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Novel horizontal-type time-of-flight neutron reflectometer SOFIA (SOFt Interface Analyzer) was installed in BL 16 of Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex (J-PARC). The design and performance of SOFIA reflectometer was described based on the preliminary results of the neutron reflectivity (NR) measurements of deuterated polystyrene (d-PS) thin films, Langmuir–Blodgett film and at deuterium oxide/ polymer brush interfaces. Time-resolved in-situ NR measurement at 1-min intervals was also demonstrated to observe interfacial mixing of d-PS on the PS brush surface during annealing.

Neutron reflectometry is a powerful method for investigating the surface and interfacial structures of materials in the spatial range from nanometers to sub-micrometers. At the Japan Proton Accelerator Research Complex (J-PARC), a high-intensity pulsed neutron beam is produced with a proton accelerator at 220kW, which will be upgraded to 1MW in future. Beamline 16 (BL16) at the Materials and Life Science Experimental Facility (MLF) in J-PARC is dedicated to a horizontal-type reflectometer, and in this beamline, neutrons are transported downward at two different angles, 2.2° and 5.7° , relative to the horizontal. In December 2008, we started to accept the neutron beam at BL16 with the old ARISA reflectometer relocated from the KENS facility, KEK, Japan; and we have now replaced it with the brand-new reflectometer SOFIA (SOFt Interface Analyzer). With a high-flux beam and instrumental upgrade, the observable reflectivity of SOFIA reaches around 10−7 within a few hours for specimens on 3” substrates. In this paper, we will present the design and performance of the SOFIA reflectometer, and discuss some preliminary results on the device development for further upgrade.