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Accurate urban boundary data can directly reflect the expansion of urban space, help us accurately grasp the scale and form of urban space, and play a vital role in urban land development and policy-making. However, the lack of reliable multiscale and high-precision urban boundary data products and relevant training datasets has become one of the major factors hindering their application. The purpose of this study is to combine Sentinel-2 remote-sensing images and supplementary geographic data to generate a reliable high-precision urban boundary dataset for Henan Province (called HNUB2018). First, this study puts forward a clear definition of "urban boundary". Using this concept as its basis, it proposes a set of operable urban boundary delimitation rules and technical processes. Then, based on Sentinel-2 remote-sensing images and supplementary geographic data, the urban boundaries of Henan Province are delimited by a visual interpretation method. Finally, the applicability of the dataset is verified by using a classical semantic segmentation deep learning model. The results show that (1) HNUB2018 has clear and rich detailed features as well as a detailed spatial structure of urban boundaries. The overall accuracy of HNUB2018 is 92.82% and the kappa coefficient reaches 0.8553, which is better than GUB (Henan) in overall accuracy. (2) HNUB2018 is well suited for deep learning, with excellent reliability and scientific validity. The research results of this paper can provide data support for studies of urban sprawl monitoring and territorial spatial planning, and will support the development of reliable datasets for fields such as intelligent mapping of urban boundaries, showing prospects and possibilities for wide application in urban research. [ABSTRACT FROM AUTHOR]