1. Importance of moderate size of pillars and dual-scale structures for stable superhydrophobic surfaces: A molecular dynamics simulation study.
- Author
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Li, Hao and Yan, Tianyu
- Subjects
- *
SUPERHYDROPHOBIC surfaces , *SURFACE dynamics , *HYDROPHOBIC surfaces , *DROP size distribution , *CONTACT angle , *MOLECULAR dynamics , *SURFACE states - Abstract
• Dual-scale structures are important for the stable Cassie state. • Small-scale structures can prevent the transition of Cassie-Wenzel. • Small-scale structures can facilitate the transition of Wenzel-Cassie. In this work, we first create three-dimensional molecular-dynamics (MD) model to study the effect of structure parameters including pillar size, pillar height, pillar groove, and intrinsic contact angle (θ e , or Young's angle) on wetting behavior of drops on the one-scale nanopillared surface. We find that drops tend to exhibit the Cassie state on the nanopillared surface with small pillar size and large θ e. Considering comprehensively the stability of the Cassie state, excellent hydrophobicity, and mechanical durability of microstructures, the pillar height and the pillar groove should be moderate. Then, only considering the wettability, we could see the dual-scale structure as the one-scale structure with large θ e * that results from the small-scale structure for increasing the θ e and cannot be achieved on the smooth surface in experiments. Importantly, we observe that the dual-scale structure, corresponding to large θ e * resulting from the small-scale structure for increasing the θ e , are important for the formation and the stability of the Cassie state. Moreover, the dual-scale structure can prevent the transition of drops from the Cassie state to the Wenzel state. Interestingly, fabricating the small-scale structure on top of the large-scale structure (corresponding to large θ e * of the one-scale structure) can facilitate the transformation of the Wenzel state of drops on the large-scale structure to the Cassie state, and the Cassie state is stable. This study provides an inspiration for the fabrication of stable artificial superhydrophobic surfaces. [ABSTRACT FROM AUTHOR]
- Published
- 2020
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