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High-purity Ge-As-Se and Ge-As-S chalcogenide glasses were prepared by modified physical and chemical purification techniques. Using the purified glasses, step-index fibers with a small core (~5.5 μm) and large numerical aperture (~1.3) were fabricated. When a 13.5-cm-long fiber was pumped with 320 fs pulses at a repetition rate of 10.5 MHz at 4.1 μm, supercontinuum spanning from ~1.8 to ~9.8 μm with a dynamic range of ±10 dB and an average power of ~3 mW was generated. [ABSTRACT FROM AUTHOR]