1. Room-temperature sub-100 nm N\'eel-type skyrmions in non-stoichiometric van der Waals ferromagnet $\rm Fe_{3-x}GaTe_{2}$ with ultrafast laser writability
- Author
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Li, Zefang, Zhang, Huai, Li, Guanqi, Guo, Jiangteng, Wang, Qingping, Deng, Ying, Hu, Yue, Hu, Xuange, Liu, Can, Qin, Minghui, Shen, Xi, Yu, Richeng, Gao, Xingsen, Liao, Zhimin, Liu, Junming, Hou, Zhipeng, Zhu, Yimei, and Fu, Xuewen
- Subjects
Condensed Matter - Materials Science - Abstract
Realizing room-temperature magnetic skyrmions in two-dimensional van der Waals ferromagnets offers unparalleled prospects for future spintronic applications. However, due to the intrinsic spin fluctuations that suppress atomic long-range magnetic order and the inherent inversion crystal symmetry that excludes the presence of the Dzyaloshinskii-Moriya interaction, achieving room-temperature skyrmions in 2D magnets remains a formidable challenge. In this study, we target room-temperature 2D magnet $\rm Fe_3GaTe_2$ and unveil that the introduction of iron-deficient into this compound enables spatial inversion symmetry breaking, thus inducing a significant Dzyaloshinskii-Moriya interaction that brings about room-temperature N\'eel-type skyrmions with unprecedentedly small size. To further enhance the practical applications of this finding, we employ a homemade in-situ optical Lorentz transmission electron microscopy to demonstrate ultrafast writing of skyrmions in $\rm Fe_{3-x}GaTe_2$ using a single femtosecond laser pulse. Our results manifest the $\rm Fe_{3-x}GaTe_2$ as a promising building block for realizing skyrmion-based magneto-optical functionalities.
- Published
- 2024
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