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Data assimilation of satellite microwave measurements is one of the importantkeys to improving weather forecasting over the Arctic region. However, the useofsurface-sensitivemicrowave-soundingchannelmeasurementsfordataassim-ilation or retrieval has been limited, especially during winter, due to the poorlyconstrained sea ice emissivity. In this study, aiming at more use of those channelmeasurements in the data assimilation, we propose an explicit method for speci-fying the surface radiative boundary conditions (namely emissivity and emittinglayer temperature of snow and ice). These were explicitly determined with aradiativetransfermodelforsnowandiceandwithsnow/icephysicalparameters(i.e. snow/ice depths and vertical distributions of temperature, density, salinity,and grain size) simulated from the thermodynamically driven snow/ice growthmodel. We conducted 1D-Var experiments in order to examine whether thisapproach can help to use the surface-sensitive microwave temperature channelmeasurements over the Arctic sea ice region for data assimilation. Results showthat (1) the surface-sensitive microwave channels can be used in the 1D-Varretrieval, and (2) the specification of the radiative boundary condition at thesurface using the snow/sea ice emission model can significantly improve theatmospheric temperature retrieval, especially in the lower troposphere (500hPato surface). The successful retrieval suggests that useful information can beextracted from surface-sensitive microwave-sounding channel radiances oversea ice surfaces through the explicit determination of snow/ice emissivity andemitting layer temperature.

The Arctic is warming faster than the global average and any other region of a similar size. One important factor in this is the poleward atmospheric transport of heat and moisture, which contributes directly to the surface and air warming. In this case study, the atmospheric circulation and spatio-temporal structure of a moisture intrusion event is assessed, which occurred from 5 to 7 June 2017 over the Nordic seas during an intensive measurement campaign over Svalbard. This analysis focuses on high-spatial-resolution simulations with the ICON (ICOsahedral Non-hydrostatic) model which is put in context with coarser-resolution runs as well the ERA5 reanalysis. A variety of observations including passive microwave satellite measurements is used for evaluation. The global operational ICON forecasts from the Deutscher Wetterdienst (DWD) at 13 km horizontal resolution are used to drive high-resolution Limited-Area Mode (LAM) ICON simulations over the Arctic with 6 and 3 km horizontal resolutions. The results show the skilful capacity of the ICON-LAM model to represent the observed spatio-temporal structure of the selected moisture intrusion event and its signature in the temperature, humidity and wind profiles, and surface radiation. In several aspects, the high-resolution simulations offer a higher accuracy than the global simulations and the ERA5 reanalysis when evaluated against observations. One feature where the high-resolution simulations demonstrated an advanced skill is the representation of the changing vertical structure of specific humidity and wind associated with the moisture intrusion passing Ny-Ålesund (western Svalbard); the humidity increase at 1–2 km height topped by a dry layer and the development of a low-level wind jet are best represented by the 3 km simulation. The study also demonstrates that such moisture intrusions can have a strong impact on the radiative and turbulent heat fluxes at the surface. A drastic decrease in downward shortwave radiat

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore cross-cutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system

Fram Strait in the northern North Atlantic is a key region for marine cold air outbreaks (MCAOs), southward discharges of polar air under northerly air flow, which have a strong impact on air-sea heat fluxes, boundary layer processes and severe weather. This study investigates climatologies and decadal trends of Fram Strait MCAOs of different intensity classes based on the ERA5 reanalysis product for 1979–2020. Among striking interannual variability, it is shown that the main MCAO season is December through March, when MCAOs occur around 2/3 of the time. We report on significant decadal MCAO decreases in December and January, and a significant increase in March. While the mid-winter decrease is mainly related to the different paces of warming between the surface and the lower atmosphere, the increase in March can be related to changes in synoptic circulation patterns. As an explanation for the latter, a possible feedback between retreating Barents Sea sea ice, enhanced cyclonic activity and Fram Strait MCAOs is postulated. Exemplifying the trend toward stronger MCAOs during March, the study details the recordbreaking MCAO season in early 2020, and an observational case study of an extreme MCAO event in March 2020 is conducted. Thereby, radiosonde observations are combined with kinematic air back-trajectories to provide rare observational evidence for the diabatic cooling and drying during the MCAO preconditioning phase.

This article presents a comprehensive analysis of the foehn episode which occurred over Svalbard on 30–31 May 2017. This episode is well documented by multiplatform measurements carried out during the Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) and Physical feedbacks of Arctic PBL, Sea ice, Cloud And AerosoL (PASCAL) campaigns. Both orographic wind modification and foehn warming are considered here. The latter is found to be primarily produced by the isentropic drawdown, which is evident from observations and mesoscale numerical modeling. The structure of the observed foehn warming was in many aspects very similar to that for foehns over the Antarctic Peninsula. In particular, it is found that the warming was proportional to the height of the mountain ridges and propagated far downstream. Also, a strong spatial heterogeneity of the foehn warming was observed with a clear cold footprint associated with gap flows along the mountain valleys and fjords. On the downstream side, a shallow stably stratified boundary layer below a well-mixed layer formed over the snow-covered land and cold open water. The foehn warming downwind of Svalbard strengthened the north–south horizontal temperature gradient across the ice edge near the northern tip of Svalbard. This suggests that the associated baroclinicity might have strengthened the observed northern tip jet. A positive daytime radiative budget on the surface, increased by the foehn clearance, along with the downward sensible heat flux provoked accelerated snowmelt in the mountain valleys in Ny-Ålesund and Adventdalen, which suggests a potentially large effect of the frequently observed Svalbard foehns on the snow cover and the glacier heat and mass balance.

Recently, a significant increase in the atmospheric moisture content has been documented over the Arctic, where both local contributions and poleward moisture transport from lower latitudes can play a role. This study focuses on the anomalous moisture transport events confined to long and narrow corridors, known as atmospheric rivers (ARs), which are expected to have a strong influence on Arctic moisture amounts, precipitation, and the energy budget. During two concerted intensive measurement campaigns – Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) and the Physical feedbacks of Arctic planetary boundary layer, Sea ice, Cloud and AerosoL (PASCAL) – that took place at and near Svalbard, three high-water-vapour-transport events were identified as ARs, based on two tracking algorithms: the 30 May event, the 6 June event, and the 9 June 2017 event. We explore the temporal and spatial evolution of the events identified as ARs and the associated precipitation patterns in detail using measurements from the French (Polar Institute Paul Emile Victor) and German (Alfred Wegener Institute for Polar and Marine Research) Arctic Research Base (AWIPEV) in Ny-Ålesund, satellite-borne measurements, several reanalysis products (the European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Analysis (ERA) Interim (ERA-Interim); the ERA5 reanalysis; the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2); the Climate Forecast System version 2 (CFSv2); and the Japanese 55-Year Reanalysis (JRA-55)), and the HIRHAM regional climate model version 5 (HIRHAM5). Results show that the tracking algorithms detected the events differently, which is partly due to differences in the spatial and temporal resolution as well as differences in the criteria used in the tracking algorithms. The first event extended from western Siberia to Svalbard, caused mixed-phase precipitation, and was associated with a retreat of the sea-ice edge.

Recently, a significant increase in the atmospheric moisture content has been documented over the Arctic, where both local contributions and poleward moisture transport from lower latitudes can play a role. This study focuses on the anomalous moisture transport events confined to long and narrow corridors, known as atmospheric rivers (ARs), which are expected to have a strong influence on Arctic moisture amounts, precipitation, and the energy budget. During two concerted intensive measurement campaigns - Arctic CLoud Observations Using airborne measurements during polar Day (ACLOUD) and the Physical feedbacks of Arctic planetary boundary layer, Sea ice, Cloud and AerosoL (PASCAL) - that took place at and near Svalbard, three high-water-vapour-transport events were identified as ARs, based on two tracking algorithms: the 30 May event, the 6 June event, and the 9 June 2017 event. We explore the temporal and spatial evolution of the events identified as ARs and the associated precipitation patterns in detail using measurements from the French (Polar Institute Paul Emile Victor) and German (Alfred Wegener Institute for Polar and Marine Research) Arctic Research Base (AWIPEV) in Ny-angstrom lesund, satellite-borne measurements, several reanalysis products (the European Centre for Medium-Range Weather Forecasts (ECMWF) Re-Analysis (ERA) Interim (ERA-Interim); the ERA5 reanalysis; the Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2); the Climate Forecast System version 2 (CFSv2); and the Japanese 55-Year Reanalysis (JRA-55)), and the HIRHAM regional climate model version 5 (HIRHAM5). Results show that the tracking algorithms detected the events differently, which is partly due to differences in the spatial and temporal resolution as well as differences in the criteria used in the tracking algorithms. The first event extended from western Siberia to Svalbard, caused mixed-phase precipitation, and was associated with a retreat of the sea-i

With the Arctic rapidly changing, the needs to observe, understand, and model the changes are essential. To support these needs, an annual cycle of observations of atmospheric properties, processes, and interactions were made while drifting with the sea ice across the central Arctic during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) expedition from October 2019 to September 2020. An international team designed and implemented the comprehensive program to document and characterize all aspects of the Arctic atmospheric system in unprecedented detail, using a variety of approaches, and across multiple scales. These measurements were coordinated with other observational teams to explore crosscutting and coupled interactions with the Arctic Ocean, sea ice, and ecosystem through a variety of physical and biogeochemical processes. This overview outlines the breadth and complexity of the atmospheric research program, which was organized into 4 subgroups: atmospheric state, clouds and precipitation, gases and aerosols, and energy budgets. Atmospheric variability over the annual cycle revealed important influences from a persistent large-scale winter circulation pattern, leading to some storms with pressure and winds that were outside the interquartile range of past conditions suggested by long-term reanalysis. Similarly, the MOSAiC location was warmer and wetter in summer than the reanalysis climatology, in part due to its close proximity to the sea ice edge. The comprehensiveness of the observational program for characterizing and analyzing atmospheric phenomena is demonstrated via a winter case study examining air mass transitions and a summer case study examining vertical atmospheric evolution. Overall, the MOSAiC atmospheric program successfully met its objectives and was the most comprehensive atmospheric measurement program to date conducted over the Arctic sea ice. The obtained data will support a broad range of coupled-system s

The Arctic is very susceptible to climate change and thus is warming much faster than the rest of the world. Clouds influence terrestrial and solar radiative fluxes and thereby impact the amplified Arctic warming. The partitioning of thermodynamic phases (i.e., ice crystals and water droplets) within mixed-phase clouds (MPCs) especially influences their radiative properties. However, the processes responsible for ice crystal formation remain only partially characterized. In particular, so-called secondary ice production (SIP) processes, which create supplementary ice crystals from primary ice crystals and the environmental conditions that they occur in, are poorly understood. The microphysical properties of Arctic MPCs were measured during the Ny-& Aring;lesund AeroSol Cloud ExperimENT (NASCENT) campaign to obtain a better understanding of the atmospheric conditions favorable for the occurrence of SIP processes. To this aim, the in situ cloud microphysical properties retrieved by a holographic cloud imager mounted on a tethered balloon system were complemented by ground-based remote sensing and ice-nucleating particle measurements. During the 6 d investigated in this study, SIP occurred during about 40 % of the in-cloud measurements, and high SIP events with number concentrations larger than 10 L-1 of small pristine ice crystals occurred in 4 % of the in-cloud measurements. This demonstrates the role of SIP for Arctic MPCs. The highest concentrations of small pristine ice crystals were produced at temperatures between -5 and -3 ?C and were related to the occurrence of supercooled large droplets freezing upon collision with ice crystals. This suggests that a large fraction of ice crystals in Arctic MPCs are produced via the droplet-shattering mechanism. From evaluating the ice crystal images, we could identify ice-ice collision as a second SIP mechanism that dominated when fragile ice crystals were observed. Moreover, SIP occurred over a large temperature range and w

During the 1-year MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition, the German icebreaker Polarstern drifted through Arctic Ocean ice from October 2019 to May 2020, mainly at latitudes between 85 and 88.5∘ N. A multiwavelength polarization Raman lidar was operated on board the research vessel and continuously monitored aerosol and cloud layers up to a height of 30 km. During our mission, we expected to observe a thin residual volcanic aerosol layer in the stratosphere, originating from the Raikoke volcanic eruption in June 2019, with an aerosol optical thickness (AOT) of 0.005–0.01 at 500 nm over the North Pole area during the winter season. However, the highlight of our measurements was the detection of a persistent, 10 km deep aerosol layer in the upper troposphere and lower stratosphere (UTLS), from about 7–8 to 17–18 km height, with clear and unambiguous wildfire smoke signatures up to 12 km and an order of magnitude higher AOT of around 0.1 in the autumn of 2019. Case studies are presented to explain the specific optical fingerprints of aged wildfire smoke in detail. The pronounced aerosol layer was present throughout the winter half-year until the strong polar vortex began to collapse in late April 2020. We hypothesize that the detected smoke originated from extraordinarily intense and long-lasting wildfires in central and eastern Siberia in July and August 2019 and may have reached the tropopause layer by the self-lifting process. In this article, we summarize the main findings of our 7-month smoke observations and characterize the aerosol in terms of geometrical, optical, and microphysical properties. The UTLS AOT at 532 nm ranged from 0.05–0.12 in October–November 2019 and 0.03–0.06 during the main winter season. The Raikoke aerosol fraction was estimated to always be lower than 15 %. We assume that the volcanic aerosol was above the smoke layer (above 13 km height). As an unambiguous sign of the dominance of smoke

Within the transpolar drifting expedition MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate), the Global Navigation Satellite System (GNSS) was used among other techniques to monitor variations in atmospheric water vapor. Based on 15 months of continuously tracked GNSS data including GPS, GLONASS and Galileo, epoch-wise coordinates and hourly zenith total delays (ZTDs) were determined using a kinematic precise point positioning (PPP) approach. The derived ZTD values agree to 1.1 ± 0.2 mm (root mean square (rms) of the differences 10.2 mm) with the numerical weather data of ECMWF's latest reanalysis, ERA5, computed for the derived ship's locations. This level of agreement is also confirmed by comparing the on-board estimates with ZTDs derived for terrestrial GNSS stations in Bremerhaven and Ny-Ålesund and for the radio telescopes observing very long baseline interferometry in Ny-Ålesund. Preliminary estimates of integrated water vapor derived from frequently launched radiosondes are used to assess the GNSS-derived integrated water vapor estimates. The overall difference of 0.08 ± 0.04 kg m−2 (rms of the differences 1.47 kg m−2) demonstrates a good agreement between GNSS and radiosonde data. Finally, the water vapor variations associated with two warm-air intrusion events in April 2020 are assessed.

Water vapor is an important component in the water and energy cycle of the Arctic. Especially in light of Arctic amplification, changes in water vapor are of high interest but are difficult to observe due to the data sparsity of the region. The ACLOUD/PASCAL campaigns performed in May/June 2017 in the Arctic North Atlantic sector offers the opportunity to investigate the quality of various satellite and reanalysis products. Compared to reference measurements at R/V Polarstern frozen into the ice (around 82∘ N, 10∘ E) and at Ny-Ålesund, the integrated water vapor (IWV) from Infrared Atmospheric Sounding Interferometer (IASI) L2PPFv6 shows the best performance among all satellite products. Using all radiosonde stations within the region indicates some differences that might relate to different radiosonde types used. Atmospheric river events can cause rapid IWV changes by more than a factor of 2 in the Arctic. Despite the relatively dense sampling by polar-orbiting satellites, daily means can deviate by up to 50 % due to strong spatio-temporal IWV variability. For monthly mean values, this weather-induced variability cancels out, but systematic differences dominate, which particularly appear over different surface types, e.g., ocean and sea ice. In the data-sparse central Arctic north of 84∘ N, strong differences of 30 % in IWV monthly means between satellite products occur in the month of June, which likely result from the difficulties in considering the complex and changing surface characteristics of the melting ice within the retrieval algorithms. There is hope that the detailed surface characterization performed as part of the recently finished Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) will foster the improvement of future retrieval algorithms.

An advanced multiwavelength polarization Raman lidar was operated aboard the icebreaker Polarstern during the MOSAiC (Multidisciplinary drifting Observatory for the Study of Arctic Climate) expedition to continuously monitor aerosol and cloud layers in the central Arctic up to 30 km height. The expedition lasted from September 2019 to October 2020 and measurements were mostly taken between 85 and 88.5∘ N. The lidar was integrated into a complex remote-sensing infrastructure aboard the Polarstern. In this article, novel lidar techniques, innovative concepts to study aerosol–cloud interaction in the Arctic, and unique MOSAiC findings will be presented. The highlight of the lidar measurements was the detection of a 10 km deep wildfire smoke layer over the North Pole region between 7–8 km and 17–18 km height with an aerosol optical thickness (AOT) at 532 nm of around 0.1 (in October–November 2019) and 0.05 from December to March. The dual-wavelength Raman lidar technique allowed us to unambiguously identify smoke as the dominating aerosol type in the aerosol layer in the upper troposphere and lower stratosphere (UTLS). An additional contribution to the 532 nm AOT by volcanic sulfate aerosol (Raikoke eruption) was estimated to always be lower than 15 %. The optical and microphysical properties of the UTLS smoke layer are presented in an accompanying paper (Ohneiser et al., 2021). This smoke event offered the unique opportunity to study the influence of organic aerosol particles (serving as ice-nucleating particles, INPs) on cirrus formation in the upper troposphere. An example of a closure study is presented to explain our concept of investigating aerosol–cloud interaction in this field. The smoke particles were obviously able to control the evolution of the cirrus system and caused low ice crystal number concentration. After the discussion of two typical Arctic haze events, we present a case study of the evolution of a long-lasting mixed-phase cloud layer embedded in Ar

A cloud particle sensor (CPS) sonde is an observing system attached with a radiosonde sensor to observe the vertical structure of cloud properties. The signals obtained from CPS sondes are related to the phase, size, and number of cloud particles. The system offers economic advantages including human resource and simple operation costs compared with aircraft measurements and land-/satellite-based remote sensing. However, the observed information should be appropriately corrected because of several uncertainties. Here we made field experiments in the Arctic region by launching approximately 40 CPS sondes between 2018 and 2020. Using these data sets, a better practical correction method was proposed to exclude unreliable data, estimate the effective cloud water droplet radius, and determine a correction factor for the total cloud particle count. We apply this method to data obtained in October 2019 over the Arctic Ocean and March 2020 at Ny-Ålesund, Svalbard, Norway, to compare with a particle counter aboard a tethered balloon and liquid water content retrieved by a microwave radiometer. The estimated total particle count and liquid water content from the CPS sondes generally agree with those data. Although further development and validation of CPS sondes based on dedicated laboratory experiments would be required, the practical correction approach proposed here would offer better advantages in retrieving quantitative information on the vertical distribution of cloud microphysics under the condition of a lower number concentration.

SynopSys plans to exploits routine meteorological weather observations from the MOSAiC expedition, remote sensing data products, and meteorological forecast data to detect and characterize synoptic events in the Arctic and evaluate their influence on mid-latitudes. We implement a diagnostic framework that will advance our knowledge on dynamical processes in the coupled troposphere-stratosphere system. Our approach is based on the reciprocal analysis of observations and models. A particular focus lies in the evaluation of enhanced predictive capability through a synergistic and unique set of measurements in the Arctic and a better representation of physical processes in weather forecast models. As well documented, the Arctic region is undergoing rapid change in a warming climate. This has many implications for mid-latitude climate and consequently on the future social, economic, and political development in both regions. Improving weather forecast taking into account the coupling of the Artic and mid-latitudes is thus essential.

The occurrence of events with increased and decreased integrated water vapor (IWV) at the Arctic site Ny-Alesund, their relation to cloud properties, and the surface cloud radiative effect (CRE) is investigated. For this study, we used almost 2.5 years (from June 2016 to October 2018) of ground-based cloud observations processed with the Cloudnet algorithm, IWV from a microwave radiometer (MWR), long-term radiosonde observations, and backward trajectories FLEXTRA. Moist and dry anomalies were found to be associated with North Atlantic flows and air transport within the Arctic region, respectively. The amount of water vapor is often correlated to cloud occurrence, presence of cloud liquid water, and liquid water path (LWP) and ice water path (IWP). In turn, changes in the cloud properties cause differences in surface CRE. During dry anomalies, in autumn, winter, and spring, the mean net surface CRE was lower by 2-37 W M-2 with respect to normal conditions, while in summer the cloud-related surface cooling was reduced by 49 W m(-2). In contrast, under moist conditions in summer the mean net surface CRE becomes more negative by 25 W m(-2), while in other seasons the mean net surface CRE was increased by 5-37 W m(-2). Trends in the occurrence of dry and moist anomalies were analyzed based on a 25-year radiosonde database. Dry anomalies have become less frequent, with rates for different seasons ranging from -12.8 % per decade to -4 % per decade, while the occurrence of moist events has increased at rates from 2.8 % per decade to 6.4 % per decade.

Low-level mixed-phase clouds (MPCs) are common in the Arctic. Both local and large-scale phenomena influence the properties and lifetime of MPCs. Arctic fjords are characterized by complex terrain and large variations in surface properties. Yet, not many studies have investigated the impact of local boundary layer dynamics and their relative importance on MPCs in the fjord environment. In this work, we used a combination of ground-based remote sensing instruments, surface meteorological observations, radiosoundings, and reanalysis data to study persistent low-level MPCs at Ny-Alesund, Svalbard, for a 2.5-year period. Methods to identify the cloud regime, surface coupling, and regional and local wind patterns were developed. We found that persistent low-level MPCs were most common with westerly winds, and the westerly clouds had a higher mean liquid (42 g m(-2)) and ice water path (16 g m(-2)) compared to those with easterly winds. The increased height and rarity of persistent MPCs with easterly free-tropospheric winds suggest the island and its orography have an influence on the studied clouds. Seasonal variation in the liquid water path was found to be minimal, although the occurrence of persistent MPCs, their height, and their ice water path all showed notable seasonal dependency. Most of the studied MPCs were decoupled from the surface (63 %-82 % of the time). The coupled clouds had 41 % higher liquid water path than the fully decoupled ones. Local winds in the fjord were related to the frequency of surface coupling, and we propose that katabatic winds from the glaciers in the vicinity of the station may cause clouds to decouple. We concluded that while the regional to large-scale wind direction was important for the persistent MPC occurrence and properties, the local-scale phenomena (local wind patterns in the fjord and surface coupling) also had an influence. Moreover, this suggests that local boundary layer processes should be described in models in order to p

In the Antarctic ozone hole, ozone mixing ratios have been decreasing to extremely low values of 0.01–0.1 ppm in nearly all spring seasons since the late 1980s, corresponding to 95–99% local chemical loss. In contrast, Arctic ozone loss has been much more limited and mixing ratios have never before fallen below 0.5 ppm. In Arctic spring 2020, however, ozonesonde measurements in the most depleted parts of the polar vortex show a highly depleted layer, with ozone loss averaged over sondes peaking at 93% at 18 km. Typical minimum mixing ratios of 0.2 ppm were observed, with individual profiles showing values as low as 0.13 ppm (96% loss). The reason for the unprecedented chemical loss was an unusually strong, long-lasting, and cold polar vortex, showing that for individual winters the effect of the slow decline of ozone-depleting substances on ozone depletion may be counteracted by low temperatures.

The impact of aerosol spatio-temporal variability on the Arctic radiative budget is not fully constrained. This case study focuses on the intra-Arctic modification of long-range transported aerosol and its direct aerosol radiative effect (ARE). Different types of air-borne and ground-based remote sensing observations (from Lidar and sun-photometer) revealed a high tropospheric aerosol transport episode over two parts of the European Arctic in April 2018. By incorporating the derived aerosol optical and microphysical properties into a radiative transfer model, we assessed the ARE over the two locations. Our study displayed that even in neighboring Arctic upper tropospheric levels, aged aerosol was transformed due to the interplay of removal processes (nucleation scavenging and dry deposition) and alteration of the aerosol source regions (northeast Asia and north Europe). Along the intra-Arctic transport, the coarse aerosol mode was depleted and the visible wavelength Lidar ratio (LR) increased significantly (from 15 to 64–82 sr). However, the aerosol modifications were not reflected on the ARE. More specifically, the short-wave (SW) atmospheric column ARE amounted to +4.4 - +4.9 W m−2 over the ice-covered Fram Strait and +4.5 W m−2 over the snow-covered Ny-Ålesund. Over both locations, top-of-atmosphere (TOA) warming was accompanied by surface cooling. These similarities can be attributed to the predominant accumulation mode, which drives the SW radiative budget, as well as to the similar layer altitude, solar geometry, and surface albedo conditions over both locations. However, in the context of retreating sea ice, the ARE may change even along individual transport episodes due to the ice albedo feedback.