1. Magnetic anisotropy of the alkali iridate Na2IrO3 at high magnetic fields: Evidence for strong ferromagnetic Kitaev correlations
- Author
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Das, Sitikantha. D, Kundu, Sarbajaya, Zhu, Zengwei, Mun, Eundeok, McDonald, Ross D., Li, Gang, Balicas, Luis, McCollam, Alix, Cao, Gang, Rau, Jeffrey. G., Kee, Hae-Young, Tripathi, Vikram, Sebastian, Suchitra E., Sebastian, Suchitra [0000-0002-1386-8138], and Apollo - University of Cambridge Repository
- Subjects
Condensed Matter - Strongly Correlated Electrons ,Strongly Correlated Electrons (cond-mat.str-el) ,FOS: Physical sciences ,Condensed Matter::Strongly Correlated Electrons ,51 Physical Sciences ,5108 Quantum Physics ,Strongly correlated electrons - Abstract
The magnetic field response of the Mott-insulating honeycomb iridate Na$_{2}$IrO$_{3}$ is investigated using torque magnetometry measurements in magnetic fields up to 60 tesla. A peak-dip structure is observed in the torque response at magnetic fields corresponding to an energy scale close to the zigzag ordering ($\approx 15~K$) temperature. Using exact diagonalization calculations, we show that such a distinctive signature in the torque response constrains the effective spin models for these classes of Kitaev materials to ones with dominant ferromagnetic Kitaev interactions, while alternative models with dominant antiferromagnetic Kitaev interactions are excluded. We further show that at high magnetic fields, long range spin correlation functions decay rapidly, signaling a transition to a long-sought-after field-induced quantum spin liquid beyond the peak-dip structure. Kitaev systems are thus revealed to be excellent candidates for field-induced quantum spin liquids, similar physics having been suggested in another Kitaev material $\alpha-$RuCl$_{3}$., Comment: 12 pages, 20 figures; text modified, one figure shifted to main text, table added to main text
- Published
- 2019