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Several studies have reported the transport of short-lived climate forcers/pollutants (SLCF/P) from the highly polluted areas in southern Asia (e.g., the Indo-Gangetic Plain and the Himalayan foothills) to the Himalayas, with significant implications for the global and regional climate, crop yields, and human health. In this work, we perform a comparison of nearly three years (February 2013–October 2015) of simultaneous black carbon (BC) and surface ozone (O3) measurements at two sites in Nepal, viz., Paknajol (1380 m a.s.l.), in the Kathmandu Valley, and the WMO/GAW global station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.), near the base camp of Mt. Everest. The two sites are only 150 km apart and are characterized by different situations: While the Kathmandu Valley is one of the regional urban “hot spots” for concerns related to air pollution, NCO-P is representative of the background conditions of the high Himalayas and the free troposphere. Therefore, the possible role played by emissions occurring in the planetary boundary layer (PBL) of the Kathmandu Valley in influencing the variability in SLCF/P at NCO-P was investigated. BC and O3 concentrations at NCO-P showed a linear correlation with the modeled PBL height over the Kathmandu urban area, providing evidence that the anthropogenic emissions occurring within the Kathmandu PBL could affect the variability in BC and O3 at NCO-P. Furthermore, when introducing an additional constraint into the analysis (viz., back-trajectories), we show that on days when air mass transport between the two measurement sites was observed (10% of the period), at least 22% and 16% of BC and O3 variability at NCO-P can be explained by concurrent variability in SLCF/P over the Kathmandu Valley.

We analysed the variability of equivalent black carbon (BC) and ozone (O3) at the global WMO/GAW station Nepal Climate Observatory-Pyramid (NCO-P, 5079 m a.s.l.) in the southern Himalayas, for evaluating the possible contribution of open vegetation fires to the variability of these short-lived climate forcers/pollutants (SLCF/SLCP) in the Himalayan region. We found that 162 days (9% of the data-set) were characterised by acute pollution events with enhanced BC and O3 in respect to the climatological values. By using satellite observations (MODIS fire products and the USGS Land Use Cover Characterization) and air mass back-trajectories, we deduced that 56% of these events were likely to be affected by emissions from open fires along the Himalayas foothills, the Indian Subcontinent and the Northern Indo-Gangetic Plain. These results suggest that open fire emissions are likely to play an important role in modulating seasonal and inter-annual BC and O3 variability over south Himalayas.© 2013 Elsevier Ltd. All rights reserved.

The Kathmandu Valley in South Asia is considered as one of the global "hot spots" in terms of urban air pollution. It is facing severe air quality problems as a result of rapid urbanization and land use change, socioeconomic transformation and high population growth. In this paper, we present the first full year (February 2013–January 2014) analysis of simultaneous measurements of two short-lived climate forcers/pollutants (SLCF/P), i.e. ozone (O3) and equivalent black carbon (hereinafter noted as BC) and aerosol number concentration at Paknajol, in the center of the Kathmandu metropolitan city. The diurnal behavior of equivalent black carbon (BC) and aerosol number concentration indicated that local pollution sources represent the major contributions to air pollution in this city. In addition to photochemistry, the planetary boundary layer (PBL) and wind play important roles in determining O3 variability, as suggested by the analysis of seasonal diurnal cycle and correlation with meteorological parameters and aerosol properties. Especially during pre-monsoon, high values of O3 were found during the afternoon/evening; this could be related to mixing and entrainment processes between upper residual layers and the PBL. The high O3 concentrations, in particular during pre-monsoon, appeared well related to the impact of major open vegetation fires occurring at regional scale. On a synoptic-scale perspective, westerly and regional atmospheric circulations appeared to be especially conducive for the occurrence of the high BC and O3 values. The very high values of SLCF/P, detected during the whole measurement period, indicated persisting adverse air quality conditions, dangerous for the health of over 3 million residents of the Kathmandu Valley, and the environment. Consequently, all of this information may be useful for implementing control measures to mitigate the occurrence of acute pollution levels in the Kathmandu Valley and surrounding area.