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Simple Summary: This review highlights the benefits of using valuable alternative feeds such as crop residues, silage, grasses, hay, browse, plant leaves, shrubs, and agro-industrial by-products in small ruminants' diets. Alternative feeds can significantly improve the productivity and reduce carbon footprints and GHG fluxes of small ruminant farms, making them both environmentally friendly and cost-effective. Additionally, these alternative feeds possess antioxidant, antimicrobial, and antiseptic properties that can enhance the quality of the meat and milk produced. Small ruminants, such as sheep (Ovisaries) and goats (Capra hircus), contribute to approximately 475 million metric tons of carbon dioxide equivalent (MtCO2e) greenhouse gas (GHG) emissions, accounting for approximately 6.5% of the global emissions in the agriculture sector. Crop residues, silage, grasses, hay, browse, plant leaves, shrubs, agro-industrial by-products, poultry litter, and other alternative feed sources are frequently utilized for small ruminant production. The use of these valuable alternative feeds can significantly improve animal productivity and reduce carbon footprints and GHG fluxes, making it both environmentally friendly and cost-effective. Additionally, these alternative feeds possess antioxidant, antimicrobial, and antiseptic properties that can enhance the quality of the meat and milk produced. By impacting the bacteria involved in ruminal biohydrogenation, alternative feeds can reduce methane emissions and contribute to a decrease in the carbon footprint. Overall, the use of alternative feed sources for small ruminants generally improves their apparent nutrient digestibility and productivity, and has an impact on the production of greenhouse gases, especially methane. Finally, this review recommends evaluating the economic analysis of reducing methane emissions in small ruminants by utilizing different feed sources and feeding techniques. [ABSTRACT FROM AUTHOR]