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Bathing water quality standards are based on international standards and legislations. However, in Europe, only the microbiological parameters are to be accomplished. Recent research has focused on chemical indicators that can determine human fecal contaminants in water. Therefore, the suitability of caffeine as a chemical marker of seawater pollution in the north Portuguese coastal area in the Atlantic Ocean during the bathing season was assessed in this study. The quality of water from the coasts of five cities was monitored. 101 seawater samples were collected from 14 beaches, and their water quality was classified as sufficient, good, and excellent. Caffeine was detected in all samples in concentration range of 18 to 525 ng/L. The highest average concentration of caffeine was found in seawater samples collected in July from beaches classified as having sufficient water quality, which were located in cities with high population density and high tourist affluence. [ABSTRACT FROM AUTHOR]

Abstract: The concentrations of 18 polycyclic aromatic hydrocarbons (PAHs) were determined in three commercially valuable fish species (sardine, Sardina pilchardus; chub mackerel, Scomber japonicus; and horse mackerel, Trachurus trachurus) from the Atlantic Ocean. Specimens were collected seasonally during 2007–2009. Only low molecular weight PAHs were detected, namely, naphthalene, acenaphthene, fluorene and phenanthrene. Chub mackerel (1.80–19.90μg/kgww) revealed to be significantly more contaminated than horse mackerel (2.73–10.0μg/kgww) and sardine (2.29–14.18μg/kgww). Inter-specific and inter-season comparisons of PAHs bioaccumulation were statistically assessed. The more relevant statistical correlations were observed between PAH amounts and total fat content (significant positive relationships, p ⩽0.05), and season (sardine displayed higher amounts in autumn–winter while the mackerel species showed globally the inverse behavior). The health risks by consumption of these species were assessed and shown to present no threat to public health concerning PAH intakes. [Copyright &y& Elsevier]