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Flexible hybrid electronic (FHE) materials and devices exploit the interaction of mechanical and electromagnetic properties to operate in new form factors and loading environments, which are key for advancing wearable sensors, flexible antennas, and soft robotic skin technologies. Dielectric elastomer (DE) architectures offer a novel substrate material for this application space as they are a class of strain‐tolerant and programmable metamaterials that derive their mechanical and dielectric properties from their architecture. Due to their hyperelasticity, dielectric elastomers can leverage reversible finite deformation to physically reconfigure their internal architecture to repeatedly tune their material behavior. Here a combined computational and experimental study of two dielectric elastomer architectures, based on square and hexagonal unit cell periodicities are presented. A shift in effective permittivity is observed due to the relative increase in matrix volume and the rearrangement of the electric field distribution in the cells. Additive fabrication allows rapid unit cell geometry customization for tuning the electromechanical response of the architectures. Effective permittivity shifts Δε2 > 0.7 under compressive strains of 35% are observed. The practical utility of this strain‐tunable permittivity is demonstrated in a microstrip patch antenna, which exhibits shifts in resonance frequency greater than 110 MHz when the dielectric elastomer substrate is compressed. [ABSTRACT FROM AUTHOR]

This paper presents a method to achieve high deformability levels in dielectric elastomer actuators (DEAs) by applying a modulated voltage waveform. The method relies on supplying the electrostatic energy during the specific phase of the oscillation cycle, resulting in the enhanced travel range at a relatively low driving voltage. We consider a standard sandwich configuration of the DE actuator with neo-Hookean material model and outline an energy-based approach for delineating the underlying principles of the proposed method. A comparison of the deformability levels achieved using the quasi-static, Heaviside step, and the modulated input waveforms is presented. Significant reduction in instability voltages together with a considerable increase in the stable actuation limit is observed in the case of the modulated voltage input. The estimates of the stability thresholds are validated by integrating the equation of motion obtained using Hamilton's principle. The effect of energy dissipation is assessed by considering variations in the quality factor. Further, a qualitative comparison with experimental observations is presented highlighting the practical feasibility of the method. This investigation can find its potential use in the design and development of DEAs subjected to a time-dependent motion. [ABSTRACT FROM AUTHOR]

Polymer-based three-dimensional (3D) printing—such as the UV-assisted layer-by-layer polymerization technique—enables fabrication of deformable microstructured materials with pre-designed properties. However, the properties of such materials require careful characterization. Thus, for example, in the polymerization process, a new interphase zone is formed at the boundary between two constituents. This article presents a study of the interphasial transition zone effect on the elastic instability phenomenon in hyperelastic layered composites. In this study, three different types of the shear modulus distribution through the thickness of the interphasial layer were considered. Numerical Bloch-Floquet analysis was employed, superimposed on finite deformations to detect the onset of instabilities and the associated critical wavelength. Significant changes in the buckling behavior of the composites were observed because of the existence of the interphasial inhomogeneous layers. Interphase properties influence the onset of instabilities and the buckling patterns. Numerical simulations showed that interlayer inhomogeneity may result in higher stability of composites with respect to classical layup constructions of identical shear stiffness. Moreover, we found that the critical wavelength of the buckling mode can be regulated by the inhomogeneous interphase properties. Finally, a qualitative illustration of the effect is presented for 3D-printed deformable composites with varying thickness of the stiff phase. [ABSTRACT FROM AUTHOR]