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Agriculture-sourced, non-point groundwater contamination (e.g., nitrate) is a serious concern from the drinking water crisis aspect across the agrarian world. India is one of the largest consumers of nitrogen fertilizers in South-Asia as well as in the world but groundwater nitrate lacks critical attention as a wide-scale drinking water pollutant in the country. Our study provides the first documentation of the distribution of groundwater nitrate and the extent of elevated nitrate contamination across India, along with the delineation of the temporal trends and the natural and anthropogenic factors that influence such occurrence of groundwater nitrate. High resolution, annual-scale spatio-temporal variability of groundwater nitrate concentration and consequent contamination was delineated using groundwater nitrate measurements from ~3 million drinking water wells spread across 7038 administrative blocks between 2010 and 2017 in India. An average 8% of the studied blocks were found affected by elevated groundwater nitrate (> 45 mg/L). Depth-dependent trend demonstrated that nitrate concentrations were about 14% higher in shallow water wells (≤ 35 m) than deep wells (>35 m). The overall temporal trend of groundwater nitrate concentration was decreasing slightly nationwide in the study period. The correlation tests and causality test results indicated that the spatial distribution of groundwater nitrate was significantly associated with agricultural N-fertilizer usage, whereas the decreasing temporal trend corresponded with the overall reduced N-fertilizer usage during the study period. Spatial autocorrelation analysis identified the clustering of high nitrate areas in central, north, and southern India, specifically in areas with higher fertilizer usage. We estimate about 71 million Indians possibly exposed to elevated groundwater nitrate concentrations and the majority of them reside in rural areas. Thus, this study provides the previously unrecognized, wide-scale, anthropogenic, diffused groundwater nitrate contamination across India. [Display omitted] • Groundwater nitrate pollution is delineated using ~3 million drinking-water wells. • Spatio-temporal trends of groundwater nitrate are analyzed for 2010–2017 in India. • Depth-dependence of groundwater nitrate concentration in the aquifer is delineated. • Rural and urban population exposed to groundwater nitrate pollution is estimated. [ABSTRACT FROM AUTHOR]

Fresh water resource of South Asia is becoming extremely stressed due to the rapid rate of groundwater depletion in recent times, particularly in the agriculture-heavy regions of India and Bangladesh. Among other factors, the relationship between climate variability and groundwater levels is critical for the security and sustainability of the water-food nexus. Thus, it is worthwhile to comprehend the poorly understood groundwater-climate continuum at basinal and sub-basinal scale. With the wavelet coherence analysis, we demonstrated the influence of global climate cycles on groundwater levels in the parts of the transboundary aquifer system of South Asia. Our findings suggest rapid groundwater response to the global climate patterns in shallow levels and relatively delayed groundwater response with increasing depth. However, this intuitive response is not visible in places with pervasive groundwater exploitation. Our findings also indicate that climate oscillations from the Pacific Ocean have a major influence on groundwater levels in the region. The findings would help in constructing resilience scenarios of groundwater impacted by climate variability and to take countermeasures, especially during climate-driven dry periods. [ABSTRACT FROM AUTHOR]