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1. Crystal Engineering of an nbo Topology Metal-Organic Framework for Chemical Fixation of CO2 under Ambient Conditions.

Author

Gao, Wen‐Yang, Chen, Yao, Niu, Youhong, Williams, Kia, Cash, Lindsay, Perez, Pastor J., Wojtas, Lukasz, Cai, Jianfeng, Chen, Yu‐Sheng, and Ma, Shengqian

Subjects
*CRYSTALS, *METAL-organic frameworks, *CARBON dioxide, *AMBIENT conditions (Electronics), *CARBON sequestration, *CATALYTIC activity
Abstract

Crystal engineering of the nbo metal-organic framework (MOF) platform MOF-505 with a custom-designed azamacrocycle ligand (1,4,7,10-tetrazazcyclododecane- N, N′, N′′, N′′′-tetra- p-methylbenzoic acid) leads to a high density of well-oriented Lewis active sites within the cuboctahedral cage in MMCF-2, [Cu2(Cu-tactmb)(H2O)3(NO3)2]. This MOF demonstrates high catalytic activity for the chemical fixation of CO2 into cyclic carbonates at room temperature under 1 atm pressure. [ABSTRACT FROM AUTHOR]

Published
2014
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