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Smøla island, situated within the mid-Norwegian passive margin, contains crystalline-basement-hosted intricate fracture and fault arrays formed during a polyphase brittle tectonic evolution. Its detailed study may strengthen correlation attempts between the well-exposed onshore domain and the inaccessible offshore domain, further the understanding of the passive margin evolution, and provide useful constraints on petrophysical properties of fractured basement blocks. A combination of geophysical and remote sensing lineament analysis, field mapping, high-resolution drill hole logging, 3D modelling, petrographic and microstructural studies, and fault gouge K–Ar geochronology made it possible to define five deformation episodes (D1 to D5). These episodes occurred between the post-Caledonian evolution of the regional-scale Møre–Trøndelag Fault Complex (MTFC) and the Late Cretaceous and younger crustal extension preceding the final stages of Greenland–Norway break-up. Each reconstructed deformation stage is associated with different structural features, fault and fracture geometries, and kinematic patterns. Synkinematic mineralisations evolved progressively from epidote–prehnite, sericite–chlorite–calcite, chlorite–hematite, hematite–zeolite–calcite, to quartz–calcite. K–Ar geochronology constrains brittle deformation to discrete localisation events spanning from the Carboniferous to the Late Cretaceous. Multiscalar geometrical modelling at scales of 100, 10, and 1 m helps constrain the extent and size of the deformation zones of each deformation episode, with D2 structures exhibiting the greatest strike continuity and D1 features the most localised. Overall, the approach highlighted here is of great utility for unravelling complex brittle tectonic histories within basement volumes. It is also a prerequisite to constrain the dynamic evolution of the petrophysical properties of basement blocks.