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Optical solitons have long been of interest both from a fundamental perspective and because of their application potential. Both cubic (Kerr) and quadratic nonlinearities can lead to soliton formation, but quadratic solitons can practically benefit from stronger nonlinearity and achieve substantial wavelength conversion. However, despite their rich physics, quadratic cavity solitons have been used only for broadband frequency comb generation, especially in the mid-infrared. Here, we show that the formation dynamics of mid-infrared quadratic cavity solitons, specifically temporal simultons in optical parametric oscillators, can be effectively leveraged to enhance molecular sensing. We demonstrate significant sensitivity enhancement while circumventing constraints of traditional cavity enhancement mechanisms. We perform experiments sensing CO2 using cavity simultons around 4 μm and achieve an enhancement of 6000. Additionally, we demonstrate large sensitivity at high concentrations of CO2, beyond what can be achieved using an equivalent high-finesse linear cavity by orders of magnitude. Our results highlight a path for utilizing quadratic cavity nonlinear dynamics and solitons for molecular sensing beyond what can be achieved using linear methods. Optical molecular sensors benefit many applications from fundamental science to industry. In this work, the authors leverage the formation dynamics of cavity solitons to achieve molecular sensing in the mid-infrared spectral region. [ABSTRACT FROM AUTHOR]

Trace gas analysis is a key tool for the investigation of man-made environmental pollution as well as for early detection of respiratory diseases. To detect tiny concentrations, sensitive methods such as cavity ring down spectroscopy or plasmonic sensors have been used. Here, we demonstrate the combination of the photoacoustic effect in a classical cell with a novel, rapidly tunable, narrowband fiber-feedback optical parametric oscillator. The high sensitivity of photoacoustic cells and the extremely narrow linewidth as well as the wide and rapid tunability of the fiber-feedback optical parametric oscillator enable a high resolution of the rotational and vibrational bands of molecules in the near-infrared region. Photoacoustic spectra of methane, carbon dioxide, and water at ambient pressure are obtained in a broad spectral range and compared to high-resolution transmission molecular absorption database. In particular, scanning the entire carbon dioxide overtone around 4965 cm−1 at 2000 ppm takes 185 s with a signal-to-noise ratio of 31. This approach enables a wide tunability in the entire near- and mid-infrared spectral region suitable for many environmental and medical applications. [ABSTRACT FROM AUTHOR]

Frequency comb spectroscopy and field-resolved broadband absorption spectroscopy are promising techniques for rapid, precise, and sensitive detection of short-lived atmospheric pollutants on-site. Enhancing detection sensitivity in absorption spectroscopy hinges on bright sources that cover molecular resonances and fast signal modulation techniques to implement lock-in detection schemes efficiently. Yb:YAG thin-disk lasers, combined with optical parametric oscillators (OPOs), present a compelling solution to fulfill these requirements. In this work, we report on a bright OPO pumped using a Yb:YAG thin-disk Kerr-lens mode-locked oscillator delivering 2.8 W, 114 fs pulses at 2.06 μm with an averaged energy of 90 nJ. The OPO cavity operates at 30.9 MHz repetition rate—twice the repetition rate of the pump laser—allowing for a broadband, efficient, and dispersion-free modulation of the OPO output pulses at a 15.45 MHz rate. With 13% optical-to-optical conversion efficiency and a high-frequency intra-cavity modulation, this scalable scheme holds promise to advance the detection sensitivity and frontiers of field-resolved spectroscopy. [ABSTRACT FROM AUTHOR]

The synthesis of 2D MoWS2 nanosheets involved the liquid-phase exfoliation technique was explored in this paper. The nonlinear optical response of MoWS2 was characterized in the 1 µm wavelength range, and its suitability as a saturable absorber (SA) was confirmed. Experimental demonstrations were conducted by using MoWS2 as an SA in an idler-resonant intracavity KTA optical parametric oscillator (OPO) driven by a dual-loss-modulated Q-switched and mode-locked (QML) YVO4/Nd:YVO4 laser with an acousto-optic modulator (AOM). By appropriately tuning the pump power and the AOM repetition rate, the Q-switched envelope pulse widths for the signal and idler waves could be significantly reduced to be shorter than the cavity round-trip transit time, i.e., the interval between two neighboring mode-locking pulses. Consequently, this enabled the generation of sub-nanosecond single mode-locking pulses with a low repetition rate, high pulse energy, and remarkable stability. With a repetition rate of 1 kHz and maximal pulse energies of 318 µJ and 169 µJ, respectively, sub-nanosecond single mode-locking pulses of the signal and idler waves were generated. The theoretical model was established using coupled rate equations with a Gaussian spatial distribution approximation. The numerical simulation results for generating sub-nanosecond single mode-locking pulses for the signal and idler waves within their respective Q-switched envelopes aligned fundamentally with the experimental results, proving that MoWS2 can be a potential nanomaterial for further optoelectronic applications. [ABSTRACT FROM AUTHOR]

We demonstrate coherent anti-Stokes Raman scattering (CARS) microscopy with 1089 foci, enabled by a high repetition rate amplified oscillator and an optical parametric amplifier. We employ a camera as a multichannel detector to acquire and separate the signals from the foci, rather than using the camera image itself. This allows us to retain the insensitivity of the imaging to scattering afforded by the non-linear excitation point-spread function, which is the hallmark of point-scanning techniques. We show frame rates of 0.3 Hz for a megapixel CARS image, limited by the camera used. The laser source and corresponding CARS signal allows for at least 1000 times higher speed, and using faster cameras would allow acquiring at that speed, opening a perspective to megapixel CARS imaging with a frame rate of more than 100 Hz. [ABSTRACT FROM AUTHOR]

In this paper, we report a new model for passively Q-switched intracavity optical parametric oscillators (IC-OPOs), using Cr:YAG as a Q-switch crystal. The model considers the effects of thermalization in the Nd:YAG laser crystal, excited state absorption in the Cr:YAG saturable absorber, nonlinear loss due to pump depletion in the nonlinear crystal, the thermal lens effect and the mode overlap of the fields within the nonlinear crystal. The calculated pulse width for the 1,064 nm pump light was 6.2 ns compared to the experimental result of 6 ns, while the signal wave was calculated to have a pulse width of 1.75 ns compared to the experimental result of 2 ns. The model is shown to accurately calculate both the temporal and output power characteristics of the IC-OPO, which has not been previously reported to the best of our knowledge. [ABSTRACT FROM AUTHOR]

The ability to confine and guide wave makes topological physics a promising platform for large local field enhancement and strong scattering immunity, which enables efficient nonlinear processes. In this research, we employ a mirror-stacking approach to achieve resonance through two distinct frequency localized states (LSs) in one-dimensional topological circuits, introducing a novel method for validating topological states to facilitate harmonic enhancement. Experimental results reveal that the harmonic wave power increases significantly, by two orders of magnitude, when both the fundamental and harmonic waves are in LSs, in contrast to cases where only one wave is localized. The conversion efficiency is 15.7 times that when the fundamental wave is in a localized state and the harmonic is in a transmission mode. This method, leveraging double-resonance in topological LSs, not only advances harmonic generation in topolectrical circuits but also opens up possibilities for innovative applications in the broader field of photonic technology. This paper presents a study on topologically enhanced third harmonic generation within resonant nonlinear topolectrical circuits. The authors demonstrate that the implementation of a mirror-stacking approach in one-dimensional topological circuits enables achieving significant harmonic wave power increase, leading to efficient nonlinear processes. [ABSTRACT FROM AUTHOR]

This work is devoted to the development of a compact source of coherent radiation with frequency-energy characteristics and a spectral generation range that allows remote determination of background concentrations of greenhouse gases in the atmosphere. The aim of this work was to create a frequency parametric converter based on ZGP, pumped by Ho:YAG laser radiation. For use as a source in a mobile lidar for remote determination of the concentration of greenhouse gases in the atmosphere. In the course of the research, a layout of an Optical parametric oscillator OPO based on a ZGP crystal with Ho:YAG laser radiation pumping was developed. The system's continuous failure-free operation time was 1.5 h at a pulse repetition rate of 10 kHz and a pulse energy of the generated radiation of 0.08 mJ. The tuning range of the OPO was from 3.3 to 5 μιτι when using a Lyot filter. The losses from the average generation power when the Lyot filter was introduced into the resonator were 30%. At the same time, it was possible to achieve a linewidth of the generated radiation of 0.7 nm. The divergence of the generated radiation did not exceed 1.5 mrad.The absorption spectrum of gases CO2, CH4, N2O, CO in a gas cell was simulated for the entire generation range of the ZnGeP2-based OPO. As a result of the simulation, the most intense absorption lines of gases CO2, CH4, N2O, CO in the OPO tuning range were revealed, the central wavelengths of the absorption lines and their spectral width were determined. [ABSTRACT FROM AUTHOR]

While nano-crystalline diamond (NCD) is a promising engineering composite material for its unique mechanical properties, achieving the ultrahigh surface quality of NCD-based components through conventional grinding and polishing is challenging due to its exceptional hardness and brittleness. In the present work, we experimentally investigate the nanosecond laser ablation-induced graphitization characteristics of NCD, which provides a critical pretreatment method of NCD for realizing its superlative surface finish. Specifically, systematic experimental investigations of the nanosecond pulsed laser ablation of NCD are carried out, in which the characteristics of graphitization are qualitatively characterized by the Raman spectroscopy detection of the ablated area of the microhole and microgroove. Subsequently, the influence of laser processing parameters on the degree and morphological characteristics of graphitization is evaluated based on experimental data and related interpretation, from which optimized parameters for maximizing the graphitization of NCD are then identified. The findings reported in the current work provide guidance for promoting the machinability of NCD via laser irradiation-induced surface modification. [ABSTRACT FROM AUTHOR]

An overview of Optical Parametric Chirped Pulse Amplification (OPCPA) is given as the basis for the next generation of ultra-intense laser systems (> 1 × 10 23 W/cm2). The benefits and drawbacks of OPCPA are discussed to explain the choice behind the decisions for the direction of the Central Laser Facility's (CLF) upcoming Vulcan 20-20 project. A history of OPCPA use at the CLF is described to surmise the foundation of the confidence in this technology for Vulcan 20-20; a 20 PW user facility for high-intensity plasma physics. [ABSTRACT FROM AUTHOR]

The gain factor of the optical parametric amplification (OPA) process is known to be negligible in the small scale due to low‐interaction‐medium length. Hence, in the nanoscale, OPA is deemed as infeasible. Therefore, in small‐scale‐integrated optical devices, stimulated‐emission‐based amplifiers (lasers) are employed instead of OPAs. In contrast, the major advantage of OPAs over lasers is that unlike lasers which only provide amplification over a narrow spectral band, OPAs provide high‐gain amplification over a very large, user‐controlled spectral band. In this article, it is shown that OPA can yield wideband high‐gain amplification over a nanoscale beam propagation distance through dispersion engineering. This is achieved by a proper tuning of the pump (source) wave frequency, which can maximize the effective medium nonlinearity by a few orders of magnitude, while concurrently maximizing the intracavity energy density, thereby compensating for the small co‐propagation distance for the input (signal) and pump beams. In this study, it is shown that an input wave can be amplified by a factor 108$\left(10\right)^{8}$ in a nanoscale cavity via precise dispersion engineering. Both empirical and computational formulations are used for the investigation, which display a reasonable agreement. [ABSTRACT FROM AUTHOR]

Chirped pulse amplification (CPA) has been a commonly used methodology to obtain powerful ultrashort laser pulses ever since its first demonstration. However, wavelength-tunable CPA systems are much less common. Wavelength-tunable ultrashort and intense laser pulses are desirable in various fields such as nonlinear spectroscopy and optical parametric amplification. In this work, we report a 1720 nm–1800 nm tunable CPA system based on Tm-doped fiber. The tunable CPA system contains a seed laser, a pulse stretcher, two cascaded amplifiers and a pulse compressor. The dispersion-managed seed laser cavity emits wavelength-tunable laser pulses with pulse durations of several ps and spectral widths from 25 nm to 34 nm. After being stretched temporally to tens of ps, the laser pulses are then amplified in two-stage amplifiers and compressed in a Treacy-type compressor. At 1720 nm, the maximum average power of 126 mW is obtained with a pulse duration of 507 fs; at 1800 nm, the maximum average power of 264 mW is obtained with a pulse duration of 294 fs. The pulse repetition rates are around 22.7 MHz. We perform an analysis of the system design based on numerical simulations and go on to suggest further steps for improvement. To the best of our knowledge, this is the first demonstration of a tunable CPA system beyond 1.1 μm. Considering the specific wavelength range, this wavelength-tunable CPA system is highly desirable for biomedical imaging, sensing, and parametric amplifiers. [ABSTRACT FROM AUTHOR]

We demonstrate the generation of broadband tunable and synchronized pulses exceeding the microjoule level using the new concept of Fiber Optical Parametric Chirped-Pulse Oscillation (FOPCPO). The oscillator is based on a collapsed-ends photonic crystal fiber pumped in the normal dispersion regime by an ytterbium fiber laser delivering highly-chirped pulses. The experimental results are compared with the results of numerical simulations and highlight that the feedback ratio appears as a key parameter for optimizing the system's efficiency and dynamics. [ABSTRACT FROM AUTHOR]

We describe an efficient long-wave infrared optical parametric oscillator based on ZnGeP2 crystal pumped by a diode-pumped AO Q-switched Ho:YAG laser in this paper. The wavelength of the laser pulse generated by Ho:YAG laser is 2.09- μιτι, and the maximum output average power is 25.3 W at repetition rate of 10 kHz. When pumped by such Ho:YAG laser, the maximum average output power of 0.66 W at 9.8 μ!Γ is achieved, corresponding to slope efficiency of 5.0% and optical efficiency of 2.6%. Furthermore, the beam quality factor of the longwave infrared beam is measured to be approximately 1.3. To the authors' best knowledge, this is the best performance reported for a long-wave infrared ZGP-OPO pumped by a diode-pumped AO Q-switched Ho:YAG laser. [ABSTRACT FROM AUTHOR]

This study's novel 13Ni400 maraging steel parts are additively manufactured through a selective laser melting process. The Taguchi approach is adopted to evaluate the combined influence of process variables (energy density), viz., laser power, layer thickness, hatch spacing, and scan speed, on responses like relative density, microhardness, surface roughness, and tensile strength. The powder and material characterization studies are conducted in terms of an optical microscope, scanning electron microscope (SEM), electron backscatter diffraction (EBSD), X-ray diffraction (XRD), and fractography analysis to explore the pre- and post-fabrication scenarios of the build parts. The consequences of energy density and process variables are studied through meticulous parametric studies. Finally, the optimum level of built parameters is identified and validated by a confirmative test predicting an average error of ~1.80%. This work is proficient in producing defect-free parts with maximum densification and improved mechanical properties for newly developed 13Ni-400 maraging steel by the selective laser melting (SLM) technique. [ABSTRACT FROM AUTHOR]

In this paper, we present a picosecond pulsed, synchronously pumped optical parametric oscillator producing vortex beam output with tunable wavelengths in the near- to mid-infrared range. The system utilizes a Nd:YVO4 picosecond pulsed solid-state laser emitting at a wavelength of 1.064 µm to pump a Z-shaped, singly resonant OPO which contains a MgO:PPLN crystal with a fan-shaped grating. The wavelength tuning characteristics of the OPO output are examined both as a function of the MgO:PPLN grating period and crystal temperature. The orbital angular momentum of the pump field can be selectively transferred to either the signal or idler fields by appropriately adjusting the location of the MgO:PPLN crystal within the OPO cavity. The maximum output power of the signal and idler vortex fields are 5.12 W and 3.46 W, respectively, for an incident pump power of 19 W. [ABSTRACT FROM AUTHOR]

In this paper, we report a theoretical systematic study of continuous wave intracavity backwards optical parametric oscillators based on periodically poled lithium niobate (PPLN) for mid-infrared (mid-IR) light generation. We study the effects of varying different cavity parameters including nonlinear crystal length, cavity size, pump laser diode spot size, output coupler radius, and cavity loss values on the output power and threshold of the proposed mid-IR laser. The effects of different physical phenomena are included in the model including pump depletion due to the nonlinear conversion process, the thermal lens effect, and mode overlap between the beams in the nonlinear crystal. We show that high output powers in the mid infrared (>500 mW at 3.2 μm) can be achieved with proper cavity design and that a laser threshold with a PPLN as short as 2 cm can be reached. [ABSTRACT FROM AUTHOR]

Quantum optical technologies promise advances in sensing, computing, and communication. A key resource is squeezed light, where quantum noise is redistributed between optical quadratures. We introduce a monolithic, chip-scale platform that exploits the (2) nonlinearity of a thin-film lithium niobate (TFLN) resonator device to efficiently generate squeezed states of light. Our system integrates all essential components--except for the laser and two detectors--on a single chip with an area of one square centimeter, reducing the size, operational complexity, and power consumption associated with conventional setups. Using the balanced homodyne measurement subsystem that we implemented on the same chip, we measure a squeezing of 0.55 decibels and an anti-squeezing of 1.55 decibels. We use 20 milliwatts of input power to generate the parametric oscillator pump field by using second harmonic generation on the same chip. Our work represents a step toward compact and effficient quantum optical systems posed to leverage the rapid advances in integrated nonlinear and quantum photonics. [ABSTRACT FROM AUTHOR]

We present a high-power, widely tunable, synchronously pumped picosecond pulsed optical parametric oscillator (OPO) generating emissions in the near to mid-infrared wavelength ranges. The OPO is pumped using a Nd:YVO4 picosecond pulsed laser and utilizes a fan-shaped, multi-grating MgO doped PPLN crystal (MgO:PPLN). The system generates near to mid-infrared output across the wavelength range 1.3–5 µm, with a high overall conversion efficiency of 75.15%. [ABSTRACT FROM AUTHOR]

Lasers operating around 2-µm have been extensively researched for various applications, such as LiDAR, remote sensing, optical communication, and medicine. One of the approaches to generate 2-µm emission is to employ an optical parametric oscillator pumped by 1-µm laser; however, improving the 2-µm laser conversion efficiency of optical parametric oscillators is still a challenge. In this study, we exploit the high nonlinear coefficient of the KTP crystal at the 2-µm band to realize a high-efficiency optical parametric oscillator. TheOPOis driven by a laser diode (LD) side-pumped, electro-optic Q-modulated Nd:YAG laser. The cavity was designed and optimized based on mode matching to increase the peak power density of the pump laser. Different powers were obtained for different pump laser focusing conditions, and the maximum power was obtained when the KTP crystal was placed in front of the pump laser focus. The output characteristics of the KTP at different phase-matching angles were also investigated. An output power of 2.44Wand an output pulse width of 9.04 ns were obtained at 2154.4 nm with an optical-to-optical conversion efficiency of 23.39% and a slope efficiency of 36.09%. [ABSTRACT FROM AUTHOR]

Detecting the electric-field waveform of an optical pulse from the terahertz to the visible spectral domain provides a complete characterization of the average field waveform and holds great potential for quantum optics, time-domain (including frequency-comb) spectroscopy, high-harmonic generation, and attosecond science, to name a few. The field-resolved measurements can be performed using electro-optic sampling, where a laser pulse is characterized through an interaction with another pulse of a much shorter duration. The measured pulse train must consist of identical pulses, including their equal carrier-envelope phase (CEP). Due to the limited coverage of broadband laser gain media, creating CEP-stable pulse trains in the mid-infrared typically requires nonlinear frequency conversion, such as difference frequency generation, optical parametric amplification, or optical rectification. These techniques operate in a single-pass geometry, often limiting efficiency. In this work, we demonstrate field-resolved analysis of the pulses generated in a resonant system, an optical parametric oscillator (OPO). Due to the inherent feedback, this device exhibits a relatively high conversion efficiency at a given level of input power. By electro-optic sampling, we prove that a subharmonic OPO pumped with CEP-stable few-cycle fiber-laser pulses generates a CEP-stable mid-infrared output. The full amplitude and phase information renders dispersion control straightforward. We also confirm the existence of an exotic "flipping" state of the OPO directly in the time domain, where the electric field of consecutive pulses has the opposite sign. [ABSTRACT FROM AUTHOR]

Laser pulse amplification by a high-pressure CO2 amplifier in the long-wave infrared (LWIR) spectral range is a feasible technology for strong-field physics research. Crystals such as ZnGeP2 (ZGP) have high nonlinear coefficients and transmittance in the LWIR region, with spectral widths of generated pulses closely matching the gain spectrum of high-pressure CO2 amplifiers. Therefore, ZGP optical parametric oscillation (OPO) may allow higher-efficiency energy extraction in amplifiers, improving the output characteristics of LWIR amplification systems. In this study, the gain measurement of ZGP OPO pulses amplified by a high-pressure CO2 amplifier was carried out for the first time. Single-detector acquisition was utilized to achieve a unified sensor responsivity, and a laser signal-triggered function generator was used to synchronize the seed pulse and amplifier. Six-pass amplification was performed successively, yielding an amplification factor of 4.5 for the peak power and a maximum coefficient of 0.42% cm−1 for the small-signal gain. The gain and loss effect during small-signal amplification were discussed. The potential capability of acquiring ultra-short pulses with ZGP OPO pulses was also explored with the FFT function of MATLAB software. [ABSTRACT FROM AUTHOR]

We present a Hamiltonian model describing two pairs of mechanical and optical modes under standard optomechanical interaction. The vibrational modes are mechanically isolated from each other and the optical modes couple evanescently. We recover the ranges for variables of interest, such as mechanical and optical resonant frequencies and naked coupling strengths, using a finite element model for a standard experimental realization. We show that the quantum model, under this parameter range and external optical driving, may be approximated into parametric interaction models for all involved modes. As an example, we study the effect of detuning in the optical resonant frequencies modes and optical driving resolved to mechanical sidebands and show an optical beam splitter with interaction strength dressed by the mechanical excitation number, a mechanical bidirectional coupler, and a two-mode mechanical squeezer where the optical state mediates the interaction strength between the mechanical modes. [ABSTRACT FROM AUTHOR]

Significance: In the analysis of two-layered turbid dental tissues, the outer finitethickness layer is modeled by an optical transport coefficient distinct from its underlying semi-infinite substrate layer. The optical and thermophysical parameters of healthy and carious teeth across the various wavelengths were measured leading to the determination of the degree of reliability of each of the fitted parameters, with most reliable being thermal diffusivity and conductivity, enamel thickness, and optical transport coefficient of the enamel layer. Quantitative pixel-by-pixel images of the key reliable optical and thermophysical parameters were constructed. Aim: We introduced a theoretical model of pulsed photothermal radiometry based on conduction-radiation theory and applied to quantitative photothermal detection and imaging of biomaterials. The theoretical model integrates a combination of inverse Fourier transformation techniques, avoiding the conventional cumbersome analytical Laplace transform method. Approach: Two dental samples were selected for analysis: the first sample featured controlled, artificially induced early caries on a healthy tooth surface, while the second sample exhibited natural defects along with an internal filling. Using an Nd:YAG laser and specific optical parametric oscillator (OPO) wavelengths (675, 700, 750, and 808 nm), photothermal transient signals were captured from different points on these teeth and analyzed as a function of OPO wavelength. Measurements were also performed with an 808-nm laser diode for comparison with the same OPO wavelength excitation, particularly for the second sample with natural defects. Results: The findings demonstrated that the photothermal transient signals exhibit a fast-decaying pattern at shorter wavelengths due to their higher scattering nature, while increased scattering and absorption in the carious regions masked conductive and radiative contributions from the underlayer. These observations were crossvalidated using micro-computed tomography, which also enabled the examination of signal patterns at different tooth locations. Conclusions: The results of our study showed the impact of optical and thermal characteristics of two-layered turbid dental tissues via an inverse Fourier technique, as well as the interactions between these layers, on the patterns observed in depth profiles. [ABSTRACT FROM AUTHOR]

We demonstrate experimentally that a recently proposed structure comprising a tens of microns thick layer of LiNbO 3 sandwiched between two totally reflecting Si prisms can serve as an efficient Cherenkov-type optical-to-terahertz converter of femtosecond laser pulses from an optical oscillator. Using Ti:sapphire laser pulses of 3.75 nJ energy as a pump, we achieved a conversion efficiency of 2.3 × 10 − 5 , which exceeds the efficiency of the conventional collinear scheme with a ZnTe crystal by an order of magnitude. The converter can be used as a reliable radiation source for performing terahertz time-domain spectroscopy. [ABSTRACT FROM AUTHOR]

Zinc germanium phosphide (ZGP) crystals have garnered significant attention for their nonlinear properties, making them good candidates for powerful mid-IR optical parametric oscillators and second-harmonic generators. A ZnGeP2 single crystal was treated by deep magnetorheological processing (MRP) until an Angstrom level of roughness. The studies presented in this article are devoted to the experimental evaluation of the influence of deep removal (up to 150 μm) from the surface of a ZnGeP2 single crystal by magnetorheological polishing on the parameters of optical breakdown. It was shown that the dependence of the ZnGeP2 laser-induced damage threshold on MRP depth is a smooth monotonically decreasing logarithmic function. The obtained logarithmic dependence indicates the thermal nature of optical breakdown and the dependence of the ZnGeP2 laser-induced damage threshold on the concentration of surface absorbing defects. [ABSTRACT FROM AUTHOR]

In this paper, a calculation model is proposed for the optical parametric oscillation (OPO) process considering the crystal thermal effects. Based on existing models, we combine a set of three-wave coupled equations with the Sellmeier equation. In order to optimize the calculation of the nonlinear process, a temperature variable t is introduced to describe the heat generated by the laser crystal during operation. The waveforms under different pump powers are analyzed. The effects of the reflectivity of the output mirror on the OPO threshold and inverse conversion are investigated. In addition, the optimal reflectivity under different pump powers can be estimated. Based on the simulation results, experiments are also performed in the near-infrared 1.57 μιτι band and mid-infrared 3.15 μιτι band. The experimental results are compared with the results of this model and a model that does not consider crystal thermal effects. The experimental results are consistent with the improved theoretical results, affirming that the proposed theoretical model can simulate the energy conversion process of OPO. This provides a theoretical basis for optimizing the parameters of the OPO output mirror and improving the efficiency of the parametric wave conversion. [ABSTRACT FROM AUTHOR]

In this work, solid-state reaction sintering was used to fabricate Ca7ZrAl6O18-Ca3Al2O6-CaZrO3:Eu3+ ternary composite ceramics and cements. The structural, microstructural, and spectroscopic properties of the ceramics with different Eu2O3 content were characterized by X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FT-IR), scanning electron microscopy (SEM) and energy dispersive X-ray spectroscopy (EDS), and spectrofluorimetry, respectively. The XRD patterns analyzed with Rietveld refinement confirm the presence of the orthorhombic phase of Ca7ZrAl6O18 and the cubic phase of Ca3Al2O6 in all the samples, indicating that doping of Eu3+ slightly changes the crystalline structure of both aluminate phosphors. EDS analysis revealed that the Eu doping element was strongly concentrated to the two phases, i.e., Ca7ZrAl6O18 and Ca3Al2O6, with the Eu concentrations of 8.45 wt.% and 8.26 wt.%, respectively. The luminescent properties of the ceramics doped with different Eu3+ ion concentrations were investigated by excitation and emission spectroscopy at room temperature. These results were compiled using a laser with an optical parametric oscillator (OPO) system. The obtained spectra indicated changes in the luminescence intensity and shape occurring with phase composition and Eu2O3 concentration. The emission spectra of the ceramics exhibit a strong dependence on the excitation wavelength in the range from 210 to 300 nm, and invariably, five peaks were assigned to the 5D0 → 7FJ (J = 0, 1, 2, 3, 4) transitions of Eu3+. The luminescence spectroscopy was then used to trace the early and long-term hydration behavior of cements. Thus, luminescence spectroscopy may provide a new tool for non-destructive testing of cement-based structures. [ABSTRACT FROM AUTHOR]

The nonlinear properties of zinc germanium diphosphide (ZGP) crystals enable their applications in powerful mid-IR optical parametric oscillators and second-harmonic generators. This paper summarizes the mechanisms of the laser-induced damage (LID) of high-purity ZGP crystals under periodically pulsed nanosecond irradiation by a Ho3+:YAG laser at 2.1 μm. The ZGP samples were manufactured by "LOC" Ent., Tomsk, Russia, or the Harbin Institute of Technology, China. The impact of processing techniques and the post-growing methods for polishing and anti-reflective coatings on the LID threshold are discussed. The importance of the defect structure of the crystal lattice and the parameters of transparent coatings for increasing the LID threshold are also discussed. The impact of the test laser parameters on the LID threshold and the transient area near the LID threshold obtained using digital holography are analyzed. The influence of the pre-damage processes on the optical parametric oscillations is reported. Lastly, the prospects for improving ZGP crystals to further increase the LID threshold are discussed. [ABSTRACT FROM AUTHOR]

In this paper, we investigated the quantum correlation of nano-electro-optomechanical system enhanced by an optical parametric amplifier (OPA) and Coulomb-type interaction. In particular, we consider a hybrid system consisting of a cavity and two charged mechanical oscillators with an OPA, where the optical cavity mode is coupled with a charged mechanical oscillator via radiation pressure, and the two charged mechanical oscillators are coupled through a Coulomb interaction. We use logarithmic negativity to quantify quantum entanglement, and quantum discord to measure the quantumness correlation between the two mechanical oscillators. We characterize quantum steering using the steerability between the two mechanical oscillators. Our results show that the presence of OPA and strong Coulomb coupling enhances the quantum correlations between the two mechanical oscillators. In addition, Coulomb interactions are more prominent in quantum correlations. Besides, in the presence of OPA, the maximum amount of quantum entanglement, quantum steering, and quantum discord were achieved between the two mechanical oscillators is greater than in the absence of OPA. Moreover, a proper phase choice of the optical field driving the OPA enhances quantum correlations under suitable conditions. We obtain quantum entanglement confines quantum steering and quantum discord beyond entanglement. Furthermore, quantum entanglement, quantum steering, and quantum discord decrease rapidly with increasing temperature as a result of decoherence. In addition, quantum discord persists at higher temperature values, although the quantum entanglement between the systems also vanishes completely. Our proposed scheme enhances quantum correlation and proves robust against fluctuations in the bath environment. We believe that the present scheme of quantum correlation provides a promising platform for the realization of continuous variable quantum information processing. [ABSTRACT FROM AUTHOR]

We present a uniquely versatile and efficient mirror system capable of real-time fine-tuning in reflection and transmission properties across a broad wavelength range and at a high optical power. Leveraging the principles of the non-cyclic geometric phase (GP) acquired by the clockwise and counterclockwise beams of the Sagnac interferometer satisfying the anti-resonant condition on propagation through the quarter-wave plate, half-wave plate, and quarter-wave plate combination having fast axes oriented at 45° (fixed), θ (variable), and −45° (fixed) with respect to the vertical, respectively, our mirror system offers dynamic transmission control across 0–100% without the need for realignment. Notably, the GP-based mirror (GP-mirror) preserves the polarization state of the reflected beam, making it ideal for polarization-sensitive applications. The wavelength insensitivity of the GP enables seamless operation of the mirror across a wide wavelength range. As a proof-of-principle, we use the GP-mirror as the output coupler of a continuous-wave, green-pumped, doubly resonant optical parametric oscillator (DRO) based on a 30-mm-long MgO:sPPLT crystal and obtain stable operation at high powers over a wide wavelength tuning range. For a pump power of 5 W, the DRO provides an output power of 2.45 W at an extraction efficiency as high as 49% when operated at optimum output coupling. The DRO shows a maximum pump depletion of 89% and delivers an optimum output power across a tuning range ≥90 nm. The demonstrated concept offers a promising approach for advancing the capabilities and control of coherent optical sources tunable across different spectral regions and in all time scales from continuous-wave to ultrafast femtosecond domain. [ABSTRACT FROM AUTHOR]

Synchronously pumped optical parametric oscillators (OPOs) provide ultra-fast light pulses at tuneable wavelengths. Their primary drawback is the need for precise cavity control (temperature and length), with flexibility issues such as fixed repetition rates and marginally tuneable pulse widths. Targeting a simpler and versatile OPO, we explore the inherent disorder of the refractive index in single-mode fibres realising the first random OPO – the parametric analogous of random lasers. This novel approach uses modulation instability (χ(3) non-linearity) for parametric amplification and Rayleigh scattering for feedback. The pulsed system exhibits high inter-pulse coherence (coherence time of ~0.4 ms), offering adjustable repetition rates (16.6–2000 kHz) and pulse widths (0.69–47.9 ns). Moreover, it operates continuously without temperature control loops, resulting in a robust and flexible device, which would find direct application in LiDAR technology. This work sets the stage for future random OPOs using different parametric amplification mechanisms. In this work the authors develop a Random optical parametric oscillator - the parametric analogous of random lasers. This system shows improved key metrics like tuneable repetition rates, tuneable pulse duration, inter-pulse coherence as well as simpler configuration compared with standard systems. [ABSTRACT FROM AUTHOR]

A widely tunable 4.16–7.31 μm high-resolution mid-infrared optical parametric oscillator with a type-I BaGa4Se7 (BGSe) crystal pumped by a 1064 nm laser was demonstrated for the first time. We have achieved a wavelength tuning accuracy of less than 5 nm through simultaneously performing temperature tuning and angular tuning on the BGSe (46°, 0°) Optical Parametric Oscillation (OPO). The wavelength resolution will be less than 1 nm when using commercial temperature control equipment. [ABSTRACT FROM AUTHOR]

The 3 μm wavelength band laser is located on the strong absorption peak of water and the atmospheric transmission window. The 3 μm laser with high single pulse energy is used in medical treatment for cutting soft tissues and bones during surgery. It is used as a pump source for optical parametric oscillators, and Fe lasers can realize 3~5 μm or 8~14 μm laser output, which has an irreplaceable role in certain areas (e.g., optoelectronic countermeasures, LIDAR, atmospheric monitoring, etc.). Commercial semiconductor-pumped Er lasers are capable of achieving 3 μm laser output of 600 mJ with the maturation of a 970 nm semiconductor laser. The conversion efficiency is significantly improved. However, the energy is lower than a flash-lamp-pumped Er laser. There are still serious crystal thermal effects and an inefficient conversion process. In this paper, the energy-level systems of 3 μm Er-doped lasers are discussed. A summary of the current state of research on Er lasers using different matrices and the commercialization of Er-doped lasers with wavelengths ranging from 2.7 μm to 3 μm is also provided. Several technical means are given to enhance laser performance. Furthermore, the development of Er-doped solid-state lasers with wavelengths between 2.7 and 3 μm is envisaged in the near future. [ABSTRACT FROM AUTHOR]

Coherent Ising machine (CIM) is a network of optical parametric oscillators that can solve large-scale combinatorial optimisation problems by finding the ground state of an Ising Hamiltonian. As a practical application of CIM, Aonishi et al., proposed a quantum-classical hybrid system to solve optimisation problems of l 0 -regularisation-based compressed sensing. In the hybrid system, the CIM was an open-loop system without an amplitude control feedback loop. In this case, the hybrid system is enhanced by using a closed-loop CIM to achieve chaotic behaviour around the target amplitude, which would enable escaping from local minima in the energy landscape. Both artificial and magnetic resonance image data were used for the testing of our proposed closed-loop system. Compared with the open-loop system, the results of this study demonstrate an improved degree of accuracy and a wider range of effectiveness. [ABSTRACT FROM AUTHOR]

We report on the use of quartz-enhanced photoacoustic spectroscopy (QEPAS) for multi-gas detection. Photoacoustic (PA) spectra of mixtures of water (H 2 O), ammonia (NH 3 ), and methane (CH 4 ) were measured in the mid-infrared (MIR) wavelength range using a mid-infrared (MIR) optical parametric oscillator (OPO) light source. Highly overlapping absorption spectra are a common challenge for gas spectroscopy. To mitigate this, we used a partial least-squares regression (PLS) method to estimate the mixing ratio and concentrations of the individual gasses. The concentration range explored in the analysis varies from a few parts per million (ppm) to thousands of ppm. Spectra obtained from HITRAN and experimental single-molecule reference spectra of each of the molecular species were acquired and used as training data sets. These spectra were used to generate simulated spectra of the gas mixtures (linear combinations of the reference spectra). Here, in this proof-of-concept experiment, we demonstrate that after an absolute calibration of the QEPAS cell, the PLS analyses could be used to determine concentrations of single molecular species with a relative accuracy within a few % for mixtures of H 2 O, NH 3 , and CH 4 and with an absolute sensitivity of approximately 300 (±50) ppm/V, 50 (±5) ppm/V, and 5 (±2) ppm/V for water, ammonia, and methane, respectively. This demonstrates that QEPAS assisted by PLS is a powerful approach to estimate concentrations of individual gas components with considerable spectral overlap, which is a typical scenario for real-life adoptions and applications. [ABSTRACT FROM AUTHOR]

We report an all-solid-state narrowband lidar system for the simultaneous detection of Ca and Ca+ layers over Yanqing (40.41°N, 116.01°E). The uniqueness of this lidar lies in its transmitter, which is based on optical parametric oscillation (OPO) and optical parametric amplification (OPA) techniques. The injection seeded OPO and the OPA are pumped by the second harmonic of an injection-seeded Nd:YAG laser, which can generate coherent light at the wavelength of 786 nm or 846 nm lasers, whose second harmonics in turn generate the 393 nm or 423 nm pulses, respectively, for the detection of thermospheric and ionospheric Ca+ and Ca layers. Compared to the conventional dye-based system, this lidar transmitter is a narrowband system (bandwidth < 200 MHz), which has produced a factor of two more output power with higher stability and reliability. The lidar system in Yingqing demonstrated Ca+ detection sensitivity of 0.1 atoms-cm−3 for long-term observation and reached a height of ~300 km. Potential applications and further improvements in this lidar technique are also discussed in this paper. [ABSTRACT FROM AUTHOR]

Wavelength‐dependent mid‐infrared (400–1,800 cm−1; 5.56–25 μm) optical constants (real and imaginary indices of refraction; n and k) are determined using reflectance spectra at a spectral sampling of 4 cm−1 for several silicate glasses of varying SiO2 wt% which include (a) basaltic volcanic glass from Kīlauea, Hawaii, (b) synthetic andesite, (c) two synthetic dacites, (d) obsidian volcanic glass from Mount Lassen, California, (e) synthetic rhyodacite, and (f) rhyolitic volcanic glass from Mexico. Because glasses are optically isotropic, no specific orientation was required for spectral measurements, and polished glass samples were measured at random orientations using micro‐FTIR spectrometer. Lorentz‐Lorenz dispersion theory and Fresnel reflectance model for high symmetry materials were used to model the optical constants by optimizing oscillator parameters in modeled spectra to match laboratory spectra. A genetic algorithm (GA) approach automatically finds the natural oscillators and their parameters for each spectrum, and then uses these parameters in a non‐linear least squares optimization routine. The study compared spectral parameters such as Christiansen feature, reststrahlen bands (RBs), and the peaks centered around 860–1,100 (peak 1) and 400–480 cm−1 (peak 2) of n and k to their respective SiO2 wt% of the glasses. CF, RBs, peak 1 of n and k, and peak 2 of n shift to higher wavenumbers with increased SiO2 wt%, whereas peak 2 of k shifts to lower wavenumbers with increased SiO2 wt%. Derived optical constants of these glasses will improve quantitative abundance mapping of volcanic materials on the surfaces of silicate targets in the Solar System. Plain Language Summary: The effective mapping of minerals and their abundances on a planet's surface from orbit is enabled by understanding the nature of the interaction of light of varying wavelengths with the planetary surface. The reflected/emitted light from the surface directly depends on the optical properties of the materials and their interaction with each other. In this study, we numerically modeled the mid‐infrared optical constants of silicate glasses using a genetic algorithm (GA) approach. The GA allows the model to automatically locate the natural harmonic oscillators and their parameters that are responsible for creating the spectral signals that can be detected by spectrometers on orbital spacecraft. Derived optical constants of the glasses could be used in radiative transfer models for quantitative mineral mapping applications. Glasses on planetary surfaces are common in volcanic and/or impact materials and the mid‐infrared spectral range has been widely used to map the surface mineralogy of planets including the Moon and Mars. Mapping the composition and abundance of these glasses therefore will help us to understand the thermal evolution of the planets themselves. Key Points: MIR optical constants (5.56–25 μm; 400–1,800 cm−1) and their oscillator parameters were modeled for seven silicate glasses of varying SiO2 wt%MicroFTIR reflectance spectra of the glasses studied were measured for the spectral region 5.56–25 μm (400–1,800 cm−1)Genetic algorithm was adopted to automatically find the natural oscillators and their parameters for the glasses studied [ABSTRACT FROM AUTHOR]

The article offers information on achieving high-Q spectral selectivity and enhancing optical interactions through nonlocal effects on metasurfaces, aiming to develop active nonlinear optical metadevices at the nanoscale. The study demonstrates significant electric and all-optical tunability of nonlocal second-harmonic generation (SHG) from nonlinear metasurfaces integrated with a twisted nematic liquid-crystal (LC) layer, leading to enhanced SHG through surface lattice resonance.

The article focuses on a study, which demonstrates the creation of ultrawidely tunable doubly resonant optical parametric oscillators (OPOs) using lithium niobate nanophotonics. With high milliwatts of output powers, output wavelengths are generated in a single chip. The study presents initial tunable source in nanophotonics, covering an octave-spanning range and extending into the mid-infrared spectrum with potential for various combined photonic applications.

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Spectroscopy in the terahertz (THz) band has been discussed as a promising tool for identifying substances such as mold in food, narcotics, or explosive materials. Other than the technological limitations, the most important difficulty is the presence of water vapor in the atmosphere, which affects THz measurements. In this paper, we present a systematic approach to the challenging subject of remote identification. We start with a brief analysis of the technical capabilities of the THz components and report the choice of devices for designing an experimental setup for reflection spectroscopy. We follow with the presentation of the transmission THz spectrometer working in an open atmosphere. Research conducted on the transmission configuration provides findings that are implemented in the experimental setup working in a reflective configuration. The final phase is an experiment providing data measured in the reflection configuration with the presence of water vapor, allowing the use of spectra in the identification of the measured samples. [ABSTRACT FROM AUTHOR]

High-power optical parametric oscillators (OPOs), as mature radiation sources in mid-infrared (MIR), degenerate gradually with wavelength increase, mainly above 3700 nm. Using a periodically poled magnesium-oxide-doped lithium niobate (MgO:PPLN) as the nonlinear crystal, we build a high-power signal-resonant OPO pumped by ytterbium-doped fiber laser (YDFL). To improve the OPO's output power at ~3.8 μm, the parameters, such as the pump beam's waist diameter and location, the curvature radius of the output coupler and the length of MgO:PPLN, are discussed in detail. When pump power is 79 ± 4 W with a repetition rate of 200 kHz, the OPO provides up to 8 ± 0.4 W average power in beam quality with M2 factors of ~1.84 and ~1.69 in the two axes. Under the highest output power, the center wavelength of the idler beam is 3768.4 nm with a full-width at half-maximum (FWHM) bandwidth of ~18.6 nm. When the output power reaches ~6.3 W, its power stability is 1.6% root mean square (RMS) over 7 h. Further analysis of the factors affecting OPO's performance and simple structure are critically essential for compact OPO prototypes with a capacity of high output power. [ABSTRACT FROM AUTHOR]

The article discusses a breakthrough in video-rate mid-infrared photothermal imaging, enabling super-resolution imaging of biological systems in water. By detecting the transient photothermal signal induced by a single infrared pulse, the imaging speed has been increased by three orders of magnitude. This advancement allows for observing the dynamics of biomolecules in living organisms and mapping fat storage in free-moving organisms.

Laser–plasma interactions (LPIs) hinder the interaction of high-energy laser pulses with targets. The use of broadband low-coherence light has been proposed to reduce the impact of LPIs. In this study, to improve the time–frequency characteristics of broadband low-coherence optical seeds, we proposed an arbitrary time-shaping technique scheme based on optical parametric amplification (OPA) that differs from traditional arbitrary time shaping. The shaping process and output characteristics were analyzed in detail. The theoretical and experimental results show that an arbitrary time-shaping pulse output with a large time-shaping contrast, fast-rising edge, and wide spectral width can be obtained. The time shaping contrast of the shaped pulse can be >300:1, and the spectral width is ~40 nm. The output time waveform is smoother than in traditional schemes, and the noise-like modulation is approximately 4% (approximately equal to the unshaped initial amplified spontaneous emission source). The arbitrary time-shaping scheme based on OPA provides a viable solution for the temporal waveform shaping of broadband low-coherence light. [ABSTRACT FROM AUTHOR]

We experimentally demonstrate a stable and compact high pulse energy mid-infrared (MIR) 6.45 μm laser, which is produced by an optical parametric oscillator (OPO) based on the non-oxide BaGa4Se7 (BGSe) nonlinear crystal pumped by 1064 nm Nd:YAG laser oscillator. With optimizing the parameters of the OPO system, a record high idler energy of 6.76 mJ at 6.45 μm was obtained with 18.85 ns of pulse duration (FWHM) at the repetition rate of 10 Hz under 93.5 mJ of pump energy, corresponding to an optical-to-optical conversion efficiency up to 7.23% from 1064 nm to 6.45 μm. The experimental results were in close approximation with the theoretical calculations. To date, it is both the highest MIR pulse energy and the highest conversion efficiency at 6.45 μm for any 1 μm pumped OPOs. Further, excellent output energy stability is demonstrated, with an energy fluctuation of less than ±0.5% over 165 min. Such a laser is interesting for both scientific and medical applications, including, for instance, for trace gas analysis and tissue ablation. [ABSTRACT FROM AUTHOR]