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7 pags., 4 figs., Situated in the so-called "island of inversion," the nucleus $^{32}$Mg is considered as an archetypal example of the disappearance of magicity at $N=20$. We report on high statistics in-beam spectroscopy of $^{32}$Mg with a unique approach, in that two direct reaction probes with different sensitivities to the underlying nuclear structure are employed at the same time. More specifically, states in $^{32}$Mg were populated by knockout reactions starting from $^{33}$Mg and $^{34}$Si, lying inside and outside the island of inversion, respectively. The momentum distributions of the reaction residues and the cross sections leading to the individual final states were confronted with eikonal-based reaction calculations, yielding a significantly updated level scheme for $^{32}$Mg and spin-parity assignments. By fully exploiting observables obtained in this measurement, a variety of structures coexisting in 32Mg was unraveled. Comparisons with theoretical predictions based on shell-model overlaps allowed for clear discrimination between different structural models, revealing that the complete theoretical description of this key nucleus is yet to be achieved., N.K. acknowledges support of the Grant-in-Aid for JSPS Fellows (18J12542) from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT), Japan. K.W. acknowledges support from the Ministerio de Ciencia e Innovación (Spain) through the Ramón y Cajal program RYC-2017-22007. A.P. is supported in part by the Ministerio de Ciencia, Innovación y Universidades (Spain), Severo Ochoa program SEV-2016-0597 and grant PGC-2018-94583. The SDPF-M calculations were enabled by the CNS-RIKEN joint project for large-scale nuclear structure calculations and were performed mainly on the Oakforest-PACS supercomputer. N.S. acknowledges support from “Priority Issue on post-K computer” (hp190160) and “Program for Promoting Researches on the Supercomputer Fugaku” (hp200130) by JICFuS and MEXT, Japan. J.A.T. acknowledges support from the U.K. Science and Technology Facilities Council Grant No. ST/L005743/1. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Nuclear Physics, under Grant No. DE-SC0020451 and by the U.S. National Science Foundation (NSF) under Grant No. PHY-1306297. GRETINA was funded by the U.S. DOE, Office of Science. Operation of the array at NSCL was supported by the U.S. NSF under Cooperative Agreement No. PHY-1102511 (NSCL) and DOE under Grant No. DE-AC02-05CH11231 (LBNL).

Background: In the "island of inversion", ground states of neutron-rich $sd$-shell nuclei exhibit strong admixtures of intruder configurations from the $fp$ shell. The nucleus $^{30}$Mg, located at the boundary of the island of inversion, serves as a cornerstone to track the structural evolution as one approaches this region. Purpose: Spin-parity assignments for excited states in $^{30}$Mg, especially negative-parity levels, have yet to be established. In the present work, the nuclear structure of $^{30}$Mg was investigated by in-beam $\gamma$-ray spectroscopy mainly focusing on firm spin-parity determinations. Method: High-intensity rare-isotope beams of $^{31}$Mg, $^{32}$Mg, $^{34}$Si, and $^{35}$P bombarded a Be target to induce nucleon removal reactions populating states in $^{30}$Mg. $\gamma$ rays were detected by the state-of-the-art $\gamma$-ray tracking array GRETINA. For the direct one-neutron removal reaction, final-state exclusive cross sections and parallel momentum distributions were deduced. Multi-nucleon removal reactions from different projectiles were exploited to gain complementary information. Results: With the aid of the parallel momentum distributions, an updated level scheme with revised spin-parity assignments was constructed. Spectroscopic factors associated with each state were also deduced. Conclusions: Results were confronted with large-scale shell-model calculations using two different effective interactions, showing excellent agreement with the present level scheme. However, a marked difference in the spectroscopic factors indicates that the full delineation of the transition into the island of inversion remains a challenge for theoretical models.

Self-conjugate nuclei in the A ≈ 70 – 80 region have attracted a great deal of attention due to phenomena such as shape coexistence and increasing collectivity along the N = Z line. We investigate the structure of nuclei in this region through lifetime measurements using the GRETINA array. The first implementation of the Differential Recoil Distance Doppler Shift technique with fast radioactive beams is demonstrated and verified through a measurement of the well-known B ( E 2 ; 2 1 + → 0 1 + ) transition strength in 74Kr. The method is then applied to determine the B ( E 2 ; 2 1 + → 0 1 + ) transition strength in 74Rb, the heaviest odd–odd N = Z nucleus for which this quantity has been determined. This result and extended systematics along N = Z suggest the dominance of the isoscalar part of the quadrupole transition strengths in self-conjugate nuclei, as well as the possible presence of shape coexistence in 74Rb.

International audience; Neutron-rich isotopes are an important source of new information on nuclear physics. Specifically, the spin-isospin components in the nucleon-nucleon (NN) interaction, e.g., the proton-neutron tensor force, are expected to modify shell structure in exotic nuclei. These potential changes in the intrinsic shell structure are of fundamental interest. The study of the excitation energy of states corresponding to specific configurations in even-even isotopes, together with the single-particle character of the first excited states of odd-A, neutron-rich Ni isotopes, probes the evolution of the neutron orbitals around the Fermi surface as a function of the neutron number a step forward in the understanding of the region and the nature of the NN interaction at large N/Z ratios. In an experiment carried out at the National Superconducting Cyclotron Laboratory [1], new spectroscopic information was obtained for 68Ni and the distribution of single-particle strengths in 67,69Ni was characterized by means of single-neutron knockout from 68,70Ni secondary beams. The spectroscopic strengths, deduced from the measured partial cross sections to the individual states tagged by their de-exciting gamma rays, is used to identify and quantify configurations that involve neutron excitations across the N = 40 harmonic oscillator shell closure. The de-excitation γ rays were measured with the GRETINA tracking array [2]. The results challenge the validity of the most current shell-model Hamiltonians and effective interactions, highlighting shortcomings that cannot yet be explained. These results suggest that our understanding of the low-energy states in such nuclei is not complete and requires further investigation.

The low-energy excitation level schemes of the neutron-rich $^{38--42}\mathrm{S}$ isotopes are investigated via in-beam $\ensuremath{\gamma}$-ray spectroscopy following the fragmentation of $^{48}\mathrm{Ca}$ and $^{46}\mathrm{Ar}$ projectiles on a $^{12}\mathrm{C}$ target at intermediate beam energies. Information on $\ensuremath{\gamma}\ensuremath{\gamma}$ coincidences complemented by comparisons to shell-model calculations were used to construct level schemes for these neutron-rich nuclei. The experimental data are discussed in the context of large-scale shell-model calculations with the SDPF-MU effective interaction in the $sd\text{\ensuremath{-}}pf$ shell. For the even-mass S isotopes, the evolution of the yrast sequence is explored as well as a peculiar change in decay pattern of the second ${2}^{+}$ states at $N=26$. For the odd-mass $^{41}\mathrm{S}$, a level scheme is presented that seems complete below 2.2 MeV and consistent with the predictions by the SDPF-MU shell-model Hamiltonian; this is a remarkable benchmark given the rapid shell and shape evolution at play in the S isotopes as the broken-down $N=28$ magic number is approached. Furthermore, the population of excited final states in projectile fragmentation is discussed.

The distribution of single-particle strength in 67,69Ni was characterized with one-neutron knockout reactions from intermediate-energy 68,70Ni secondary beams, selectively populating neutron-hole configurations at N = 39 and 41, respectively. The spectroscopic strengths deduced from the measured partial cross sections to the individual final states, as tagged by their γ-ray decays, are used to identify and quantify neutron configurations in the wave functions. While 69Ni compares well to shell-model predictions, the results for 67Ni challenge the validity of current effective shell-model Hamiltonians by revealing discrepancies that cannot be explained so far. These results suggest that our understanding of the low-lying states in the neutron-rich, semi-magic Ni isotopes may be incomplete and requires further investigation on both the experimental and theoretical sides.

The quadrupole transition rate for the 41+→21+ transition of Ni58 was determined from an application of the recoil distance method with the Gamma-Ray Energy Tracking In-beam Nuclear Array (GRETINA). The present result of the B(E2;41+→21+) was found to be 50-6+11e2fm4, which is about three times smaller than the literature value, indicating substantially less collectivity than previously believed. Shell model calculations performed with the GXPF1A effective interaction agree with the present data and the validity of the standard effective charges in understanding collectivity in the nickel isotopes is discussed.

International audience; One-neutron knockout reactions have been performed on a beam of radioactive 53Co in a high-spinisomeric state. The analysis is shown to yield a highly selective population of high-spin states in an exoticnucleus with a significant cross section, and hence represents a technique that is applicable to the plannednew generation of fragmentation-based radioactive beam facilities. Additionally, the relative cross sectionsamong the excited states can be predicted to a high level of accuracy when reliable shell-model input isavailable. The work has resulted in a new level scheme, up to the 11þ band-termination state, of the protonrichnucleus 52Co (Z ¼ 27, N ¼ 25). This has in turn enabled a study of mirror energy differences inthe A ¼ 52 odd-odd mirror nuclei, interpreted in terms of isospin-nonconserving (INC) forces in nuclei.The analysis demonstrates the importance of using a full set of J-dependent INC terms to explain theexperimental observations.

Comprehensive spectroscopy of the N = 29 nucleus 47Ar is presented, based on two complemen-tary direct reaction mechanisms: one-neutron pickup onto 46Ar projectiles and one-proton removal from the 1− ground state of 48K. The results are compared to shell-model calculations that use the state-of-the-art SDPF-U and SDPF-MU effective interactions. Also, from the 9Be(46Cl,45S+γ)X one-proton removal reaction, we report the first γ-ray transitions observed from 45S. Using compar-isons with shell-model calculations, and from the observed intensities and energy sums, we propose a first tentative level scheme for 45S.

The highly selective, intermediate-energy heavy-ion-induced neutron-pickup reaction, in combination with γ-ray spectroscopy using the γ-ray energy-tracking in-beam nuclear array (GRETINA), is shown to provide reliable relative spectroscopic strengths for high-l orbitals in nuclei more neutron rich than the projectile. The reaction mechanism gives a significant final-state-spin alignment that is validated through γ-ray angular-distribution measurements enabled by the position sensitivity of GRETINA. This is the first time that γ-ray angular distributions could be extracted from a high-luminosity, fast-beam reaction other than inelastic scattering. This holds great promise for the restriction and assignment of Jπ quantum numbers in exotic nuclei. We advance this approach to study the crucial N=28 shell closure and extract the ratio g9/2:f5/2 of bound neutron single-particle strengths in Ca49, a benchmark for emerging multi-shell ab initio and configuration-interaction theories that are applicable along the Ca isotopic chain.

Background: The study of excited states in mirror nuclei allows us to extract information on charge-dependent (i.e., isospin-nonconserving) interactions in nuclei. Purpose: To extend previous studies of mirror nuclei in the f7/2 region, investigating charge symmetry breaking of the strong nuclear force. Methods: γ-ray spectroscopy has been performed for the mirror (Tz= ±3/2) pair 53Ni and 53Mn, produced via mirrored one-nucleon knockout reactions. Results: Several new transitions have been identified in 53Ni from which a new level scheme has been constructed. Cross sections for knockout have been analyzed and compared with reaction model calculations where evidence is found for knockout from high-spin isomeric states. Mirror energy differences between isobaric analog states have been computed, compared to large scale shell-model calculations, and interpreted in terms of isospin-nonconserving effects. In addition, lifetimes for the long-lived J π = 5 /2 − 1 analog states in both 53Mn and 53Ni have been extracted through lineshape analysis, giving half-lives of t1/2 = 120 (14) ps and t1/2 = 198 (12) ps,respectively. Conclusions: The inclusion of a set of isovector isospin-nonconserving matrix elements to the shell-model calculations gave the best agreement with the experimental data.

The neutron-deficient nucleus Sn 107 has been studied by using the one-neutron knockout reaction. By measuring the decay γ rays and momentum distributions of reaction residues, the spins of the ground, 5/2 + , and first-excited, 7/2 + , states of Sn 107 have been assigned by comparisons to eikonal-model reaction calculations. Limits on the inclusive and exclusive cross sections have been measured and transitions due to neutron removals from below the N=50 closed shell have been observed. New excited states up to 5.5 MeV in Sn 107 have been identified.

Author(s): Henry, TW; Bentley, MA; Clark, RM; Davies, PJ; Bader, VM; Baugher, T; Bazin, D; Beausang, CW; Berryman, JS; Bruce, AM; Campbell, CM; Crawford, HL; Cromaz, M; Fallon, P; Gade, A; Henderson, J; Iwasaki, H; Jenkins, DG; Lee, IY; Lemasson, A; Lenzi, SM; Macchiavelli, AO; Napoli, DR; Nichols, AJ; Paschalis, S; Petri, M; Recchia, F; Rissanen, J; Simpson, EC; Stroberg, SR; Wadsworth, R; Weisshaar, D; Wiens, A; Walz, C | Abstract: Background: Triplet energy differences (TED) can be studied to yield information on isospin-non-conserving interactions in nuclei. Purpose: The systematic behavior of triplet energy differences (TED) of T=1, Jπ=2+ states is examined. The A=62 isobar is identified as having a TED value that deviates significantly from an otherwise very consistent trend. This deviation can be attributed to the tentative assignments of the pertinent states in Ga62 and Ge62. Methods: An in-beam γ-ray spectroscopy experiment was performed to identify excited states in Ga62 using Gamma-Ray Energy Tracking In-Beam Nuclear Array with the S800 spectrometer at NSCL using a two-nucleon knockout approach. Cross-section calculations for the knockout process and shell-model calculations have been performed to interpret the population and decay properties observed. Results: Using the systematics as a guide, a candidate for the transition from the T=1, 2+ state is identified. However, previous work has identified similar states with different Jπ assignments. Cross-section calculations indicate that the relevant T=1, 2+ state should be one of the states directly populated in this reaction. Conclusions: As spins and parities were not measurable, it is concluded that an unambiguous identification of the first T=1, 2+ state is required to reconcile our understanding of TED systematics.

International audience; Analyses of data from both deep inelastic reactions at Argonne National Laboratory and single-and multiple-particle knockout reactions at Michigan State University revealed new gamma-ray transitions in even-even Ni-66,68,70,72(38,40,42,44) and in Co-67(40) that provide strong evidence for multiple shape coexistence at N = 38 and 40 and deep prolate minima in Ni-70(42) and isotonic Cu-71(42). A new transition at 642 keV is proposed for Ni-66 as the prolate 2(+) to 0(+) transition. Two new transitions in Ni-72 at 915 and 1225 keV were identified in the knock-out reaction study and could represent de-population of prolate states. Taken together with recent theoretical work using the Monte Carlo shell model, a well defined region of shape coexistence can be seen existing precisely between 38

Transition strengths for decays from low-lying states in A ∼ 70 nuclei have been deduced from lifetime measurements using the recoil distance Doppler shift technique. The results confirm the collectivity previously reported for the 21+→0gs+ decay in 68 Se and reveal a relative decrease in collectivity in 70 Br. This trend is reproduced by shell model calculations using the GXPF1A interaction in an fp model space including the Coulomb, spin-orbit and isospin non-conserving interactions. The 31+→21+ decay in 70 Br is found to have a very small B(M1) value, which is consistent with the configuration of the state being dominated by the coupling of f52 protons and neutrons. The results suggest that the g92 orbit does not play an important role at low spin in these nuclei. The B(E2) values for the decays of the (T = 1) 21+ states in 70 Br and 70 Se are almost identical, suggesting there is no major shape change between the two nuclei at low spin.

We report on the experimental study of quadrupole collectivity in the neutron-deficient nucleus \nuc{104}{Sn} using intermediate-energy Coulomb excitation. The $B(E2; 0^+_1 \rightarrow 2^+_1)$ value for the excitation of the first $2^+$ state in \nuc{104}{Sn} has been measured to be $0.180(37)~e^2$b$^2$ relative to the well-known $B(E2)$ value of \nuc{102}{Cd}. This result disagrees by more than one sigma with a recently published measurement \cite{Gua13}. Our result indicates that the most modern many-body calculations remain unable to describe the enhanced collectivity below mid-shell in Sn approaching $N=Z=50$. We attribute the enhanced collectivity to proton particle-hole configurations beyond the necessarily limited shell-model spaces and suggest the asymmetry of the $B(E2)$-value trend around mid-shell to originate from enhanced proton excitations across $Z=50$ as $N=Z$ is approached., Accepted for publication as rapid communication in Physical Review C

Production cross sections for neutron-rich nuclei from the fragmentation of a ${}^{82}$Se beam at 139 MeV/u were measured. The longitudinal momentum distributions of 126 neutron-rich isotopes of elements $11\ensuremath{\le}Z\ensuremath{\le}32$ were scanned using an experimental approach of varying the target thickness. Production cross sections with beryllium and tungsten targets were determined for a large number of nuclei including several isotopes first observed in this work. These are the most neutron-rich nuclides of the elements $22\ensuremath{\le}Z\ensuremath{\le}25$ (${}^{64}$Ti, ${}^{67}$V, ${}^{69}$Cr, and ${}^{72}$Mn). One event was registered consistent with ${}^{70}$Cr and another one with ${}^{75}$Fe. The production cross sections are correlated with ${Q}_{g}$ systematics to reveal trends in the data. The results presented here confirm our previous results from a similar measurement using a ${}^{76}$Ge beam and can be explained with a shell model that predicts a subshell closure at $N=34$ around $Z=20$. This is demonstrated by systematic trends and calculations with the abrasion-ablation model that are sensitive to separation energies.

The low-spin level scheme of ${}^{68}$Ni was investigated following two-neutron-knockout and multinucleon-transfer reactions. The energy of the first excited state was determined to be ${E}_{x}({0}_{2}^{+})=1603.5(3)$ keV. Relative $B(E2)$ transition probabilities were deduced and compared with shell-model calculations using several modern effective interactions. Theory reproduces the data well, but indicates substantial mixing of multi-particle, multi-hole configurations for the lowest observed ${0}^{+}$ and ${2}^{+}$ states.

Beta-delayed proton emission from nuclides in the neighborhood of 100Sn was studied at the National Superconducting Cyclotron Laboratory. The nuclei were produced by fragmentation of a 120 MeV/nucleon 112Sn primary beam on a Be target. Beam purification was provided by the A1900 Fragment Separator and the Radio Frequency Fragment Separator. The fragments of interest were identified and their decay was studied with the NSCL Beta Counting System (BCS) in conjunction with the Segmented Germanium Array (SeGA). The nuclei 96Cd, 98Ing, 98Inm and 99In were identified as beta-delayed proton emitters, with branching ratios bp = 5.5(40)%, 5.5+3 -2%, 19(2)% and 0.9(4)%, respectively. The bp for 89Ru, 91,92Rh, 93Pd and 95Ag were deduced for the first time with bp = 3+1.9 -1.7%, 1.3(5)%, 1.9(1)%, 7.5(5)% and 2.5(3)%, respectively. The bp = 22(1)% for 101Sn was deduced with higher precision than previously reported. The impact of the newly measured bp values on the composition of the type-I X-ray burst ashes was studied.

The lifetimes of the first 2${}^{+}$ states in the neutron-deficient ${}^{76,78}$Sr isotopes were measured using a unique combination of the $\ensuremath{\gamma}$-ray line-shape method and two-step nucleon exchange reactions at intermediate energies. The transition rates for the 2${}^{+}$ states were determined to be $B(\mathrm{E}2;{2}^{+}\ensuremath{\rightarrow}{0}^{+})=2220(270)$ ${e}^{2}$fm${}^{4}$ for ${}^{76}$Sr and 1800(250) ${e}^{2}$fm${}^{4}$ for ${}^{78}$Sr, corresponding to large deformation of ${\ensuremath{\beta}}_{2}$ $=$ 0.45(3) for ${}^{76}$Sr and 0.40(3) for ${}^{78}$Sr. The present data provide experimental evidence for mutually enhanced collectivity that occurs at $N$ $=$ $Z$ $=$ 38. The systematic behavior of the excitation energies and $B(\mathrm{E}2)$ values indicates a signature of shape coexistence in ${}^{76}$Sr, characterizing ${}^{76}$Sr as one of most deformed nuclei with an unusually reduced $E$(4${}^{+}$)$/E$(2${}^{+}$) ratio.

The isomeric and $\ensuremath{\beta}$ decays of the $N=Z+2$ nucleus ${}^{96}\phantom{\rule{-0.16em}{0ex}}$Ag were investigated at the National Superconducting Cyclotron Laboratory. A cascade of $\ensuremath{\gamma}$-ray transitions originating from the deexcitation of a microsecond isomer was observed for the first time and was found in coincidence with two previously known transitions with energies of 470 and 667 keV. The isomeric half-life was determined as 1.45(7) $\ensuremath{\mu}$s, more precise than previously reported. The existence of a second, longer-lived microsecond isomer, associated with a 743-keV $\ensuremath{\gamma}$ transition, is also proposed here. Shell model results within the $({p}_{3/2}{p}_{1/2}{f}_{5/2}{g}_{9/2})$ model space, using the jj44b interaction, reproduced level energies and isomeric decay half-lives reasonably well.

The isomeric and $\beta$-decay properties of neutron-rich $^{53-57}$Sc and $^{53,54}$Ca nuclei near neutron number $N$=32 are reported, and the low-energy level schemes of $^{53,54,56}$Sc and $^{53-57}$Ti are presented. The low-energy level structures of the $_{21}$Sc isotopes are discussed in terms of the coupling of the valence $1f_{7/2}$ proton to states in the corresponding $_{20}$Ca cores. Implications with respect to the robustness of the $N$=32 subshell closure are discussed, as well as the repercussions for a possible $N$=34 subshell closure., Comment: 17 pages, 17 figures, accepted to Phys. Rev. C

Direct reaction techniques are powerful tools to study the single-particle nature of nuclei. Performing direct reactions on short-lived nuclei requires radioactive ion beams produced either via fragmentation or the Isotope Separation OnLine (ISOL) method. Some of the most interesting regions to study with direct reactions are close to the magic numbers where changes in shell structure can be tracked. These changes can impact the final abundances of explosive nucleosynthesis. The structure of the chain of tin isotopes is strongly influenced by the Z=50 proton shell closure, as well as the neutron shell closures lying in the neutron-rich, N=82, and neutron-deficient, N=50, regions. Here we present two examples of direct reactions on exotic tin isotopes. The first uses a one-neutron transfer reaction and a low-energy reaccelerated ISOL beam to study states in 131Sn from across the N=82 shell closure. The second example utilizes a one-neutron knockout reaction on fragmentation beams of neutron-deficient 106,108Sn. In both cases, measurements of gamma rays in coincidence with charged particles proved to be invaluable., 11 pages, 5 figures, Zakopane Conference on Nuclear Physics "Extremes of the Nuclear Landscape", Zakopane, Poland, August 31 - September 7, 2014

First experimental evidence for a high-spin isomer ( 25 / 2 + ) in 97Cd, a waiting point in the astrophysical rapid proton capture process, is presented. The data were obtained in β-decay studies at NSCL using the new RF Fragment Separator system and detecting β-delayed protons and β-delayed γ rays. Decays from ground and isomeric states were disentangled, and proton emission branches were determined for the first time. We find half-lives of 1.10(8) s and 3.8(2) s, and β-delayed proton emission branches of 12(2)% and 25(4)% were deduced for the ground and isomeric states, respectively. With these results, the nuclear data needed to determine an rp-process contribution to the unknown origin of solar 96Ru are in place. When the new data are included in astrophysical rp-process calculations, one finds that an rp-process origin of 96Ru is unlikely.

The first spectroscopy of excited states in 52Ni (Tz=2) and 51Co (Tz=-3/2) has been obtained using the highly selective two-neutron knockout reaction. Mirror energy differences between isobaric analogue states in these nuclei and their mirror partners are interpreted in terms of isospin nonconserving effects. A comparison between large scale shell-model calculations and data provides the most compelling evidence to date that both electromagnetic and an additional isospin nonconserving interactions for J=2 couplings, of unknown origin, are required to obtain good agreement., Comment: Accepted for publication in Physical Review Letters