1. Oxidative Molecular Layer Deposition Tailoring Eco-Mimetic Nanoarchitecture to Manipulate Electromagnetic Attenuation and Self-Powered Energy Conversion.
- Author
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Shu, Jin-Cheng, Zhang, Yan-Lan, Qin, Yong, and Cao, Mao-Sheng
- Subjects
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ENERGY conversion , *ELECTROMAGNETIC devices , *ELECTROMAGNETIC radiation , *ELECTROMAGNETIC pulses , *AEROSPACE engineering , *AEROSPACE engineers , *WASTE recycling - Abstract
Highlights: Drawing wisdom and inspiration from nature, an eco-mimetic nanoarchitecture is constructed, featuring tunable electromagnetic properties and high-efficiency energy attenuation. Through in-depth insight into the microstructure, the material basis of electromagnetic response is clearly revealed to establish an intrinsic connection between microscopic electronic structure and macroscopic electromagnetic properties. A creative self-powered energy conversion device is constructed, with the integrated functions including electromagnetic protection and waste energy recycling, which offers a new horizon for the fields of energy and environment. Advanced electromagnetic devices, as the pillars of the intelligent age, are setting off a grand transformation, redefining the structure of society to present pluralism and diversity. However, the bombardment of electromagnetic radiation on society is also increasingly serious along with the growing popularity of "Big Data". Herein, drawing wisdom and inspiration from nature, an eco-mimetic nanoarchitecture is constructed for the first time, highly integrating the advantages of multiple components and structures to exhibit excellent electromagnetic response. Its electromagnetic properties and internal energy conversion can be flexibly regulated by tailoring microstructure with oxidative molecular layer deposition (oMLD), providing a new cognition to frequency-selective microwave absorption. The optimal reflection loss reaches ≈ − 58 dB, and the absorption frequency can be shifted from high frequency to low frequency by increasing the number of oMLD cycles. Meanwhile, a novel electromagnetic absorption surface is designed to enable ultra-wideband absorption, covering almost the entire K and Ka bands. More importantly, an ingenious self-powered device is constructed using the eco-mimetic nanoarchitecture, which can convert electromagnetic radiation into electric energy for recycling. This work offers a new insight into electromagnetic protection and waste energy recycling, presenting a broad application prospect in radar stealth, information communication, aerospace engineering, etc. [ABSTRACT FROM AUTHOR]
- Published
- 2023
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