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Previous works have demonstrated that the generation of secondary CMB anisotropies due to the molecular optical depth is likely too small to be observed. In this paper, we examine additional ways in which primordial chemistry and the dark ages might influence the CMB. We present a detailed and updated chemical network and give an overview of the interactions of molecules with the CMB. We consider the optical depth due to line absorption, photoionization, photodissociation and free-free processes, and estimate the resulting changes in the CMB temperature and its power spectrum. The most promising results are obtained for the negative hydrogen ion \HM and the \HeHII molecule. The free-free process of \HM yields a relative change in the CMB temperature of up to $2\times10^{-11}$, and leads to a frequency-dependent change in the power spectrum of the order $10^{-7}$ at 30 GHz. With a change of the order $10^{-10}$ in the power spectrum, our result for the bound-free process of \HM is significantly below a previous suggestion. \HeHII efficiently scatters CMB photons and smears out primordial fluctuations, leading to a change in the power spectrum of the order $10^{-8}$. Improvements in the accuracy of future CMB experiments may thus help to constrain and finally detect these interesting signals from the dark ages of the universe., Comment: 16 pages, 15 figures, accepted for publication at A&A. Discussion section updated

The goals of this project were: (1) to present evidence to the scientific community for the importance of the small comet population and (2) to develop techniques for optimum detection in order to characterize the population. The work has been carried out by D. Schleicher (Lowell Observatory), M. A'Hearn and Y. Fernandez (University of Maryland), I.A.F. Stewart, C. Randall, and J. Brandt (University of Colorado).

Narrow-band filter photometry of comet P/Giacobini-Zinner was obtained on 15 nights at Lowell Observatory in the interval from June 15 to Nov. 20, 1985. The emission bands of OH, NH, CN, C3, and C2 were isolated, along with continuum points at 3650 A and 4845 A. All observed species showed pronounced asymmetry about perihelion, with preperihelion abundances being greater by more than a factor of 2 than postperihelion abundances over the heliocentric distance range of 1.0-1.5 AU. The characteristics of the asymmetry were significantly different than observed in previous apparitions, with the peak production rates occurring in late July/early August. The unusually low C2/CN abundance ratio seen in previous apparitions is confirmed by the present observations. Furthermore, the QH data demonstrate that the C2 in Giacobini-Zinner (along with C3 and NH) is depleted when compared to water (the dominant species), rather than CN being unusually over abundant.

Narrowband photometry of Halley obtained at Cerro Tololo Inter-American Observatory (CTIO), Mauna Kea Observatory (MKO), and Perth Observatory was combined to determine the relative level of activity during the interval spanning the spacecraft encounters. Measurements of the flux from the comet in emission bands of OH, NH, CN, C3, and C2, as well as at 2 continuum points, were obtained at CTIO on each night between 5 March and 17 March 1986. Observations were made on many of these same dates at MKO and Perth using comparable interference filters. The date clearly show variation of a factor of 2.5 in the production of all observed species with a characteristic time scale of a few days.

A calculation has been made of the complete fluorescent equilibrium of OD in sunlight including ultraviolet (A-X) transitions, vibrational and rotational transitions (A-A and X-X), and Lambda-doubling transitions in the X state. The dependence on heliocentric radial velocity is strong. No lines of OD are visible in any cometary spectra taken with IUE, but the limits vary, considerably from one comet to another. In the most favorable case, comet Austin 1982 VI, the limit is OD/OH less than 0.004. Optimum conditions for detecting OD in comet Halley are also discussed.

The first direct evidence for the onset of sublimation of a comet nucleus is reported. Emission due to CN observed in spectra of the comet P/Halley provides evidence for the development of the gas coma. Broad-band photometric observations of the comet indicate that the dust coma developed near a preperihelion heliocentric distance r of about 6 AU. Rates of gas production and brightening for the comet have been derived at r of 4-6 AU. The mean preperihelion nuclear magnitude derived for the comet was used to calculate an effective radius of the nucleus, which for plausible values of the geometric albedo lies in the range 1-4 km.

Ultraviolet spectra of comet Austin (1982) obtained in July 1982 at heliocentric distances ranging from 1.10 to 0.81 AU preperihelion with the IUE reveal that the comet is very similar in chemical composition and appearance to comet Bradfield (1979X). In addition, the derived H2O production rate is found to vary with heliocentric distance as r to the -3.6, similar to the r to the -3.7 behavior found for comet Bradfield. It is pointed out, however, that the limited sample rate precludes the observation of the short-term variations which could be produced by a rotating nonuniform cometary nucleus.

Ultraviolet spectra of comet IRAS-Araki-Alcock 1983d, obtained with the International Ultraviolet Explorer spacecraft when the comet was only 0.032 AU from earth, show strong emission bands due to S2, the first detection of this species in an astronomical object. The spatial profiles imply that the S2 is released directly from the nucleus and has a lifetime of the order of 450 s. The derived production rate of S2 was 2 x 10 to the 25th per s. It is suggested that the S2 can be formed by cosmic-ray irradiation of other sulfurous compounds in the ices and that it need not be primordial. It has been also determined that the scale length of the parent of CS (presumably CS2) is 300 km and that the CS production is approximately equal to that of S2, both near 5 x 10 to the -4th that of OH and comparable to that of other trace species observed in comets.

The importance of coordinating different types of observations of a comet is illustrated in terms of spectral data on Comet Bowell. Photometric data in 1980 indicated that OH emissions were occurring when the comet was still more than 4 AU from the sun. Further measurements were arranged with the IUE satellite, the photoelectric scanner at Cerro Tololo and the IR telescope on Mauna Kea. Several sizes of diaphragms were used in order to estimate variations with respect to aperture. Calculations were made to quantify the wavelengths observed as a function of the grains' cross-sections. The OH emission was confirmed by the spectrographic and photometric data. It is suggested that sufficient dark materials are present on the cometary surface to have enhanced the absorption of solar radiation to levels sufficient for heating and dissociating surface ice particles.

Detailed fluorescence calculations for OH including the Swings effect were performed. These calculations were used to reproduce the high resolution spectra of Comets Seargent and Bradfield taken with IUE. The calculations also provide the OH fluorescence efficiencies (g factors), as a function of heliocentric radial velocity, which are needed to derive OH abundances from measured fluxes. A close examination of the spectra shows no sign of the corresponding emission bands of OD allowing upper limits to be placed on the ratio N(OD)/N(OH). Preliminary attempts to reproduce the CO+ band structure by fluorescence are discussed.