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Abstract: Accurate regional air pollution simulation relies strongly on the accuracy of the mesoscale meteorological simulation used to drive the air quality model. The framework of the Air Quality Model Evaluation International Initiative (AQMEII), which involved a large international community of modeling groups in Europe and North America, offered a unique opportunity to evaluate the skill of mesoscale meteorological models for two continents for the same period. More than 20 groups worldwide participated in AQMEII, using several meteorological and chemical transport models with different configurations. The evaluation has been performed over a full year (2006) for both continents. The focus for this particular evaluation was meteorological parameters relevant to air quality processes such as transport and mixing, chemistry, and surface fluxes. The unprecedented scale of the exercise (one year, two continents) allowed us to examine the general characteristics of meteorological models’ skill and uncertainty. In particular, we found that there was a large variability between models or even model versions in predicting key parameters such as surface shortwave radiation. We also found several systematic model biases such as wind speed overestimations, particularly during stable conditions. We conclude that major challenges still remain in the simulation of meteorology, such as nighttime meteorology and cloud/radiation processes, for air quality simulation. [Copyright &y& Elsevier]

Abstract: The extremely warm summer of 2003, with its August heat wave, is taken as a prototype of future summer weather in Europe. The stagnant circulation led to accumulation of heat and pollutants, increased forest fires, and induced high ozone and particulate matter levels. After a description of the meteorological conditions encountered, we review here the effects of the heat-wave meteorology on photochemistry, wild fires, and particulate matter, at the continental and urban scales. We discuss the extent to which this special summer can be taken for projecting air quality in a future warmer climate, especially in the perspective of changes in regional and global emissions. For ozone, the effect of regional reduction of emissions will dominate over summer climate change, but the increase in baseline ozone should significantly raise the mean ozone levels. [Copyright &y& Elsevier]

Abstract: Despite the major international efforts devoted to the understanding and to the future estimate of global climate change and its impact on regional scale processes, the evolution of the atmospheric composition in a changing climate is far to be understood. In particular, the future evolution of the concentration of near-surface pollutants determining air quality at a scale affecting human health and ecosystems is a subject of intense scientific research. This thematic issue reviews the current scientific knowledge of the consequences of global climate change on regional air quality and its related impact on the biosphere and on human mortality. This article provides a presentation of the key issues, summarizes the current knowledge, and introduces the thematic issue. [Copyright &y& Elsevier]

Abstract: Over twenty modeling groups are participating in the Air Quality Model Evaluation International Initiative (AQMEII) in which a variety of mesoscale photochemical and aerosol air quality modeling systems are being applied to continental-scale domains in North America and Europe for 2006 full-year simulations for model inter-comparisons and evaluations. To better understand the reasons for differences in model results among these participating groups, each group was asked to use the same source of emissions and boundary concentration data for their simulations. This paper describes the development and application of the boundary concentration data for this AQMEII modeling exercise. The European project known as GEMS (Global and regional Earth-system Monitoring using Satellite and in-situ data) has produced global-scale re-analyses of air quality for several years, including 2006 (http://gems.ecmwf.int). The GEMS trace gas and aerosol data were made available at 3-hourly intervals on a regular latitude/longitude grid of approximately 1.9° resolution within 2 “cut-outs” from the global model domain. One cut-out was centered over North America and the other over Europe, covering sufficient spatial domain for each modeling group to extract the necessary time- and space-varying (horizontal and vertical) concentrations for their mesoscale model boundaries. Examples of the impact of these boundary concentrations on the AQMEII continental simulations are presented to quantify the sensitivity of the simulations to boundary concentrations. In addition, some participating groups were not able to use the GEMS data and instead relied upon other sources for their boundary concentration specifications. These are noted, and the contrasting impacts of other data sources for boundary data are presented. How one specifies four-dimensional boundary concentrations for mesoscale air quality simulations can have a profound impact on the model results, and hence, this aspect of data preparation must be performed with considerable care. [Copyright &y& Elsevier]

The current state of the art in three-dimensional chemistry-transport models allows them to be considered as mature and reliable enough to be combined with observations networks for implementing integrated air quality monitoring systems over large territories. A cooperative initiative of tour research and operational organizations in France has led to the creation of an integrated air quality platform providing near-real-time and forecasted information using last model developments. Since summer 2003, this system, Prévisions et Observations de la Qualité de l'Air en France et en Europe (PRBV AIR; available online at www.prevair. org), has been delivering daily air quality observations short-term (0-3 days) forecasts, and real-time analyses of ozone, nitrogen dioxide, and particulate matter (PM) at the global and European scales, with a focus over France. It has become a powerful scientific and communication tool to inform the public, sensitive population about the potential occurrence of air pollutant concentrations exceeding regulatory thresholds. The architecture of the operational system is described in this paper. Its setup allows the partners to cope with stringent operational constraints regarding the timely availability of the forecasts and the reliability and the quality of the products delivered. The system relies on a chain of numerical models and methods, and on real-time air quality observations, it uses National Centers for Environmental Predictions (NCEP) and Météo-France weather forecasts. Methods used for producing air pollutant concentration forecasts and analyses are described, as well as the final products, with case examples. A synthesis of the operational system skill results obtained over three consecutive years of operation (2003-06) is given. Lessons learned are presented and issues related to the use of the PREV'AIR system as a complementary tool for air quality management are discussed. [ABSTRACT FROM AUTHOR]

Abstract: Ground-level ozone concentrations in the atmospheric boundary layer over Spain are still exceeding thresholds established in EU legislation to protect human health and prevent damage to ecosystems. The increasing role that air quality models play in air quality management requires comparison between model results and previous observations in order to determine the capacity of the model to reproduce past events. The CHIMERE chemistry-transport model has been used by several research groups to estimate air pollutant concentrations in different European countries. An evaluation of the model performance of the CHIMERE air quality model was carried out for the spring and summer periods of 2003–2005 in Spain, using EMEP emissions. This evaluation has demonstrated a fair agreement between observed and modelled ozone values for background stations, with a mean normalized absolute error below 15% for rural background air quality sites. This value lays inside the range proposed in EPA''s guideline for an acceptable level of model performance. In spite of this acceptable model performance, further studies need to be carried out to explain some underestimation found over Madrid surroundings. [Copyright &y& Elsevier]

In the framework of the IMPACT2C project, we have evaluated the future European particulate matter concentrations under the influence of climate change and anthropogenic emission reductions. To do so, 30-year simulations for present and future scenarios were performed with an ensemble of four regional Chemical Transport Models. +2 °C scenarios were issued from different regional climate simulations belonging to the CORDEX experiment (RCP4.5 scenario). Comparing present day simulations to observations shows that these simulations meet the requested quality criteria even if some biases do exist. Also, we showed that using regional climate models instead of meteorological reanalysis was not critical for the quality of our simulations. Present day as well as future scenarios show the large variability between models associated with different meteorology and process parameterizations. Future projections of PM concentrations show a large reduction of PM10 and PM2.5 concentrations in a +2 °C climate over the European continent (especially over Benelux), which can be mostly attributed to emission reduction policies. Under a current legislation scenario, annual PM10 could be reduced by between 1.8 and 2.9 μg m −3 (14.1–20.4%). If maximum technologically feasible emission reductions were implemented, further reductions of 1.4–1.9 μg m −3 (18.6–20.9%) are highlighted. Changes due to a +2 °C warming, in isolation from emission changes, are in general much weaker (−1.1 to +0.4 μg m −3 ,-0.3 to +5.1% for annual PM10 averaged over the European domain). Even if large differences exist between models, we have determined that the decrease of PM over Europe associated with emission reduction is a robust result. The patterns of PM changes resulting from climate change (for example the increase of PM over Spain and southern France and the decrease of PM10 over eastern Europe) are also robustly predicted even if its amplitude remains weak compared to changes associated with emission reductions. [ABSTRACT FROM AUTHOR]

The evolution of ozone and nitrogen dioxide over Europe between the present day and a future period with a +2 °C global warming relative to the pre-industrial climate was studied using four offline chemistry transport models, each driven by a different climate model. Given the recent outcome of the COP21 negotiations, understanding the implications of climate change around the +2 °C threshold has never been more pressing or relevant. One of the objectives of this study was to show how changes in anthropogenic emissions and +2 °C climate change are expected to affect future air quality, which may have important implications upon human health. It was found that a +2 °C climate change alone was responsible for a modest, and not statistically significant, increase in surface O 3 concentrations (of between −0.1–0.8 ppb in the summer averaged over the European domain) compared to the present climate. Two different emission scenarios were used for the future time period in order to provide an estimate of the extent of air pollution reductions that could occur if (a) all currently planned air quality legislation is implemented and (b) all maximum technologically feasible emission reductions are implemented. The results showed that summer O 3 could be reduced by between 4 and 5 ppb under a current legislation scenario, with at least 3 ppb of further reductions under the maximum mitigated scenario. Calculations of summer ozone enhancement were used as a metric to analyse the results after having removed background ozone level changes. In conclusion it was found that future air quality on a regional scale will depend upon the implementation of effective emission reduction policy; the positive effects of which should not be hindered by a +2 °C global warming. [ABSTRACT FROM AUTHOR]

A 2-degree global warming is likely to affect the production, deposition, and transport of air pollutants, leading to impacts on air quality and health. In the present study we use an ensemble of four regional chemistry-transport models, driven by meteorological data from different climate models, to assess such changes and their uncertainties for PM2.5 and SOMO35. Changes and uncertainties are compared to the inter-model variability. We find that the impact of regional climate change on PM2.5, averaged over the model ensemble, ranges from −0.5 μg.m to +1.3 μg.m over Europe. It mainly results from changes in natural and biogenic emissions, such as desert dust, sea salt and biogenic VOCs. Statistically significant decreases in PM2.5 are found over southwestern Russia and Ukraine as well as an increase over Southern Spain. Modeled changes in summer ozone levels range from −1.7 to 1.6 ppbv. We find a smaller ensemble-mean evolution of SOMO35 as compared to inter-model variability. We also investigate the uncertainty due to inter-decadal variability and find that 10-year periods may not be sufficient to allow the detection of statistically significant change signals. [ABSTRACT FROM AUTHOR]

The impact of meteorological forcings on gas phase air pollutants (ozone and nitrogen dioxide) over Europe was studied using four offline chemistry transport models (CTMs) as part of the IMPACT2C project. This study uses long (20- and 30-year) simulations to evaluate the present-day performance of the CTMs, which is a necessary first step before undertaking any analysis of future air quality impacts. Two sets of meteorological forcings were used for each model: reanalysis of past observation data (ERA-Interim) and Global Climate Model (GCM) output. The results for the simulations forced by reanalysis data were assessed in relation to AirBase v7 measurement data, and it was determined that all four models slightly overpredict annual O 3 values (mean biases range between 0.7 and 6.6 ppb) and three out of the four models underpredict observed annual NO 2 (mean biases range between −3.1 and −5.2 ppb). The simulations forced by climate models result in spatially averaged monthly concentrations of O 3 that are generally between 0 and 5 ppb higher than the values obtained from simulations forced by reanalysis data; therefore it was concluded that the use of climate models introduces an additional bias to the results, but this bias tends not to be significant in the majority of cases. The bias in O 3 results appears to be correlated mainly to differences in temperature and boundary layer height between the two types of simulations, whereas the less significant bias in NO 2 is negatively correlated to temperature and boundary layer height. It is also clear that the selection of chemical boundary conditions is an important factor in determining the variability of O 3 model results. These results will be used as a baseline for the interpretation of future work, which will include an analysis of future climate scenarios upon European air quality. [ABSTRACT FROM AUTHOR]

In order to evaluate the future potential benefits of emission regulation on regional air quality, while taking into account the effects of climate change, off-line air quality projection simulations are driven using weather forcing taken from regional climate models. These regional models are themselves driven by simulations carried out using global climate models (GCM) and economical scenarios. Uncertainties and biases in climate models introduce an additional 'climate modeling' source of uncertainty that is to be added to all other types of uncertainties in air quality modeling for policy evaluation. In this article we evaluate the changes in air quality-related weather variables induced by replacing reanalyses-forced by GCM-forced regional climate simulations. As an example we use GCM simulations carried out in the framework of the ERA-interim programme and of the CMIP5 project using the Institut Pierre-Simon Laplace climate model (IPSLcm), driving regional simulations performed in the framework of the EURO-CORDEX programme. In summer, we found compensating deficiencies acting on photochemistry: an overestimation by GCM-driven weather due to a positive bias in short-wave radiation, a negative bias in wind speed, too many stagnant episodes, and a negative temperature bias. In winter, air quality is mostly driven by dispersion, and we could not identify significant differences in either wind or planetary boundary layer height statistics between GCM-driven and reanalyses-driven regional simulations. However, precipitation appears largely overestimated in GCM-driven simulations, which could significantly affect the simulation of aerosol concentrations. The identification of these biases will help interpreting results of future air quality simulations using these data. Despite these, we conclude that the identified differences should not lead to major difficulties in using GCM-driven regional climate simulations for air quality projections. [ABSTRACT FROM AUTHOR]