear model to calculate the sediment source contributions was obtained through the use of a range test, the Kruskal–Wallis H test and a linear discriminant analysis. Results and discussion: Nine selected colour parameters correctly classified 100% of the source samples (i.e. forest, subsoil and cultivated sources). The results illustrate that cultivated landscapes were the main source of sediment to these river systems (mean 56%, SD 34%) followed by subsoil (mean 26%, SD 16%) and forest sources (mean 21%, SD 24%). However, these contributions varied strongly over time, with a peak of subsoil contributions (mean 57%, SD 17%) in Fall 2015, coinciding with the occurrence of a typhoon after the remediation works. These results were consistent with monitoring studies conducted in the same area that showed the major impact of typhoon Etau in September 2015 on sediment and radiocaesium fluxes. Conclusions: These original results demonstrate that spectrocolourimetric measurements may contribute to the routine monitoring of the effectiveness of remediation works in this post-accidental context. Owing to the inexpensive, rapid and non-destructive analyses, spectrocolourimetric-based tracing methods have significant potential to provide information on the dominant erosion processes occurring in the Critical Zone. [ABSTRACT FROM AUTHOR]

The Fukushima Dai-ichi nuclear power plant accident released limited amounts of actinides on soils of Japan. Characterisation of these particles is essential to determine the fate of actinides in the environment. The method presented in this paper, based on α-tracks detections, microscope observations and mass-spectrometry measurements, was designed to identify and characterize actinide-bearing particles in soil samples. The method was tested on a road dust sample collected in the main radioactive plume of the Fukushima region. Accordingly, α-tracks detection was demonstrated to provide a powerful technique to localise these particles and prepare their morphological, elemental and isotopic characterization. [ABSTRACT FROM AUTHOR]

Radiocarbon and radiocesium were measured on litter fractions (LF) collected on November 19th, 2011 at 40 km NW of the FDNPP. The 137Cs concentration is much higher in the lower fraction LFb at 226,650 ± 170 Bq kg−1 than in the upper fraction LFa at 7290 ± 40 Bq kg−1. From leaf-air 14C comparison, no excess 14C due to the FDNPP accident is detected in LFa deposited in 2010-2011. A significant 14C difference of 1.4% exists between pine needles and deciduous leaves in LFb, which may be due either to post-depositional processes or to a turnover time of 0.5-1 year of stored carbon for deciduous leaves growth. [ABSTRACT FROM AUTHOR]

Purple soil is highly susceptible for overland flow and surface erosion, therefore understanding surface runoff and soil erosion processes in the purple soil region are important to mitigate flooding and erosion hazards. Slope angle is an important parameter that affects the magnitude of runoff and thus surface erosion in hilly landscapes or bare land area. However, the effect of slope on runoff generation remains unclear in many different soils including Chinese purple soil. The aim of this study was to investigate the relationship between different slope gradients and surface runoff for bare-fallow purple soil, using 5 m × 1.5 m experimental plots under natural rainfall conditions. Four experimental plots (10°, 16°, 20° and 26°) were established in the Yanting Agro-ecological Experimental Station of Chinese Academy of Science in central Sichuan Basin. The plot was equipped with water storage tank to monitor water level change. Field monitoring from July 1 to October 31, 2012 observed 42 rainfall events which produced surface runoff from the experimental plots. These water level changes were converted to runoff. The representative eight rainfall events were selected for further analysis, the relationship between slope and runoff coefficient were determined using ANOVA, F-test, and z-score analysis. The results indicated a strong correlation between rainfall and runoff in cumulative amount basis. The mean value of the measured runoff coefficient for four experimental plots was around 0.1. However, no statistically significant relationship was found between slope and runoff coefficient. We reviewed the relationship between slope and runoff in many previous studies and calculated z-score to compare with our experimental results. The results of z-score analysis indicated that both positive and negative effects of slope on runoff coefficient were obtained, however a moderate gradient (16°-20° in this study) could be a threshold of runoff generation for many different soils including the Chinese purple soil. [ABSTRACT FROM AUTHOR]

Key message: Thinning resulted in evapotranspiration decrease and caused the relative contributions of each component to evapotranspiration to become very close. Abstract: To increase the understanding of forest management to control water cycles, we examined the effect of 50% strip thinning on evapotranspiration (ET) and its partitioning into canopy interception ( E ), tree transpiration ( E ), and forest floor evaporation ( E ) in a Japanese cypress ( Chamaecyparis obtusa Endl.) plantation. Intensive measurements were employed to monitor each component of ET during the pre- and post-thinning periods. The results showed the annual E was the dominant component of ET followed by E , whereas E was the smallest component in both periods. Thinning has significant impact on the process of ET partitioning. In such that it decreased from 42.3 to 33.7% in E /ET and from 45.0 to 34.9% in E /ET, and increased from 12.7 to 31.4% in E /ET on an annual scale. The relative contributions of each ET component to the whole ET became more or less the same after thinning. Additionally, the monthly E / P had relative stable values in both pre- and post-thinning periods, contributing significantly to the ET/ P during heavy rainfall conditions. After thinning, ET decreased by 21.4% from 629.3 to 494.8 mm during the growing season and by 20.4% from 979.8 to 780.1 mm at the annual scale, demonstrating that thinning results in an increase in water availability in the forested watershed. This study can improve the understanding of forest water budget in response to thinning and aid in development of appropriate forest management practices accordingly. [ABSTRACT FROM AUTHOR]

There were two sources of ionizing irradiation after the atomic bombings of Hiroshima and Nagasaki: (1) initial gamma-neutron irradiation at the moment of detonation and (2) residual radioactivity. Residual radioactivity consisted of two components: radioactive fallout containing fission products, including radioactive fissile materials from nuclear device, and neutron-activated radioisotopes from materials on the ground. The dosimetry systems DS86 and DS02 were mainly devoted to the assessment of initial radiation exposure to neutrons and gamma rays, while only brief considerations were given for the estimation of doses caused by residual radiation exposure. Currently, estimation of internal exposure of atomic bomb survivors due to dispersed radioactivity and neutron-activated radioisotopes from materials on the ground is a matter of some interest, in Japan. The main neutron-activated radionuclides in soil dust were Na, Al, Si, P, Cl, K, Ca, Sc, Mn, Fe, Co, and Cs. The radionuclide Mn ( T = 2.58 h) is known as one of the dominant beta- and gamma emitters during the first few hours after neutron irradiation of soil and other materials on ground, dispersed in the form of dust after a nuclear explosion in the atmosphere. To investigate the peculiarities of biological effects of internal exposure to Mn in comparison with external gamma irradiation, a dedicated experiment with Wistar rats exposed to neutron-activated Mn dioxide powder was performed recently by Shichijo and coworkers. The dosimetry required for this experiment is described here. Assessment of internal radiation doses was performed on the basis of measured Mn activity in the organs and tissues of the rats and of absorbed fractions of internal exposure to photons and electrons calculated with the MCNP-4C Monte Carlo using a mathematical rat phantom. The first results of this international multicenter study show that the internal irradiation due to incorporated Mn powder is highly inhomogeneous, and that the most irradiated organs of the experimental animals are: large intestine, small intestine, stomach, and lungs. Accumulated absorbed organ doses were 1.65, 1.33, 0.24, 0.10 Gy for large intestine, small intestine, stomach, and lungs, respectively. Other organs were irradiated at lower dose levels. These results will be useful for interpretation of the biological effects of internal exposure of experimental rats to powdered Mn as observed by Shichijo and coworkers. [ABSTRACT FROM AUTHOR]

We examined changes in suspended-sediment yields (SSY) after a 50 % strip thinning in headwater streams draining a Japanese cedar ( Cryptomeria japonica) and cypress ( Chamaecyparis obtusa) plantation forest. We applied a paired-catchment analysis to treated ( K: 17.1 ha) and control ( K: 8.9 ha) catchments. Annual suspended-sediment yield (SSY) in the prethinning period in the K and K catchments was 110.0 and 142.1 kg/ha per year. For the postthinning period, SSY in the K catchment became 5055.6 kg/ha per year, whereas that in the K catchment increased 893.2 kg/ha per year. The paired-catchment analysis revealed that SSY in the K catchment increased 17.0-fold compared with the prethinning period. However, the dominant hysteresis pattern remained clockwise in both pre- and postthinning periods. Sequences of large storm events in the postthinning period elevated SSY in both catchments. Increase in suspended sediment in the K catchment was associated with the combined impacts of thinning and sequences of storm events during the period of thinning operation. [ABSTRACT FROM AUTHOR]

We collected fluvial suspended sediments in Fukushima after the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident and analyzed the Cs concentration in bulk and size-fractioned samples to investigate the particle-size-dependent distribution of radiocesium. The Cs concentration in bulk suspended sediments decreased from August to December 2011, possibly reflecting a decrease of radiocesium concentration in its source materials. Smaller particles had higher radiocesium concentrations, reflecting larger specific surface areas. Silt- and sand-size fractions occupied more than 95 % of the total Cs in the suspended sediments. The contribution of clay-size fractions, which had the highest Cs concentration, was quite small because of their low frequency. A line of the data showed that the particle size distribution of radiocesium was essential to evaluate the migration and distribution of radiocesium in river systems where radiocesium is mainly present as particulate form after the FDNPP accident. [ABSTRACT FROM AUTHOR]

This study aimed to quantify the flux of radiocesium in the Abukuma Basin (5,172 km2), the largest river system affected by fallout from the Fukushima Daiichi Nuclear Power Plant (FDNPP) event. In the period from 10 August 2011 to 11 May 2012 an estimated 84 to 92% of the total radiocesium transported in the basin's fluvial system was carried in particulate form. During this monitoring period Typhoon Roke (September 2011) was observed to induce a significant and temporally punctuated redistribution of radiocesium. The storm-mobilised radiocesium was an estimated 6.18 Terabecquerels corresponding to 61.4% of the total load delivered to the coastal zone during the observation period. The total flux of radiocesium into the Pacific Ocean estimated at the outlet station (basin area 5,172 km2) was 5.34 TBq for 137Cs, and 4.74 TBq for 134Cs, corresponding to 1.13% of the total estimated radiocesium fallout over the basin catchment (890 TBq). This was equivalent to the estimated amount of direct leakage from FDNPP to the ocean during June 2011 to September 2012 of 17 TBq and the Level 3 Scale Leakage on 21August 2013 (24 TBq). [ABSTRACT FROM AUTHOR]

We analyzed fresh and dead leaves collected in forests in Fukushima after the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident, using autoradiography. Both fresh and dead leaves of Cryptomeria japonica were contaminated by radionuclides (Cs and Cs). Contamination of the fresh leaves was possibly attributed to interception of radionuclides by tree canopies, whereas the dead leaves indicated the direct deposition of radionuclides by fallout and/or washout of radionuclides intercepted by tree canopies. Translocation of radiocesium from a contaminated branch to new leaves growing after the FDNPP accident was not clearly observed, although transfer of radiocesium from leaf parts to male flowers occurred. Fallen leaves of Quercus serrata, which started growing after the FDNPP accident, did not show radioactivity, indicating that significant amounts of translocation from other parts to new leaves did not occur. Fallen leaves of Q. serrata collected from a litter showed hot spots originating from direct fallout. Needles of Pinus densiflora were also contaminated by fallout. Leaching with pure water removed soluble fractions of radiocesium and hot particles from the surface of the contaminated leaves, but significant amounts of radioactivity remained. This means that foliar absorption occurred in both fresh and dead leaves. Further leaching experiments using surfactant and acetone could not remove the remaining radiocesium from the leaves. The leaching experiments indicate that radiocesium in the contaminated leaves is strongly fixed in leaf tissues and is not readily released unless leaf tissues are decomposed. [ABSTRACT FROM AUTHOR]

A low-cost and simple monitoring method for early warning of landslides is proposed. To detect abnormal deformation of a slope, this method employs a tilt sensor in place of an extensometer on the slope surface. In order to examine the relevance of measuring rotation angle on a slope surface by tilt sensor, model tests were conducted, and rotation on the slope surface was observed together with slide displacement along the surface. The rotation data responded 30 min before failure in a model test, which could be useful as a signal for early warning. However, the behavior of rotation before failure varies from case to case, and thus, criteria to issue warning should be defined more carefully. For a model slope made of uniform loose sand, measurement of slide displacement along the slope surface is sensitive to failure at the toe, while the measurement of rotation on the slope surface is useful to detect the development of progressive failure upward along the slope. Wireless sensor units with microelectromechanical systems (MEMS) tilt sensor and volumetric water content sensor were also examined on a real slope in Kobe City, and a long-term monitoring was attempted. A simple but possible way to define the criteria of judgment to issue warning can be proposed based on combination of data obtained by the tilt sensors and volumetric water content sensors. [ABSTRACT FROM AUTHOR]

Despite continued interest in stream water temperature (Tw) analysis, there are few studies of Tw response to rainfall events at forested watersheds. We examined 61 sets of data on Tw for 21 rainfall events at 16 watersheds with various slope gradients (from 0.08 to 0.56) in four regions of Japan from June 2004 to December 2005. The investigation focused on the changes of specific discharge (ΔQs) and ΔTw at medium-sized watersheds (0.5–100 ha). The results clearly demonstrated different flow patterns expressed by Qs vs. Tw hysteretic loops. Those were clockwise in Period I (April–September) and counterclockwise in Period II (October–March), except for lower slope gradient at Aichi, where counterclockwise loops were observed in both periods. These differences in hysteretic loops could be explained by the differences in Tw and in response times to rainfall between surface/subsurface and groundwater flows. The response times were probably determined by the slope gradient and the vertical level of groundwater. We also found that the changes in air temperature (ΔTa) influenced ΔTw to a lesser degree than Qs. The average rainfall intensities in Period I and Period II (9.3 ± 1.7 and 5.4 ± 0.2 mm/h, respectively) affected the average values of ΔQs and ΔTw (6.62 ± 4.08 mm/h and 1.7 ± 0.4°C; 0.85 ± 0.68 mm/h and 0.9 ± 0.3°C, respectively). This indicates that slope gradient and Qs influenced ΔTw by changing the relative proportions of flow paths. In addition, the water table changes influenced the percentage of groundwater flow to the stream. [ABSTRACT FROM AUTHOR]

It is the conventional understanding that rain removes aerosols from the atmosphere. However, the question of whether rain plays a role in releasing aerosols to the atmosphere has recently been posed by several researchers. In the present study, we show additional evidence for rain-induced aerosol emissions in a forest environment: the occurrence of radiocaesium-bearing aerosols in a Japanese forest due to rain. We carried out general radioactive aerosol observations in a typical mountainous village area within the exclusion zone in Fukushima Prefecture to determine the impacts and major drivers of the resuspension of radiocaesium originating from the nuclear accident in March 2011. We also conducted sampling according to the weather (with and without rain conditions) in a forest to clarify the sources of atmospheric radiocaesium in the polluted forest. We found that rain induces an increase in radiocaesium in the air in forests. With further investigations, we confirmed that the fungal spore sources of resuspended radiocaesium seemed to differ between rainy weather and nonrainy weather. Larger fungal particles (possibly macroconidia) are emitted during rainy conditions than during nonrainy weather, suggesting that splash generation by rain droplets is the major mechanism of the suspension of radiocaesium-bearing mould-like fungi. The present findings indicate that radiocaesium could be used as a tracer in such research fields as forest ecology, meteorology, climatology, public health and agriculture, in which fungal spores have significance. [ABSTRACT FROM AUTHOR]

Our study focused on radiocaesium (137Cs) partitioning in forests, three vegetation periods after the Fukushima Daiichi nuclear power plant accident. 137Cs distribution in forest components (organic and mineral soil layers as well as tree compartments: stem, bark, needles, branches and roots) was measured for two Japanese cedar stand ages (17 and 33 years old). The results showed that around 85% of the initial deposit was found in the forest floor and topsoil. For the youngest stand almost 70% of the deposit is present in the forest floor, whereas for the oldest stand 50% is present in the 0-3 cm mineral soil layer. For trees, old and perennial organs (including dead and living needles and branches, litter fall and outer bark) directly exposed to the fallout remained the most contaminated. The crown concentrated 61-69% of the total tree contamination. Surprisingly the dead organs concentrated 25 ± 9% (young cedars) to 36 ± 20% (mature cedar) of the trees' residual activity, highlighting the importance of that specific compartment in the early post-accident phase for Japanese cedar forests. Although the stem (including bark) represents the highest biomass pool, it only concentrates 3.3% and 4.6% of the initial 137Cs deposit for mature and young cedars, respectively. [ABSTRACT FROM AUTHOR]