Search

The p-nuclei are the few stable nuclei heavier than iron on the neutron-deficient side of the valley of stability that cannot be produced through astrophysical neutron-capture reactions. The limited experimental data on reactions through which the p-nuclei might be produced leaves the origin of their production largely unknown. This work presents the first cross section measurements of the 76Se( α , γ )80Kr reaction. The rate of the time reversed reaction, 80Kr( γ , α )76Se, is one of the most uncertain of possible reactions which can occur at the 80Kr branching point on the γ-process photo-disintegration pathway. The reaction flow through 80Kr will directly affect the final abundance of the p-nuclide 78Kr. Experimental cross sections at two astrophysically relevant energies are reported and compared to cross sections calculated using Hauser-Feshbach codes talys , non-smoker , and smaragd . The success of these first ( α , γ ) cross section measurements performed in inverse kinematics in the energy region of the γ-process opens the door for future studies of reactions on radioactive γ-process nuclides.

During the slow neutron capture process in massive stars, reactions on light elements can both produce and absorb neutrons thereby influencing the final heavy element abundances. At low metallicities, the high neutron capture rate of 16-O can inhibit s-process nucleosynthesis unless the neutrons are recycled via the 17O(a,n)20Ne reaction. The efficiency of this neutron recycling is determined by competition between the 17O(a,n)20Ne and 17O(a,g)21Ne reactions. While some experimental data are available on the former reaction, no data exist for the radiative capture channel at the relevant astrophysical energies. The 17O(a,g)21Ne reaction has been studied directly using the DRAGON recoil separator at the TRIUMF Laboratory. The reaction cross section has been determined at energies between 0.6 and 1.6 MeV Ecm, reaching into the Gamow window for core helium burning for the first time. Resonance strengths for resonances at 0.63, 0.721, 0.81 and 1.122 MeV Ecm have been extracted. The experimentally based reaction rate calculated represents a lower limit, but suggests that significant s-process nucleosynthesis occurs in low metallicity massive stars., 7 pages, 5 figures

Background: Nucleosynthesis of mid-mass elements is thought to occur under hot and explosive astrophysical conditions. Radiative α capture on S34 has been shown to impact nucleosynthesis in several such conditions, including core and shell oxygen burning, explosive oxygen burning, and type Ia supernovae. Purpose: Broad uncertainties exist in the literature for the strengths of three resonances within the astrophysically relevant energy range (ECM=1.94-3.42MeV at T=2.2GK). Further, there are several states in Ar38 within this energy range which have not been previously measured. This work aimed to remeasure the resonance strengths of states for which broad uncertainty existed as well as to measure the resonance strengths and energies of previously unmeasured states. Methods: Resonance strengths and energies of eight narrow resonances (five of which had not been previously studied) were measured in inverse kinematics with the DRAGON facility at TRIUMF by impinging an isotopically pure beam of S34 ions on a windowless He4 gas target. Prompt γ emissions of de-exciting Ar38 recoils were detected in an array of bismuth germanate scintillators in coincidence with recoil nuclei, which were separated from unreacted beam ions by an electromagnetic mass separator and detected by a time-of-flight system and a multianode ionization chamber. Results: The present measurements agree with previous results. Broad uncertainty in the resonance strength of the ECM=2709keV resonance persists. Resonance strengths and energies were determined for five low-energy resonances which had not been studied previously, and their strengths were determined to be significantly weaker than those of previously measured resonances. Conclusions: The five previously unmeasured resonances were found not to contribute significantly to the total thermonuclear reaction rate. A median total thermonuclear reaction rate calculated using data from the present work along with existing literature values using the STARLIB rate calculator agrees with the NON-SMOKER statistical model calculation as well as the REACLIB and STARLIB library rates at explosive and nonexplosive oxygen-burning temperatures (T=3-4GK and T=1.5-2.7GK, respectively).

How does nature hold together protons and neutrons to form the wide variety of complex nuclei in the Universe? Describing many-nucleon systems from the fundamental theory of quantum chromodynamics has been the greatest challenge in answering this question. The chiral effective field theory description of the nuclear force now makes this possible but requires certain parameters that are not uniquely determined. Defining the nuclear force needs identification of observables sensitive to the different parametrizations. From a measurement of proton elastic scattering on ^{10}C at TRIUMF and ab initio nuclear reaction calculations, we show that the shape and magnitude of the measured differential cross section is strongly sensitive to the nuclear force prescription.

Background: The rate of the F18(p,γ)Ne19 reaction affects the final abundance of the radioisotope F18 ejected from novae. This nucleus is important as its abundance is thought to significantly influence the first-stage 511-keV and continuum γ-ray emission in the aftermath of novae. No successful measurement of this reaction existed prior to this work, and the rate used in stellar models had been calculated based on incomplete information from contributing resonances. Purpose: Of the two resonances thought to provide a significant contribution to the astrophysical reaction rate, located at Ec.m.=330 and 665 keV, the former has a radiative width estimated from the assumed analog state in the mirror nucleus, F19, while the latter resonance does not have an analog state assignment, resulting in an arbitrary radiative width being assumed. As such, a direct measurement was needed to establish what role this resonance plays in the destruction of F18 at nova temperatures. This paper extends and takes the place of a previous Letter which reported the strength of the Ec.m.=665 keV resonance. Method: The DRAGON recoil separator was used to directly measure the strength of the important 665-keV resonance in this reaction, in inverse kinematics, by observing Ne19 reaction products. A radioactive F18 beam was provided by the ISAC facility at TRIUMF. R-matrix calculations were subsequently used to evaluate the significance of the results at astrophysical energies. Results: We report the direct measurement of the F18(p,γ)Ne19 reaction with the reevaluation of several detector efficiencies and the use of an updated Ne19 level scheme in the reaction rate analysis. The strength of the 665-keV resonance (Ex=7.076 MeV) is found to be an order of magnitude weaker than currently assumed in nova models. An improved analysis of the previously reported data is presented here, resulting in a slightly different value for the resonance strength. These small changes, however, do not alter the primary conclusions. Conclusions: Reaction rate calculations definitively show that the 665-keV resonance plays no significant role in the destruction of F18 at nova temperatures.

We have performed the first direct measurement of the 38Kðp; γÞ39Ca reaction using a beam of radioactive 38K. A proposed l ¼ 0 resonance in the 38K þ p system has been identified at 679(2) keV with an associated strength of 120 þ50 −30 meV. Upper limits of 1.16 (3.5) and 8.6 (26) meV at the 68% (95%) confidence level were also established for two further expected l ¼ 0 resonances at 386 and 515 keV, respectively. The present results have reduced uncertainties in the 38Kðp; γÞ39Ca reaction rate at temperatures of 0.4 GK by more than 2 orders of magnitude and indicate that Ar and Ca may be ejected in observable quantities by oxygen-neon novae. However, based on the newly evaluated rate, the 38Kðp; γÞ39Ca path is unlikely to be responsible for the production of Ar and Ca in significantly enhanced quantities relative to solar abundances.

The DRAGON facility for the study of radiative capture reactions has an extended gas target, surrounded by an array of BGO detectors. The distribution of detected gamma rays amongst the segmented array permits an estimate of the reaction position and consequently of the resonance energy. We report a study of the technique, using the 24 Mg(p, γ ) 25 Al reaction. Energy determination to better than 0.5% has been demonstrated.

Several lifetimes in $^{23}\text{Mg}$ have been determined for the first time using the Doppler-shift attenuation method. A Monte Carlo simulation code has been written to model the $\ensuremath{\gamma}$-ray line shape. An upper limit of $\ensuremath{\tau}l12$ fs at the 95% C.L. has been obtained for the astrophysically important 7787 keV state.

We report on the mass measurements of several neutron-rich $\mathrm{Rb}$ and $\mathrm{Sr}$ isotopes in the $A \approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}\mathrm{Rb}$ and $^{98-100}\mathrm{Sr}$ have been determined with a precision of $6 - 12\ \mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}\mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measurement and a deviation of $3\sigma$ when compared to the Atomic Mass Evaluation. We also confirm the mass of $^{100}\mathrm{Rb}$ from a previous measurement. Furthermore, our data indicates the existance of a low-lying isomer with $80\ \mathrm{keV}$ excitation energy in $^{98}\mathrm{Rb}$. We show that our updated mass values lead to minor changes in the r-process by calculating fractional abundances in the $A\approx 100$ region of the nuclear chart., Comment: 8 pages, 5 figures

The ${}^{33}$S($p,\ensuremath{\gamma}$)${}^{34}$Cl reaction is important for constraining predictions of certain isotopic abundances in oxygen-neon novae. Models currently predict as much as 150 times the solar abundance of ${}^{33}$S in oxygen-neon nova ejecta. This overproduction factor may vary by orders of magnitude due to uncertainties in the ${}^{33}$S($p,\ensuremath{\gamma}$)${}^{34}$Cl reaction rate at nova peak temperatures. Depending on this rate, ${}^{33}$S could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the ${}^{33}$S($p,\ensuremath{\gamma}$)${}^{34}$Cl rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the ${}^{33}$S($p,\ensuremath{\gamma}$)${}^{34}$Cl reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of $0.2--0.4$ GK there are seven known states in ${}^{34}$Cl both below the 432-keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON (Detector of Recoils And Gammas of Nuclear reactions) recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the ${}^{33}$S($p,\ensuremath{\gamma}$)${}^{34}$Cl rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of $\ensuremath{\approx}$20--150 for the expected ${}^{33}$S overproduction factor, and a range of $\ensuremath{\approx}$100--450 for the ${}^{32}$S/${}^{33}$S ratio expected in ONe novae.

The ${}^{20}$Ne${(p,\ensuremath{\gamma})}^{21}$Na reaction is the starting point of the NeNa cycle, which is an important process for the production of intermediate mass elements. The ${E}_{\text{c.m.}}=1113$ keV resonance plays an important role in the determination of stellar rates for this reaction since it is used to normalize experimental direct capture yields at lower energies. The commonly accepted strength of this resonance, $\ensuremath{\omega}\ensuremath{\gamma}=1.13\ifmmode\pm\else\textpm\fi{}0.07$ eV, has been misinterpreted as the strength in the center-of-mass frame when it is actually the strength in the laboratory frame. This has motivated a new measurement of the ${E}_{\text{c.m.}}=1113$ keV resonance strength in ${}^{20}$Ne${(p,\ensuremath{\gamma})}^{21}$Na using the DRAGON recoil mass spectrometer. The DRAGON result, $0.972\ifmmode\pm\else\textpm\fi{}0.11$ eV, is in good agreement with the accepted value when both are calculated in the same frame of reference.

Exploration of the physics involved in the production of cosmogenic radionuclides requires experiments using the same rare, radioactive nuclei in sufficient quantities. For this work, such exotic radionuclides have been extracted from previously proton-irradiated stainless steel samples using wet chemistry separation techniques. The irradiated construction material has arisen from an extended material research programme at the Paul Scherrer Institute, called STIP (SINQ Target Irradiation Program), where several thousand samples of different materials were irradiated with protons and neutrons of energies up to 570 MeV. In total, 8 × 1017 atoms of 44Ti, ∼1016 atoms of 26Al and ∼1019 atoms of 53Mn are available from selected samples. These materials may now be used to produce targets or radioactive beams for nuclear reaction studies with protons, neutrons and α-particles. The work is part of the ERAWAST initiative (Exotic Radionuclides from Accelerator Waste for Science and Technology), aimed at facilitating new collaborations between the isotope producers and users from different scientific fields including nuclear astrophysics.