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We examine long‐term trends in the near‐surface black carbon mass concentration, using multiyear primary data obtained from a dense network (ARFINET) of observatories over the Indian region. We report for the first time the statistically significant decreasing trend in black carbon mass concentration, based on primary data from this region, at an average rate of ~242 ± 53 ng · m−3 · year−1 during the period 2007–2016. This finding contrasts with the generally increasing trend in the columnar aerosol optical depth, reported earlier, and the steadily increasing trend in anthropogenic activities over this region. The roles of different possible mechanisms, including possible changes in the vertical redistribution of aerosols, are discussed. Over the period 2007–2015, a significant though weak, increasing trend is seen in the contribution from aerosols above 1 km to the columnar aerosol optical depth. These observations imply possible long‐term climate consequences. Key Points: We report the first time regional synthesis of black carbon aerosols over the Indian region using primary dataThe study revealed surprising observation of decreasing trend in the near surface black carbon aerosol concentrationWe found an increasing trend in contribution from free tropospheric aerosols to the columnar aerosol optical depth [ABSTRACT FROM AUTHOR]

Climate change has great significance in Asia in general, and India in particular; and atmospheric aerosols have a decisive role in this. The climate forcing potential of aerosols is closely linked to their optical, microphysical and chemical properties. Systematic efforts to characterize these properties over the Indian region started about 5 decades ago, and evolved over the years through concerted efforts in the form of long-term scientific programmes as well as concerted fields experiments. All these have resulted in this activity becoming one of the most vibrant fields of climate research in India and have brought several important issues in the national and international foci. The field experiment, RAWEX--GVAX (Regional Aerosol Warming Experiment--Ganges Valley Aerosol Experiment), conducted during 2011-12 jointly by the US Department of Energy, Indian Space Research Organization and Department of Science and Technology, has emerged as a direct outcome of the above efforts. This overview provides a comprehensive account of the development of aerosol--climate research in India and south Asia, and the accomplishment and newer issues that warranted the above field campaign. Details of RAWEX--GVAX, the major outcomes and the subsequent and more recent efforts are presented, followed by the way forward in this field for the next several years to come. [ABSTRACT FROM AUTHOR]

Aerosol absorption is poorly quantified because of the lack of adequate measurements. It has been shown that the Ozone Monitoring Instrument (OMI) aboard EOS-Aura and the Moderate Resolution Imaging Spectroradiometer (MODIS) aboard EOS-Aqua, which fly in formation as part of the A-train, provide an excellent opportunity to improve the accuracy of aerosol retrievals. Here, we follow a multi-satellite approach to estimate the regional distribution of aerosol absorption over continental India for the first time. Annually and regionally averaged aerosol single-scattering albedo over the Indian landmass is estimated as 0.94±0.03. Our study demonstrates the potential of multisatellite data analysis to improve the accuracy of retrieval of aerosol absorption over land. [ABSTRACT FROM AUTHOR]

During March-May 2006, an extensive, multi-institution, multi-instrument, and multi-platform integrated field experiment 'Integrated Campaign for Aerosols, gases and Radiation Budget' (ICARB) was carried out under the Geosphere Biosphere Programme of the Indian Space Research Organization (ISRO-GBP). The objective of this largest and most exhaustive field campaign, ever conducted in the Indian region, was to characterize the physico-chemical properties and radiative effects of atmospheric aerosols and trace gases over the Indian landmass and the adjoining oceanic regions of the Arabian Sea, northern Indian Ocean, and Bay of Bengal through intensive, simultaneous observations. A network of ground-based observatories (over the mainland and islands), a dedicated ship cruise over the oceanic regions using a fully equipped research vessel, the Sagar Kanya, and altitude profiling over selected regions using an instrumented aircraft and balloonsondes formed the three segments of this integrated experiment, which were carried out in tandem. This paper presents an overview of the ICARB field experiment, the database generated, and some of its interesting outcomes though these are preliminary in nature. The ICARB has revealed significant spatio-temporal heterogeneity in most of the aerosol characteristics both over land and ocean. Observed aerosol loading and optical depths were comparable to or in certain regions, a little lower than those reported in some of the earlier campaigns for these regions. The preliminary results indicate: • low (< 0.2) aerosol optical depths (AOD) over most part of the Arabian Sea, except two pockets; one off Mangalore and the other, less intense, in the central Arabian Sea at ∼18°N latitude; • High Ångström exponent in the southern Arabian Sea signifying steep AOD spectra and higher abundance of accumulation mode particles in the southern Arabian Sea and off Mangalore; • Remarkably low Ångström exponents signifying increased concentration of coarse mode aerosols and high columnar abundance in the northern Arabian Sea; • Altitude profiles from aircraft showed a steady BC level up to 3 km altitude with structures which were associated with inversions in the atmospheric boundary layer (ABL); • A surprisingly large increase in the BC mass fraction with altitude; • Presence of a convectively mixed layer extending up to about 1 km over the Arabian Sea and Bay of Bengal; • A spatial off shore extent of <100 km for the anthropogenic impact at the coast; and • Advection of aerosols, through airmass trajectories, from west Asia and NW arid regions of India leading to formation of elevated aerosol layers extending as far as 400 km off the east coast. [ABSTRACT FROM AUTHOR]

Extensive measurements of columnar aerosol optical depth (AOD), composite (MT) and black carbon aerosol mass (MB) concentrations were made over the tropical Indian and Southern Oceans as a part of the Pilot Expedition to the Southern Ocean during the boreal winter. The AOD, MT and MB show large latitudinal gradient towards south up to ITCZ. Beyond ITCZ, up to 56°S, AOD and MB show very low and steady values. However MT shows large variations in the Southern Ocean due to the enhanced production of sea salt aerosols associated with high sea surface winds. The short wave aerosol radiative forcing at the surface over north of equator is in the range - 10 to - 23 W m-2, whereas that over the Southern Ocean was in the range - 4 to - 5 W m-2. The corresponding atmospheric forcing was in the range of 6-13 W m-2 and 0.8-1.4 W m-2. This large north-south change in the aerosol radiative forcing has important implications to the meridional circulation and hence to climate. [ABSTRACT FROM AUTHOR]

During the second phase of the Arabian Sea Monsoon Experiment (ARMEX-II), extensive measurements of spectral aerosol optical depth, mass concentration, and mass size distribution of ambient aerosols as well as mass concentration of aerosol black carbon (BC) were made onboard a research vessel during the intermonsoon period (i.e., when the monsoon winds are in transition from northeasterlies to westerlies/southwesterlies) over the Arabian Sea (AS) adjoining the Indian Peninsula. Simultaneous measurements of spectral aerosol optical depths (AODs) were made at different regions over the adjoining Indian landmass. Mean AODs (at 500-nm wavelength) over the ocean (∼0.44) were comparable to those over the coastal land (∼0.47), but were lower than the values observed over the plateau regions of central Indian Peninsula (∼0.61). The aerosol properties were found to respond distinctly with respect to change in the trajectories, with higher optical depths and flatter AOD spectra associated with trajectories indicating advection from west Asia, and northwest and west-coastal India. On average, BC constituted only ∼2.2% to total aerosol mass compared to the climatological values of ∼6% over the coastal land during the same season. These data are used to characterize the physical properties of aerosols and to assess the resulting short-wave direct aerosol forcing. The mean values were –27 W m-2 at the surface and -12 W m-2 at the top of the atmosphere (TOA), resulting in a net atmospheric forcing of +15 W m-2. The forcing also depended on the region from where the advection predominates. The surface and atmospheric forcing were in the range -40 to -57 W m-2 and +27 to +39 W m-2, respectively, corresponding to advection from the west Asian and western coastal India where they were as low as -19 and +10 W m-2, respectively, when the advection was mainly from the Bay of Bengal and from central/peninsular India. In all these cases, the net atmospheric forcing (heating) efficiency was lower than the values reported for northern Indian Ocean during northern winter, which is attributed to the reduced BC mass fraction. [ABSTRACT FROM AUTHOR]

Simultaneous and collocated measurements of total and hemispherical backscattering coefficients (σ and β, respectively) at three wavelengths, mass size distributions, and columnar spectral aerosol optical depth (AOD) were made onboard an extensive cruise experiment covering, for the first time, the entire Bay of Bengal (BoB) and northern Indian Ocean. The results are synthesized to understand the optical properties of aerosols in the marine atmospheric boundary layer and their dependence on the size distribution. The observations revealed distinct spatial and spectral variations of all the aerosol parameters over the BoB and the presence of strong latitudinal gradients. The size distributions varied spatially, with the majority of accumulation modes decreasing from north to south. The scattering coefficient decreased from very high values (resembling those reported for continental/urban locations) in the northern BoB to very low values seen over near-pristine environments in the southeastern BoB. The average mass scattering efficiency of BoB aerosols was found to be 2.66 ± 0.1 m2 g-1 at 550 nm. The spectral dependence of columnar AOD deviated significantly from that of the scattering coefficients in the northern BoB, implying vertical heterogeneity in the aerosol type in that region. However, a more homogeneous scenario was observed in the southern BoB. Simultaneous lidar and in situ measurements onboard an aircraft over the ocean revealed the presence of elevated aerosol layers of enhanced extinction at altitudes of 1 to 3 km with an offshore extent of a few hundred kilometers. Back-trajectory analyses showed these layers to be associated with advection from west Asia and western India. The large spatial variations and vertical heterogeneity in aerosol properties, revealed by the present study, need to be included in the regional radiative forcing over the Bay of Bengal. [ABSTRACT FROM AUTHOR]

Spectral aerosol optical depth (AOD) measurements, carried out regularly from a network of observatories spread over the Indian mainland and adjoining islands in the Bay of Bengal and Arabian Sea, are used to examine the spatio-temporal and spectral variations during the period of ICARB (March to May 2006). The AODs and the derived Ångström parameters showed considerable variations across India during the above period. While at the southern peninsular stations the AODs decreased towards May after a peak in April, in the north Indian regions they increased continuously from March to May. The Ångström coefficients suggested enhanced coarse mode loading in the north Indian regions, compared to southern India. Nevertheless, as months progressed from March to May, the dominance of coarse mode aerosols increased in the columnar aerosol size spectrum over the entire Indian mainland, maintaining the regional distinctiveness. Compared to the above, the island stations showed considerably low AODs, so too the northeastern station Dibrugarh, indicating the prevalence of cleaner environment. Long-range transport of aerosols from the adjoining regions leads to remarkable changes in the magnitude of the AODs and their wavelength dependencies during March to May. HYSPLIT back-trajectory analysis shows that enhanced long-range transport of aerosols, particularly from the west Asia and northwest coastal India, contributed significantly to the enhancement of AOD and in the flattening of the spectra over entire regions; if it is the peninsular regions and the island Minicoy are more impacted in April, the north Indian regions including the Indo Gangetic Plain get affected the most during May, with the AODs soaring as high as 1.0 at 500 nm. Over the islands, the Ångström exponent (α) remained significantly lower (∼1) over the Arabian Sea compared to Bay of Bengal (BoB) (∼1.4) as revealed by the data respectively from Minicoy and Port Blair. Occurrences of higher values of α, showing dominance of accumulation mode aerosols, over BoB are associated well with the advection, above the boundary layer, of fine particles from the east Asian region during March and April. The change in the airmass to marine in May results in a rapid decrease in α over the BoB. [ABSTRACT FROM AUTHOR]