Search

We investigated the characteristics of the total ozone column (TOC) around West Antarctica (near the Weddell Sea) compared with ambient meteorological factors. For this analysis, we used ground-based and satellite TOC measurements as well as meteorology (air temperature, potential vorticity and wind field) from reanalysis data. Long-term patterns of TOC show the large year-to-year variation (e.g., maximumly ∼200 DU at King Sejong) but a steady recovering trend recently. Despite a generally consistent pattern, the TOC around West Antarctica did not correlate well between high- and low-latitude regions during austral spring; this result implies that the ozone hole area had a spatial variation over West Antarctica. The TOC pattern around West Antarctica correlated well with air temperature but showed a vertical difference; high positive correlations appeared in the lower stratosphere (maximumly R > 0.9 at ∼50–100 hPa height) showing enhanced ozone depletion in colder conditions, but negative correlations appeared in the upper stratosphere (minimum R 0.9 at ∼500–600 K height) during the austral spring but a moderately negative correlation in the lower stratosphere (minimum R

Spring dust frequency in northeast Asia has been investigated using various approaches to understand the mechanisms of dust emission and transport. However, little attention has been paid to the linkage between dust activity and the Siberian High (SH), particularly when the SH pressure system is highly variable. In this study, we characterize the possible physical mechanisms of dust emission and transport associated with the Siberian High Intensity (SHI) and Siberian High Position Index (SHPI) in March using 18 years of ground-based observations and reanalysis data. We found that when the SHI was strong and the SH’s center was farther east (“Strong–East period”), surface and atmospheric temperatures were cooler than when the SHI was weak and the SH’s center was farther west (“Weak-West period”), due to anomalous anticyclonic pressure and strong easterlies. As a result, a reduction in the meridional temperature gradient in the lower atmosphere suppressed dust emission and transport, due to stagnant atmospheric conditions. This anomalous anticyclonic pressure in the Strong-East case seems to reduce the development of extratropical cyclones (ETC) in northeast Asia, leading to a less effective dust transport. A case study with composite analysis also showed a similar physical mechanism: stagnant air accompanying weakened westerlies in the Strong-East period suppressed dust transport to South Korea. Our findings reveal that the intensity and position of the SH can be utilized to identify spring transboundary air pollutants in northeast Asia.

By using multiple satellite measurements, the changes of the aerosol optical depth (AOD) and nitrogen dioxide (NO2) over South Korea were investigated from January to March 2020 to evaluate the COVID-19 effect on the regional air quality. The NO2 decrease in South Korea was found but not significant, which indicates the effects of spontaneous social distancing under the maintenance of ordinary life. The AODs in 2020 were normally high in January, but they became lower starting from February. Since the atmosphere over Eastern Asia was unusually stagnant in January and February 2020, the AOD decrease in February 2020 clearly reveals the positive effect of the COVID-19. Considering the insignificant NO2 decrease in South Korea and the relatively long lifetime of aerosols, the AOD decrease in South Korea may be more attributed to the improvement of the air quality in neighboring countries. In March, regional atmosphere became well mixed and ventilated over South Korea, contributing to large enhancement of air quality. While the social activity was reduced after the COVID-19 outbreak, the regional meteorology should be also examined significantly to avoid the biased evaluation of the social impact on the change of the regional air quality.

Solar irradiance derived from satellite imagery is useful for solar resource assessment, as well as climate change research without spatial limitation. The University of Arizona Solar Irradiance Based on Satellite–Korea Institute of Energy Research (UASIBS-KIER) model has been updated to version 2.0 in order to employ the satellite imagery produced by the new satellite platform, GK-2A, launched on 5 December 2018. The satellite-derived solar irradiance from UASIBS-KIER model version 2.0 is evaluated against the two ground observations in Korea at instantaneous, hourly, and daily time scales in comparison with the previous version of UASIBS-KIER model that was optimized for the COMS satellite. The root mean square error of the UASIBS-KIER model version 2.0, normalized for clear-sky solar irradiance, ranges from 4.8% to 5.3% at the instantaneous timescale when the sky is clear. For cloudy skies, the relative root mean square error values are 14.5% and 15.9% at the stations located in Korea and Japan, respectively. The model performance was improved when the UASIBS-KIER model version 2.0 was used for the derivation of solar irradiance due to the finer spatial resolution. The daily aggregates from the proposed model are proven to be the most reliable estimates, with 0.5 km resolution, compared with the solar irradiance derived by the other models. Therefore, the solar resource map built by major outputs from the UASIBS-KIER model is appropriate for solar resource assessment.

The attenuating effects of clouds and aerosols on global horizontal irradiance (GHI) and ultraviolet erythemal irradiance (UVER) were evaluated and compared using data from four sites in South Korea (Gangneung, Pohang, Mokpo, and Gosan) for the period 2005&ndash, 2016. It was found that GHI and UVER are affected differently by various attenuating factors, resulting in an increase in the ratio of UVER to GHI with a decrease in the clearness index of GHI. A comparative analysis of the clearness indices of GHI and UVER identified an almost linear relationship between two transmittances by applying UVER with fixed slant ozone ( UVER 300 ) and there was a latitudinal difference in the relationship. Some nonlinearity remained in this relationship, which suggests a contribution by other factors such as clouds and aerosols. Variations of the UVER 300 ratio to GHI with cloud cover and aerosol optical depth were analyzed. The ratio increased with cloud cover and decreased with aerosol optical depth, indicating that clouds attenuate GHI more efficiently than UVER and that the attenuation by aerosols is greater for UVER than for GHI. A multiple linear regression analysis of the clearness indices of GHI and UVER 300 quantitively demonstrates differences in the radiation-reducing effects of clouds and aerosols, with some regional differences by site that can be attributed to local climatic characteristics in South Korea.

This study examines the semi-empirical models to evaluate the atmospheric broadband transmission of erythemally weighted ultraviolet (EUV), total ultraviolet (TUV), and global solar radiation (GS) by clouds, aerosols, and ozone in Seoul, Korea (37.57°N, 128.98°E). Climatological values of surface solar irradiance (SSI) for Seoul are briefly summarized, and atmospheric transmission is defined as the ratio of measured SSI to clear-sky irradiance calculated using harmonic analysis. Three multiple linear regression models are developed for the EUV, TUV, and GS spectral bands for all-sky (clear and cloudy conditions) transmission using three independent variables: cloud-cover amount, aerosol optical depth, and total ozone. The modeled total transmissions are 75%, 71%, and 67% for the EUV, TUV, and GS spectral bands, respectively, which are slightly overestimated than the measured values. The modeled annual mean clearness index, KT, is 1%, 45%, and 48% for the three spectral bands, respectively. Four semi-empirical models were developed to calculate transmission and were evaluated. Among the various empirical models, estimates from the exponential models were found to be the closest to measured values, having the lowest mean bias error (−0.3% to −2.4%) and highest explained variance (R2 = 0.17 to 0.50; p = 0.000), as was expected from their theoretical bases. The annual average transmissions of cloud, aerosol, ozone, and all three combined show decrease from the EUV to the TUV and GS bands.

Using NASA’s Modern-Era Retrospective Analysis for Research and Applications, version 2 (MERRA-2) reanalysis for aerosol optical depth (AOD) and satellite-observed carbon monoxide (CO) data, we examined the basic pattern of AOD variations over the three polar stations of Korea: the Jangbogo and King Sejong stations in Antarctica and the Dasan station in the Arctic. AOD values at the King Sejong and Dasan stations show maximum peaks in spring and appear to be associated with large amounts of atmospheric CO emitted from natural burning and biomass burning. The Jangbogo station shows a much lower AOD than the other two stations and does not appear to be strongly affected by the transport of airborne particles generated from mid-latitude regions. All three polar stations show an increasing trend in AOD in general, indicating that the polar background air quality is becoming polluted.

In this study, we present and compare regional correlations between CO total column density (TCD CO ) from the data set of Measurement of Pollution in the Troposphere (MOPITT), and high-absorbing BC dominant aerosol optical depth (AOD BC ) from the retrieval algorithm using Moderate Resolution Imaging Spectroradiometer (MODIS) and Ozone Monitoring Instrument (OMI) (MODIS-OMI algorithm, MOA). TCD CO shows positive relationship to both fine-mode AOD (AOD FM ) and AOD BC in general, but TCD CO better correlates with AOD BC than AOD FM . This enhanced correlation between TCD CO and AOD BC appears more clearly during spring and summer. Correlation between TCD CO and AOD BC is exceptionally poor in Northern Africa where the BC-dominated aerosols are frequently mixed with mineral dust particles from the Sahara. Another issue is also found in Southern Africa; the correlation between AOD BC and TCD CO in this region is not much higher than that between the AOD FM and TCD CO in spite of large occurrence of biomass burning and wildfire. This can be explained by the cloud perturbation near the source regions and dispersion effect due to the typical wind pattern. Correlations between AOD BC and TCD CO increase further when fire detected areas are only considered, but does not change much over the urban area. This difference clarifies the large contribution of burning events to the positive relationship between BC and CO. All findings in this study demonstrate a possible use of satellite CO product in evaluating the BC-dominated aerosol product from satellite remote sensing over the globe.

It is important to estimate the effects of the long-range transport of atmospheric pollutants for efficient and effective strategies to control air quality. In this study, the contributions of trans-boundary transport to the mean concentrations of SO 2 , NO 2 , CO, and PM 10 in Seoul, Korea from 2001 to 2014 were estimated based on the conditional potential source contribution function (CPSCF) method. Eastern China was found to be the major source of trans-boundary pollution in Seoul, but moderate sources were also located in northeastern China. The contribution of long-range transport from Japan was negligible. The spatial distributions of the potential source contribution function (PSCF) values of each pollutant showed reasonable consistency with their emission inventory and satellite products. The PSCF values of SO 2 and PM 10 from eastern China were higher than those of NO 2 and CO. The mean concentrations of SO 2 , NO 2 , CO, and PM 10 in Seoul for the period from 2001 to 2014 were 5.34, 37.0, and 619.1 ppb, and 57.4 4 μg/m 3 , respectively. The contributions of long-range transport to the mean concentrations of SO 2 , NO 2 , CO, and PM 10 in Seoul were 0.74, 3.4, and 39.0 ppb, and 12.1 μg/m 3 , respectively, which are 14%, 9%, 6%, and 21% of the mean concentrations, respectively. The annual mean concentrations of SO 2 and NO 2 followed statistically significant increasing linear trends (0.5 and 1.6 ppb per decade, respectively), whereas the trends in the annual mean concentrations of CO and PM 10 were statistically insignificant. The trends in the ratio of the increased concentrations associated with long-range transport to the annual mean concentrations of the pollutants were statistically insignificant. However, the results indicate that the trans-boundary transport of SO 2 , NO 2 , CO, and PM 10 from eastern China consistently affected air quality in Seoul over the study period (2001–2014). Regionally, the effects of the long-range transport of pollutants from Beijing and Harbin-Changchun on air quality in Seoul have become more significant over this period.

Springtime trans-Pacific transport of Asian air pollutants has been investigated in many ways to figure out its mechanism. Based on the Western Pacific (WP) pattern, one of climate variabilities in the Northern Hemisphere known to be associated with the pattern of atmospheric circulation over the North Pacific Ocean, in this study, we characterize the pattern of springtime trans-Pacific transport using long-term satellite measurements and reanalysis datasets. A positive WP pattern is characterized by intensification of the dipole structure between the northern Aleutian Low and the southern Pacific High over the North Pacific. The TOMS/OMI Aerosol Index (AI) and MOPITT CO show the enhancement of Asian pollutant transport across the Pacific during periods of positive WP pattern, particularly between 40 and 50°N. This enhancement is confirmed by high correlations of WP index with AI and CO between 40 and 50°N. To evaluate the influence of the WP pattern, we examine several cases of trans-Pacific transport reported in previous research. Interestingly, most trans-Pacific transport cases are associated with the positive WP pattern. During the period of negative WP pattern, reinforced cyclonic wave breaking is consistently found over the western North Pacific, which obstructs zonal advection across the North Pacific. However, some cases show the trans-Pacific transport of CO in the period of negative WP pattern, implying that the WP pattern is more influential on the transport of particles mostly emitted near ∼40°N. This study reveals that the WP pattern can be utilized to diagnose the strength of air pollutant transport from East Asia to North America.

To assess air pollution emitted in Southern Hemisphere mid-latitudes and transported to Antarctica, we investigate the climatological mean and temporal trends in aerosol optical depth (AOD), carbon monoxide (CO), nitrogen dioxide (NO2), and formaldehyde (HCHO) columns using satellite observations. Generally, all these measurements exhibit sharp peaks over and near the three nearby inhabited continents: South America, Africa, and Australia. This pattern indicates the large emission effect of anthropogenic activities and biomass burning processes. High AOD is also found over the Southern Atlantic Ocean, probably because of the sea salt production driven by strong winds. Since the pristine Antarctic atmosphere can be polluted by transport of air pollutants from the mid-latitudes, we analyze the 10-day back trajectories that arrive at Antarctic ground stations in consideration of the spatial distribution of mid-latitudinal AOD, CO, NO2, and HCHO. We find that the influence of mid-latitudinal emission differs across Antarctic regions: western Antarctic regions show relatively more back trajectories from the mid-latitudes, while the eastern Antarctic regions do not show large intrusions of mid-latitudinal air masses. Finally, we estimate the long-term trends in AOD, CO, NO2, and HCHO during the past decade (2005–2016). While CO shows a significant negative trend, the others show overall positive trends. Seasonal and regional differences in trends are also discussed.

The threshold exposure time for synthesis of vitamin D was simulated by using a radiative transfer model considering variations in total ozone, cloud, and surface conditions. The prediction of total ozone took the form of an empirical linear regression with the variables of meteorological parameters in the upper troposphere and lower stratosphere and the climatology value of total ozone. Additionally, to consider cloud extinction after the estimation of clear-sky UV radiation using a radiative transfer model simulation, a cloud modification factor was applied. The UV irradiance was estimated at one-hour intervals, and then, to improve the temporal resolution of the exposure time simulation, it was interpolated to a one-minute resolution. Exposure times from the simulation clearly followed seasonal and diurnal cycles. However, upon comparison with observations, biases with large variations were found, and the discrepancy in the exposure time between the observations and simulations was higher in low UV irradiance conditions. The large deviations in the prediction errors for total ozone and the simplified assumption for the cloud modification factor contributed to the large deviations in exposure time differences between the model estimation and observations. To improve the accuracy of the simulated exposure time, improved predictions of total ozone with a more detailed cloud treatment will be essential.

We investigated aerosol optical depth (AOD) under background and polluted conditions using Aerosol Robotic Network (AERONET) and Visible Infrared Imaging Radiometer Suite (VIIRS) observations. The AOD data were separated into background, high, and median AOD (BAOD, HAOD, and MAOD, respectively) based on the cumulative AOD distribution at each point and then their spatiotemporal variations were analyzed. Persistent pollutant emissions from industrial activity in South Asia (SUA) and Northeast Asia (NEA) produced the highest BAOD values. Gridded-BAODs obtained from VIIRS Deep Blue AOD products showed widespread high-level BAOD over the oceans associated with transport from dust and biomass burning events. The temporal variations in BAOD and HAOD were generally consistent with that of MAOD, but differences were found in seasonal variation as well as in long-term trends in some regions. Southeast Asia (SEA) and South America/South Africa (SAM/SAF) showed similar HAOD levels owing to biomass burning, but BAODs were higher in SEA than in SAM/SAF. In NEA, BAOD was lowest during the summer rainy season, as opposed to the peaks in MAOD and HAOD. Long-term trends of the AODs show clear regional characteristics. The AODs have decreasing trends in NEA, Europe/Mediterranean basin, and Northeast America but increasing trends in SUA, North Africa, and the Middle East. The trend of HAOD in Northwest America and Australia was opposite to that of BAOD. The spatiotemporal patterns of the HAOD and BAOD provide detailed information on changes in aerosol loading compared to using only MAOD.

Ocean-atmosphere energy exchange is an important factor in the maintenance of oceanic and atmospheric circulation and the regulation of meteorological and climate systems. Oceanic sensible and latent heat fluxes around the Korean Peninsula were determined using satellite-based air-sea variables (wind speed, sea surface temperature, and atmospheric specific humidity and temperature) and the coupled ocean-atmosphere response experiment (COARE) 3.5 bulk algorithm for six years between 2014 and 2019. Seasonal characteristics of the marine heat flux and its short-term fluctuations during summer typhoons were also investigated. air-sea variables were produced through empirical relationships and verified with observational data from marine buoys around the Korean Peninsula. Satellite-derived wind speed, sea surface temperature, atmospheric specific humidity, and air temperature were strongly correlated with buoy data, with R2 values of 0.80, 0.97, 0.90, and 0.91, respectively. Satellite-based sensible and latent heat fluxes around the peninsula were also validated against fluxes calculated from marine buoy data, and displayed low values in summer and higher values in autumn and winter as the difference between air-sea temperature and specific humidity increased. Through analyses of spatio-temporal fluctuations in the oceanic turbulent heat flux and variations in intensities of typhoons, this study assessed the possibility of monitoring air-sea energy exchange using satellite-based ocean turbulent heat fluxes during high-impact weather.

Absorption and scattering characteristics of various aerosol events are investigated using 2-years of measurements from a skyradiometer at Yonsei University in Seoul, Korea. Both transported dust and anthropogenic aerosols are observed at distinct geo-location of Seoul, a megacity located a few thousand kilometers away from dust source regions in China. We focus on the wavelength dependence of Angstrom exponent (AE) and single scattering albedo (SSA), showing the characteristics of regional aerosols. The correlation between spectral SSAs and AEs calculated using different wavelength pairs generally indicates relatively weak absorption of fine-mode aerosols (urban pollution and/or biomass burning) and strong absorption of coarse-mode aerosols (desert dust) at this location. AE ratio (AER), a ratio of AEs calculated using wavelength pair between shorter (340–675 nm) and longer wavelength pair (675–1020 nm) correlates differently with SSA according to the dominant size of local aerosols. Correlations between SSA and AER show strong absorption of aerosols for AER 2.0. Based on the seasonal pattern of wavelength dependence of AER and SSA, this correlation difference looks to reveal the separated characteristics of transported dust and anthropogenic particles from urban pollution respectively. The seasonal characteristics of AER and SSAs also show that the skyradiometer measurement with multiple wavelengths may be able to detect the water soluble brown carbon, one of the important secondary organic aerosols in the summertime atmospheric composition.

Radiative transfer model simulations were used to investigate the erythemal ultraviolet (EUV) correction factors by separating the UV-A and UV-B spectral ranges. The correction factor was defined as the ratio of EUV caused by changing the amounts and characteristics of the extinction and scattering materials. The EUV correction factors (CFEUV) for UV-A [CFEUV(A)] and UV-B [CFEUV(B)] were affected by changes in the total ozone, optical depths of aerosol and cloud, and the solar zenith angle. The differences between CFEUV(A) and CFEUV(B) were also estimated as a function of solar zenith angle, the optical depths of aerosol and cloud, and total ozone. The differences between CFEUV(A) and CFEUV(B) ranged from −5.0% to 25.0% for aerosols, and from −9.5% to 2.0% for clouds in all simulations for different solar zenith angles and optical depths of aerosol and cloud. The rate of decline of CFEUV per unit optical depth between UV-A and UV-B differed by up to 20% for the same aerosol and cloud conditions. For total ozone, the variation in CFEUV(A) was negligible compared with that in CFEUV(B) because of the effective spectral range of the ozone absorption band. In addition, the sensitivity of the CFEUVs due to changes in surface conditions (i.e., surface albedo and surface altitude) was also estimated by using the model in this study. For changes in surface albedo, the sensitivity of the CFEUVs was 2.9%–4.1% per 0.1 albedo change, depending on the amount of aerosols or clouds. For changes in surface altitude, the sensitivity of CFEUV(B) was twice that of CFEUV(A), because the Rayleigh optical depth increased significantly at shorter wavelengths.

Surface NO2 volume mixing ratio (VMR) at a specific time (13:45 Local time) (NO2 VMRST) and monthly mean surface NO2 VMR (NO2 VMRM) are estimated for the first time using three regression models with Ozone Monitoring Instrument (OMI) data in four metropolitan cities in South Korea: Seoul, Gyeonggi, Daejeon, and Gwangju. Relationships between the surface NO2 VMR obtained from in situ measurements (NO2 VMRIn-situ) and tropospheric NO2 vertical column density obtained from OMI from 2007 to 2013 were developed using regression models that also include boundary layer height (BLH) from Atmospheric Infrared Sounder (AIRS) and surface pressure, temperature, dew point, and wind speed and direction. The performance of the regression models is evaluated via comparison with the NO2 VMRIn-situ for two validation years (2006 and 2014). Of the three regression models, a multiple regression model shows the best performance in estimating NO2 VMRST and NO2 VMRM. In the validation period, the average correlation coefficient (R), slope, mean bias (MB), mean absolute error (MAE), root mean square error (RMSE), and percent difference between NO2 VMRIn-situ and NO2 VMRST estimated by the multiple regression model are 0.66, 0.41, −1.36 ppbv, 6.89 ppbv, 8.98 ppbv, and 31.50%, respectively, while the average corresponding values for the other two models are 0.75, 0.41, −1.40 ppbv, 3.59 ppbv, 4.72 ppbv, and 16.59%, respectively. All three models have similar performance for NO2 VMRM, with average R, slope, MB, MAE, RMSE, and percent difference between NO2 VMRIn-situ and NO2 VMRM of 0.74, 0.49, −1.90 ppbv, 3.93 ppbv, 5.05 ppbv, and 18.76%, respectively.

Cloud and aerosol modification factors are investigated in the spectral range of ultraviolet (UV) to correct for cloud and aerosol extinction effects from clear sky irradiance. The cloud modification factor (CMF) and aerosol modification factor (AMF) are estimated using radiative transfer model (RTM) simulations and ground-based observations in Seoul, Korea. The modification factors show a spectral dependence within the spectral range of 300 to 360 nm, which is the range used to estimate erythemal UV. The CMF and AMF values are estimated with high spectral resolution with considerations of solar zenith angle (SZA), cloud/aerosol amount, and total ozone variation. From the simulation studies, the variation in the CMFs within the spectral range of 300–360 nm is estimated to be 0.031–0.055, which is twice as large as the decrease in CMFs resulting from a SZA increase of 10°. In addition, the CMFs estimated from observational data show significant spectral dependence, varying from 2.5% to 10.0%. Because of the small aerosol optical depth (AOD) value, however, the variation in the AMF calculated from simulations is estimated to be between 0.007 and 0.045, indicating lower spectral dependence than the CMF. Furthermore, the spectral difference in the AMF calculated from observational data is insignificant relative to the daily-averaged total ozone error and uncertainties related to the reference irradiance spectrum under aerosol-free conditions.

Atmospheric broadband transmissions of clouds, aerosols, and ozone in the erythemally weighted ultraviolet (EUV, 290–320 nm), total (spectrally integrated) ultraviolet (TUV, 290–363 nm), and total global solar (GS, 305–2800 nm) spectral regions were analysed with ground-based measurements in Seoul, Korea (37.57°N, 128.98°E) from March 2004 to February 2013. The annual average total transmission expressed as a fraction of the clear-sky irradiance was 77.6% in the EUV, 73.6% in the TUV, and 72.0% in the GS spectral regions. The corresponding values for cloud transmission were 78.4%, 73.9%, and 71.7%. In overcast cloudy conditions, atmospheric transmission was reduced by 45.9%, 50.2%, and 56.6% in the three spectral regions, respectively, indicating the dominant effect of clouds. Aerosol and ozone transmissions had almost the same annual average. Annual average atmospheric transmission effectively decreases with increasing wavelength from EUV to GS regions. However, we found that there was a difference in wavelength dependence of atmospheric transmission for monthly averages, which seems related to the monthly variation of total column ozone (TCO), aerosol, and cloud amount. It is also found that there is a critical value of TCO (TCO =370 DU) for the wavelength dependence of transmission. Higher ozone amount than this turnaround value can cause an increase in transmission from the EUV to GS regions. The monthly wavelength-dependent effects may be attributable more to the different climatological characteristics of the TCO rather than aerosols and clouds.

Recently, temporal changes in Aerosol Optical Thickness (AOT) have been investigated based on model simulations, satellite and ground-based observations. Most AOT trend studies used monthly or annual arithmetic means that discard details of the generally right-skewed AOT distributions. Potentially, such results can be biased by extreme values (including outliers). This study additionally uses percentiles (i.e., the lowest 5%, 25%, 50%, 75% and 95% of the monthly cumulative distributions fitted to Aerosol Robotic Network (AERONET)-observed and ECHAM/MESSy Atmospheric Chemistry (EMAC)-model simulated AOTs) that are less affected by outliers caused by measurement error, cloud contamination and occasional extreme aerosol events. Since the limited statistical representativeness of monthly percentiles and means can lead to bias, this study adopts the number of observations as a weighting factor, which improves the statistical robustness of trend estimates. By analyzing the aerosol composition of AERONET-observed and EMAC-simulated AOTs in selected regions of interest, we distinguish the dominant aerosol types and investigate the causes of regional AOT trends. The simulated and observed trends are generally consistent with a high correlation coefficient (R = 0.89) and small bias (slope±2σ = 0.75 ± 0.19). A significant decrease in EMAC-decomposed AOTs by water-soluble compounds and black carbon is found over the USA and the EU due to environmental regulation. In particular, a clear reversal in the AERONET AOT trend percentiles is found over the USA, probably related to the AOT diurnal cycle and the frequency of wildfires. In most of the selected regions of interest, EMAC-simulated trends are mainly attributed to the significant changes of the dominant aerosols; e.g., significant decrease in sea salt and water soluble compounds over Central America, increase in dust over Northern Africa and Middle East, and decrease in black carbon and organic carbon over Australia.