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Nonintrusive velocity measurements using femtosecond laser electronic excitation tagging (FLEET) were conducted at 1 kHz for both air and nitrogen flows in a Mach 6 Ludwieg tube under ~600 Pa static pressure conditions. The signal from air and nitrogen were compared in freestream conditions and with a blunt cone model (7 deg half-angle). The long-laser time series operation relative to the facility operation time allowed the characterization of the mean velocity over the entire tunnel operation. The measurement uncertainty for both air and nitrogen FLEET were thoroughly examined. Our finding shows that the measured freestream velocity differed by ~1-2% from that of the compressible flow calculations. Additionally, the velocity near the leading bow shock was measured at six and three locations in nitrogen and air, respectively, to resolve the large velocity gradient at several locations along the shock layer. The velocity results for the freestream and bow shock were averaged in space and time. [ABSTRACT FROM AUTHOR]

The prediction of flowfield evolution can provide valuable reference information for the development of hypersonic technology. Flowfield prediction with the introduction of deep learning techniques is a promising method to provide future flowfield evolution in scramjet isolators. A multipath flowfield prediction model has been proposed to achieve flowfield prediction based on wall pressure sequence. The prediction model is mainly constructed with a convolutional neural network. An experimental dataset was built with supersonic experimental data under different evolution laws in an isolator. The flowfield prediction model is trained and validated using independent experimental data. The proposed model's prediction performance under different prediction spans is discussed in depth. The results demonstrate that the predicted flowfield is in good agreement with the ground truth, and the background wave and shock train structure are basically restored, even when the shock train leading edge changes intermittently. The influence of pressure sequence length on the proposed model's prediction performance is also analyzed. [ABSTRACT FROM AUTHOR]

Direct measurements of the slip velocity in rarefied gas flows produced by local thermodynamic non-equilibrium at the wall represent crucial information for the validation of existing theoretical and numerical models. In this work, molecular tagging velocimetry (MTV) by direct phosphorescence is applied to argon and helium flows at low pressures in a 1-mm deep channel. MTV has provided accurate measurements of the molecular displacement of the gas at average pressures of the order of 1 kPa. To the best of our knowledge, this work reports the very first flow visualizations of a gas in a confined domain and in the slip flow regime, with Knudsen numbers up to 0.014. MTV is cross-validated with mass flowrate measurements by the constant volume technique. The two diagnostic methods are applied simultaneously, and the measurements in terms of average velocity at the test section are in good agreement. Moreover, preliminary results of the slip velocity at the wall are computed from the MTV data by means of a reconstruction method.

Molecular tagging velocimetry (MTV) is a nonintrusive velocimetry technique based on laser spectroscopy. It is particularly effective in challenging gas flow conditions encountered in thermal hydraulics where particle-based methods such as particle image (or tracking) velocimetry do not perform well. The main principles for designing and operating this diagnostic are presented as well as a set of gases that have been identified as potential seeds. Two gases [H2O and nitrous oxide (N2O)] have been characterized extensively for thermodynamic conditions ranging from standard temperature and pressure to environments encountered in integral effects test (IET) facilities for high-temperature gas reactors. A flexible, modular, and transportable laser system has been designed and demonstrated with H2O and N2O seed gases. The laser system enables determining the optimum excitation wavelength, tracer concentration, and timing parameters. Velocity precision and thermodynamic domain of applicability are discussed for both tracers. The spectroscopic nature of the diagnostics enables one to perform first-principle uncertainty analysis, which makes it attractive for validating numerical models. Molecular tagging velocimetry is demonstrated for two flows. First, in blowdown tests with H2O seed, the unique laser system enables one of the largest dynamic ranges reported to date for velocimetry: 5000:1 (74 dB). N2O-MTV is then deployed in situ in an IET facility, i.e., the High-Temperature Test Facility at Oregon State University, during a depressurized conduction cooldown (DCC) event. Data enable researchers to gain insights into flow instabilities present during DCC. Thus, MTV shows a strong potential to gain a fundamental understanding of gas flows in nuclear thermal hydraulics and to provide validation data for numerical solvers. [ABSTRACT FROM AUTHOR]

Femtosecond laser electronic excitation tagging (FLEET) is a molecular tagging velocimetry technique that can be applied in combustion flow fields, although detailed studies of its application in combustion are still needed. We report the applicability of FLEET in premixed CH4–air flames. We found that FLEET can be applied in all of the combustion areas (e.g., the unburned region, the burned region and the reaction zone). The FLEET signal in the unburned region is significantly higher than that in the burned region. This technique is suitable for both lean and rich CH4–air combustion flow fields and its performance in lean flames is better than that in rich flames. [ABSTRACT FROM AUTHOR]

Highlights • New data on acetone and diacetyl phosphorescence at low pressure are provided. • Phosphorescence intensity is optimized as a function of the excitation wavelength. • He with 5–10% of acetone tagged at 310 nm exhibits strong phosphorescence at 1 kPa. • MTV is able to analyze internal gas flows in the slip flow regime. • Extraction of velocity from displacement profiles is possible in the slip flow regime. Abstract Rarefied gas flows have a central role in microfluidic devices for many applications in various scientific fields. Local thermodynamic non-equilibrium at the wall-gas interface produces macroscopic effects, one of which is a velocity slip between the gas flow and the solid surface. Local experimental data able to shed light on this physical phenomenon are very limited in the literature. The molecular tagging velocimetry (MTV) could be a suitable technique for measuring velocity fields in gas micro flows. However, the implementation of this technique in the case of confined and rarefied gas flows is a difficult task: the reduced number of molecules in the system, which induces high diffusion, and the low concentration of the molecular tracer both drastically reduce the intensity and the duration of the exploitable signal for carrying out the velocity measurements. This work demonstrates that the application of the 1D-MTV by direct phosphorescence to gas flows in the slip flow regime and in a rectangular long channel is, actually, possible. New experimental data on phosphorescence emission of acetone and diacetyl vapors at low pressures are presented. An analysis of the optimal excitation wavelength is carried out to maximize the intensity and the lifetime of the tracer emission. The experimental results demonstrate that a low concentration of about 5–10% of acetone vapor excited at 310 nm or of diacetyl vapor excited at 410 nm in a helium mixture at pressures on the order of 1 kPa provides an intense and durable luminescent signal. In a 1-mm deep channel, a gas flow characterized by these thermodynamic conditions is in the slip flow regime. Moreover, numerical experiments based on DSMC simulations are carried out to demonstrate that an accurate measurement of the velocity profile in a laminar pressure-driven flow is possible for the rarefied conditions of interest. [ABSTRACT FROM AUTHOR]

The effects of light‐driven enhancement of Evans Blue dye complexes with blood plasma proteins were observed for the first time, both in vitro and in vivo. The possible background of the effect concerns the photochemical cis‐trans isomerization of the azo dye molecules. The effect was induced in the solution with a red laser with a wavelength of 638 nm, which corresponds to the peak of the dye absorption. The lifetime of the enhanced fluorescence is approximately 1 second and enables its use as an optically tagged molecular flow tracer for blood flow velocity measurements. Utilizing the effect, we performed for the first time the intravital molecular tagging velocimetry of the blood velocity in blood vessels in a living animal. The results of the measurements of the blood flow velocities in the cerebral veins of a group of healthy mice are presented. [ABSTRACT FROM AUTHOR]

Background: The molecular rotor 9-(2-Carboxy-2-cyanovinyl)julolidine (CCVJ) is presumed to have a sensitivity towards velocity or shear which is supposed to result in a change in fluorescence quantum yield. Furthermore, a previously reported photoisomeric behavior may contribute to the measured fluorescence intensity changes. The goal of this research was to examine the hypothesized behavior theoretically and experimentally from the perspective of fluid dynamics. Results: A correlation between stirring rate and intensity could not be established in the present experiments with a completely illuminated sample in contrast to previously reported experiments in spectrofluorometers. Experiments and theoretical models of a Poiseuille flow were in good agreement with the photoisomeric behavior but excluded the influence of shear. Further experiments in a flow chamber supported the photoisomery hypothesis as well. Conclusion: No experimental evidence for the influence of velocity on the fluorescence intensity of CCVJ was found. The hypothesis of shear sensitivity was excluded as well. The results are consistent with the photoisomeric behavior of CCVJ. [ABSTRACT FROM AUTHOR]

Molecular tagging velocimetry is a little-intrusive technique based on the properties of specific molecules able to emit luminescence once properly excited. Several variants of this technique have been successfully developed for analyzing external gas flows or internal gas flows in large systems. There is, however, very few experimental data on molecular tagging velocimetry for gas flows in mini or microsystems, and these data are strongly affected by the molecular diffusion of the tracer molecules. In the present paper, it is demonstrated that the velocity field in gas microflows cannot be directly deduced from the measured displacement field without taking into account Taylor dispersion effects. For that purpose, the benchmark case of a Poiseuille gas flow through a rectangular channel 960 μm in depth is experimentally investigated by micro molecular tagging velocimetry using acetone vapor as a molecular tracer. An appropriate reconstruction method based on the advection diffusion equation is used to process the data and to correctly extract the velocity profiles. The comparison of measured velocities with flowrate data and with theoretical velocity profiles shows a good agreement, whereas when the reconstruction method is not implemented, the extracted velocity field exhibits qualitative and quantitative anomalies, such as a non-physical slip at the walls. The robustness of the reconstruction method is demonstrated on flows with light and heavy molecular species, namely helium and argon, at atmospheric as well as at lower pressure conditions, for which diffusion effects are stronger. The obtained results represent an encouraging step for future analysis of rarefied gas microflows. [ABSTRACT FROM AUTHOR]

In this paper, a new type of molecular tagging velocimetry based on NH fluorescence was developed and validated for the velocity measurements of a high-enthalpy rarefied gas wind tunnel where the maximum flow velocity exceeds 6 km/s near the nozzle exit at 0.2 Pa. The feasibility of this technique using the short-lived NH fluorescence was demonstrated in the hypersonic rarefied gas flow with yielding velocity profiles at multiple downstream locations from the nozzle exit. The total uncertainty of the measured flow velocities was estimated to be less than 6% when the flow velocity is above 2000 m/s. For the new tagging technique, only a single laser and a single time-gated camera are required for velocity measurement, due to the existence of NH radicals in the arc-discharged N mixed with a small amount of H. Therefore, the NH-MTV not only shows great promise for tagging in high-enthalpy rarefied gas of nitrogen or air flows without seeding, but also possesses high practicability and facility for velocity measurement. [ABSTRACT FROM AUTHOR]

The molecular tagging velocimetry (MTV) is a well-suited technique for velocity field measurement in gas flows. Typically, a line is tagged by a laser beam within the gas flow seeded with light emitting acetone molecules. Positions of the luminescent molecules are then observed at successive times and the velocity field is deduced from the analysis of the tagged line displacement and deformation. However, the displacement evolution is expected to be affected by molecular diffusion, when the gas is rarefied. Therefore, there is no direct and simple relationship between the velocity field and the measured displacement of the initial tagged line. This paper addresses the study of tracer molecules diffusion through a background gas flowing in a channel delimited by planar walls. Tracer and background species are supposed to be governed by a system of coupled Boltzmann equations, numerically solved by the direct simulation Monte Carlo (DSMC) method. Simulations confirm that the diffusion of tracer species becomes significant as the degree of rarefaction of the gas flow increases. It is shown that a simple advection-diffusion equation provides an accurate description of tracer molecules behavior, in spite of the non-equilibrium state of the background gas. A simple reconstruction algorithm based on the advection-diffusion equation has been developed to obtain the velocity profile from the displacement field. This reconstruction algorithm has been numerically tested on DSMC generated data. Results help estimating an upper bound on the flow rarefaction degree, above which MTV measurements might become problematic. [ABSTRACT FROM AUTHOR]

This review article reports the recent progress in the development of a new group of molecule-based flow diagnostic techniques, which include molecular tagging velocimetry (MTV) and molecular tagging thermometry (MTT), for both qualitative flow visualization of thermally induced flow structures and quantitative whole-field measurements of flow velocity and temperature distributions. The MTV and MTT techniques can also be easily combined to result in a so-called molecular tagging velocimetry and thermometry (MTV&T) technique, which is capble of achieving simultaneous measurements of flow velocity and temperature distribution in fluid flows. Instead of using tiny particles, the molecular tagging techniques (MTV, MTT, and MTV&T) use phosphorescent molecules, which can be turned into long-lasting glowing marks upon excitation by photons of appropriate wavelength, as the tracers for the flow velocity and temperature measurements. The unique attraction and implementation of the molecular tagging techniques are demonstrated by three application examples, which include: (1) to quantify the unsteady heat transfer process from a heated cylinder to the surrounding fluid flow in order to examine the thermal effects on the wake instabilities behind the heated cylinder operating in mixed and forced heat convection regimes, (2) to reveal the time evolution of unsteady heat transfer and phase changing process inside micro-sized, icing water droplets in order to elucidate the underlying physics pertinent to aircraft icing phenomena, and (3) to achieve simultaneous droplet size, velocity and temperature measurements of 'in-flight' droplets to characterize the dynamic and thermodynamic behaviors of flying droplets in spray flows. [ABSTRACT FROM AUTHOR]

Particle image velocimetry (PIV) has become a powerful tool for flow velocity measurements in wind tunnel testing. However, it is generally difficult to apply the PIV technique to supersonic flows because of unreliable particle traceability. In the present study, the PIV and MTV (molecular tagging velocimetry) techniques are applied to transonic and supersonic flows, in which a normal shock wave appears, to evaluate particle traceability. Based on this work, it is found that the PIV data largely deviate from the MTV data behind a normal shock wave for both flows. The drag coefficient is also estimated for a particle from the velocity data measured by the two techniques. Its value is then compared to the drag coefficient value calculated from an empirical formula for particle Mach numbers ranging between 0.1 and 0.9. Based on the results, it is found that the experimental data can be reproduced reasonably well by the formula for particle Reynolds numbers higher than ~1. However, the data associated with particle Reynolds numbers lower than ~1 deviate largely from the formula. Graphical abstract: [Figure not available: see fulltext.] [ABSTRACT FROM AUTHOR]

Recent advances in ultra-high repetition rate (100 kHz and above) laser diagnostics for fluid dynamic measurements are reviewed. The development of the pulse burst laser system, which enabled several of these advances, is described. The pulse burst laser system produces high repetition rate output by slicing the output of a low power continuous wave laser and passing the resulting burst of pulses through a series of pulsed Nd:YAG amplifiers. Several systems have been built with output approaching 1.0 J/pulse over bursts of up to 100 pulses generated at between 50 and 1000 kHz. Combined with the capabilities of several types of commercially available high-speed cameras, these systems have been used to make a wide variety of high repetition rate and 3D flow measurements. Several examples of various high repetition rate laser diagnostics are described, including flow visualization, filtered Rayleigh scattering, planar Doppler velocimetry, particle image velocimetry, planar laser induced fluorescence, molecular tagging velocimetry and 3D flow visualization. [ABSTRACT FROM AUTHOR]

Laser measurement techniques are becoming more commonly applied to many areas of thermofluids and heat transfer. An area of their application, which presents highly challenging requirements, is in the measurement of aerospace flows. In this case the experimentalist may encounter high mass flowrates, high-speed flows and in some cases high temperatures, and the measurements may also have to be taken with restricted optical access. Such types of flow have already been measured using established laser techniques such as particle image velocimetry, laser Doppler anemometry, laser-induced fluorescence and liquid crystal thermography. Other more recent techniques which have seen application include Doppler global velocimetry and molecular tagging velocimetry for velocity measurement and thermographic phosphor thermometry for surface temperature measurement. This paper reviews the most recent advances in laser techniques and their application to aerospace environments. [ABSTRACT FROM AUTHOR]

Femtosecond laser electronic excitation tagging (FLEET) is a new non-seed molecular tagging velocity measurement method. Fluorescent light excited by femtosecond laser is used as tagging filament, and will disturb local temperature which may affect the flow field measurement precision. In this paper, the Rayleigh scattered of nanosecond laser is used to measure the ambient air temperature changing. The feasibility of this measurement method is proved. The key data processing of low signal to noise ratio (SNR) images including the filament segmentation, noise filtering, skeleton extraction of filament position is tested. The preliminary test on the heating process between 1 us and 800 us is demonstrated. The limitations of this measurement method due to the gas media condition changing are discussed briefly. [ABSTRACT FROM AUTHOR]

Direct measurements of the slip velocity in rarefied gas flows produced by local thermodynamic non-equilibrium at the wall represent crucial information for the validation of existing theoretical and numerical models. In this work, molecular tagging velocimetry (MTV) by direct phosphorescence is applied to argon and helium flows at low pressures in a 1-mm deep channel. MTV has provided accurate measurements of the molecular displacement of the gas at average pressures of the order of 1 kPa. To the best of our knowledge, this work reports the very first flow visualizations of a gas in a confined domain and in the slip flow regime, with Knudsen numbers up to 0.014. MTV is cross-validated with mass flowrate measurements by the constant volume technique. The two diagnostic methods are applied simultaneously, and the measurements in terms of average velocity at the test section are in good agreement. Moreover, preliminary results of the slip velocity at the wall are computed from the MTV data by means of a reconstruction method. [ABSTRACT FROM AUTHOR]