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International audience; Agile management of the optical orbital angular momentum encompasses temporal, spatial, and spectral aspects that, once combined, offer new perspectives in our way to manipulate light. To date the spectral control is mainly limited to tunable operating wavelength and polychromatic capabilities. Recently, a multispectral approach has been proposed [Phys. Rev. Lett. 121, 213901 (2018)] to achieve independent orbital angular momentum state control on multiple spectral channels. Here we report on the design, fabrication and implementation of a solid-state multispectral approach that consists of arrays of optical diamond micro-metasurfaces. Obtained device exhibits superior performances with respect to the original attempt, both regarding the spectral vortex purity, the ability to deal with high photon flux, and the orbital angular momentum diversity across the spectrum. These results motivate further development of metasurface-based integrated spin-orbit photonics technologies.

International audience

Among the properties of light that dictate its mechanical effects, polarization has held a special place since the mechanical identification of the photon spin1. Nowadays, little surprise might be expected from the mechanical action of linearly polarized weakly focused (paraxial) beams on transparent and homogeneous dielectrics. Still, here we unveil vectorial optomechanical effects mediated by the material anisotropy and the longitudinal field component inherent to real-world beams2,3. Experimentally, this is demonstrated by using an elastic anisotropic medium prone to exhibit a sensitive and reversible effect, that is, a nematic liquid crystal, and our results are generalized to vector beams4. This represents an alternative to irreversible damaging approaches restricted to strongly non-paraxial fields5. The reported creation of multiple self-induced lenses from a single beam also open up topology assisted all-optical information routing strategies. Moreover, our findings point out the transverse internal optical energy flows (spin and orbital)6 as novel triggers to tailor structured optical nonlinearities. Researchers demonstrate vectorial optomechanical effects using a nematic liquid crystal and report creation of multiple self-induced lenses from a single beam.

International audience; Structuring light attracts continuous research effort due to its impactful applications in optical information and communications, laser material processing, optical imaging, or optical manipulation of matter. In particular, femtosecond laser direct writing of photoresists is a technology dedicated to the creation of optically isotropic free-form 3D micro-optical elements with size, spatial resolution, and surface quality that qualify to demanding integrated optics needs. Here, we report on the design, production, and characterization of dielectric metasurface birefringent optical retarders made from femtosecond laser 3D printing technology whose polarization conversion efficiency is more than 10 times larger than that previously reported Wang et al., Appl. Phys. Lett. 110, 181101 (2017)]. As the flexibility of the fabrication process allows considering arbitrary orientation of the artificially engineered optical axis, these results open up for 3D printed geometric phase optical elements.

We report on the conversion of an infrared vector beam into THz vortex beams using a ZnTe cubic crystal. We provide a theoretical analysis demonstrating how an infrared vector beam with the azimuthal order l can be transformed into a THz beam endowed with an orbital angular moment content that consists of optical vortices with topological charge ±2l. Experimentally, quasi-monochromatic THz vortex beams with topological charges +2 and −2 are produced and characterized both in amplitude and phase using real-time two-dimensional imaging of the terahertz electric field.

International audience; We propose an approach to achieve achromatic pure geometric phase shaping of light from anisotropic media by exploiting the fundamental laws of electromagnetic waves. Its practical implementation requires a cover layer made of a dispersive isotropic medium. The approach applies to any anisotropic material and any geometric phase spatial distribution and preserves the geometric phase reversal upon the reversal of the incident polarization handedness. An experimental demonstration is made over the whole visible range but can be extended to any wavelength range without conceptual issues.

International audience; Spontaneously formed liquid crystal topological defects under external fields offer a nature-assisted route to the creation of geometric phase optical vortex generators (q-plates). Here we report on the consequences of the unavoidable swirled transverse spatial distribution of the optical axis of such optical elements on the beam shaping and we propose a swirl-compensation scheme based on the arithmetic of geometric phase optical elements.

International audience; We report on a programmable liquid crystal spatial light modulator enabling independent orbital angular momentum state control on multiple spectral channels. This is done by using electrically controllable “topological pixels" that independently behave as geometric phase micro-optical elements relying on selfengineered liquid crystal defects. These results open interesting opportunities in optical manipulation, sensing, imaging, and communications, as well as information processing. In particular, spectral vortex modulation allows considering singular spatiotemporal shaping of ultrashort pulses which may find applications in many areas such as material processing, spectroscopy, or elementary particles acceleration.

International audience; Photonics have developed greatly over the last several decades and brought about a variety of new concepts in communica tions, sensing, solar energy and many other fields. With the emerging applications of quantum technologies and all optical data processing, the impact of photonics on technology is unde niable, as evidenced through the International Year of Light and Light based Technologies in 2015.

International audience; We present and test the integration of a static orbital angular momentum mode multiplexer with a dynamical geometric-phase optical element, enabling on-demand spin-controlled angular momentum multiplexing. A diffractive optic multiplexer fabricated by 3D high-resolution electron beam lithography performs a conformal mapping for the conversion from linear to azimuthal phase gradients. The latter is functionalized by a dynamic spin-orbit add-on that consists of a self-engineered electrically activated liquid crystal optical vortex generator having large clear-aperture and high-resolution. By combining several functionalities based on the optical angular momentum of light in a compact manner, the proposed hybrid device could find applications in next-generation high-dimensional mode switchers and routers based on orbital angular momentum.

In this work we reveal an influence of polarization of the laser beam on polymerization in direct laser writing. It was experimentally found that the width of suspended lines fabricated in SZ2080, OrmoComp and PETA (pentaerythritol triacrylate) pre-polymers directly depends on the incident polarization and is largest when the angle between the electric field vector and the sample translation direction is α = 90° and the smallest when α = 0°. The size of polymerized structures is consistent with theoretical simulations based on vectorial Debye theory. Experiments were performed by using average laser power corresponding to the middle value of the fabrication window. Polarization was found to be affecting feature sizes while structuring various widespread photoresists, the observed variation was material dependent and measured from 5 to 22% in the line-width. The performed study proves that polarization can be used as a variable parameter for fine tuning of the voxel's aspect ratio.

International audience; We report on the design, fabrication, and experimental characterization of reflective geometric phase optical elements enabling the generation of scalar and vectorial high-order Laguerre-Gauss optical beams over a broad spectral range. This is made possible by combining azimuthal and radial structuring of helix-based liquid-crystal films exhibiting the circular Bragg reflection phenomenon. By extending the previously introduced concept of Bragg-Berry optical elements to the polychromatic shaping of the radial degrees of freedom and showing their combination with azimuthal ones, this work suggests that spectrally broadband spin-orbit processing of optical information over multiple spatial degrees of freedom can be further considered on experimental grounds.

International audience; Geometric phase optical elements based on structured anisotropy are widely used for phase shaping via their orienta-tional degree of freedom. To date, amplitude shaping via space-variant retardance is much less investigated, a practical reason being that the spin-orbit interaction of light couples retardance with the dynamic part of the optical phase. Inspired by the complementary diffractive elements associated with Babinet's principle, a bilayered subwavelength grating design is proposed in order to cancel out the spatial modulation of the dynamic phase usually associated with space-variant birefringent phase retardation. This concept is illustrated in the framework of single-mode Laguerre Gauss –beam shaping.

International audience; Optical vortex phase masks are now installed at many ground-based large telescopes for high-contrast astronomical imaging. To date, such instrumental advances have been restricted to the use of helical phase masks of the lowest even order, while future giant telescopes will require high-order masks. Here we propose a single-stage on-axis scheme to create high-order vortex coronagraphs based on second-order vortex phase masks. By extending our approach to an off-axis design, we also explore the implementation of multiple-star vortex coronagraphy. An experimental laboratory demonstration is reported and supported by numerical simulations. These results offer a practical roadmap to the development of future coronagraphic tools with enhanced performances.

International audience; Artificially engineered geometric phase optical elements may have tunable photonic functionalities owing to their sensitivity to external fields, as is the case for liquid crystal based devices. However, liquid crystal technology combining high-resolution topological ordering with tunable spectral behavior remains elusive. Here, by using a magnetoelectric external stimulus, we create robust and efficient self-engineered liquid crystal geometric phase vortex masks with a broadly tunable operating wavelength, centimeter-size clear aperture, and high-quality topological ordering.

Observing and taming unusual effects arising from non-trivial light-matter interaction has always triggered scientists to better understand Nature and develop technological tools towards implementing novel applications. Recently, several unusual optomechanical effects have been unveiled when subtle spin-orbit interactions come at play to build up optical forces and torques that are hardly seen in everyday life, such as negative optical radiation pressure, transverse optical forces, or left-handed optical torques. To date, there are only a few experimental proposals to reveal these effects despite tremendous conceptual advances. In particular, spin-dependent lateral forces and their angular analog are done either at the expense of direct observations or at the cost of specific instrumental complexity. Here we report on naked-eye identification of light-induced spin-dependent lateral displacements of centimeter-sized objects endowed with structured birefringence. Its angular counterpart is also discussed and the observation of left-handed macroscopic rotational motion is reported. The unveiled effects are ultimately driven by lateral optical force fields that are five orders of magnitude larger than those reported so far. These results allow structured light-matter interaction to move from a scientific curiosity to a new asset for the existing multidisciplinary optical manipulation toolbox across length scales. In addition, this highlights the spin-orbit optomechanics of anisotropic and inhomogeneous media, which is just beginning to be explored.

International audience; By making use of the spin angular momentum of light, rotational frequency shifts of harmonic waves generated by spinning nonlinear media have been observed.

The realization of geometric phase optical device operating over a broad spectral range is usually confronted with intrinsic limitations depending of the physical process at play. Here we propose to use chiral nematic liquid crystal slabs with helical ordering that varies in three dimensions. Namely, gradient-pitch cholesterics endowed with in-plane space-variant angular positioning of the supramolecular helix. By doing so, we show that the recently introduced Bragg-Berry mirrors [Opt. Lett. {\bf 41}, 3972-3975 (2016)] can be endowed with ultra-broadband spectral range. Experimental demonstration is made in the case of ultra-broadband optical vortex generation in the visible domain. These results offer practical solution to the polychromatic management of the orbital angular momentum of light combining the circular Bragg reflection of chiral media with the Berry phase., Comment: 11 pages, 13 figures

International audience; Structured light beams, such as optical vortices, vector beams, and non-diffracting beams, have been recently studied in a variety of fields, such as optical manipulations, optical telecommunications, nonlinear interactions, quantum physics, and 'super resolution' microscopy.. Their unique physical properties, such as annular intensity profile, helical wavefront and orbital angular momentum, give rise to a plethora of new, fundamental light-matter interactions and device applications. Recent progress in nanostructured materials, including metamaterials and metasurfaces, opened new opportunities for structured light generation on the microscale that exceed the capabilities of bulk-optics approaches such as computer generated holography and diffractive optics. Furthermore, structured optical fields may interact with matters on the subwavelength scale to yield new physical effects, such as spin-orbital momentum coupling. This special issue of Optics Express focuses on the state-of-the-art fundamental research and emerging technologies and applications enabled by the interplay of " structured light " and " structured materials " .

Three dimensional (3D) fast (< 0.5 hour) printing of micro-optical elements down to sub-wavelength resolution over 100 micrometers footprint areas using femtosecond (fs-)laser oscillator is presented. Using sub-1 nJ pulse energies, optical vortex generators made of polymerised grating segments with an azimuthally changing orientation have been fabricated in SZ2080 resist; width of polymerised rods was ~150 nm and period 0.6-1 micrometers. Detailed phase retardance analysis was carried out manually with Berek compensator (under a white light illumination) and using an equivalent principle by an automated Abrio implementation at 546 nm. Direct experimental measurements of retardance was required since the period of the grating was comparable (or larger) than the wavelength of visible light. By gold sputtering, transmission-type optical vortex generators were turned into reflective ones with augmented retardance, n.h defined by the form birefringence, n, and the height h = 2d where d is the thickness of the polymerised structure. Retardance reached 315 nm as measured with Berek compensator at visible wavelengths. Birefringent phase delays of 180 degrees (or half-wavelength) required for high purity vortex generators can be made based on the proposed approach. Optical vortex generators for telecom wavelengths with sub-wavelength patterns of azimuthally oriented gratings are amenable by direct laser polymerisation., Pacific Rim Laser Damage 2017: Optical Materials for High Power Lasers (PLD17); Shanghai, China 21 - 24 May 2017. Invited talk

We propose a topological beam-shaping strategy of terahertz beams using geometric phase elements made of space-variant birefringent slabs. Quasi-monochromatic terahertz vortex beams are produced and characterized both in amplitude and phase from the reconstructed real-time two-dimensional imaging of the electric field. Nonseparable superpositions of such vortex beams are also obtained and characterized by two-dimensional polarimetric analysis. These results emphasize the versatility of the spin-orbit electromagnetic toolbox to prepare on-demand structured light endowed with polarization-controlled orbital angular momentum content in the terahertz domain, which should find many uses in future terahertz technologies.

International audience; Reflective geometric phase flat optics made from chiral anisotropic media recently unveiled a promising route towards polychromatic beam shaping. However, these broadband benefits are strongly mitigated by the fact that flipping the incident helicity does not ensure geometric phase reversal. Here we overcome this fundamental limitation by a simple and robust add-on whose advantages are emphasized in the context of spin-to-orbital angular momentum mapping.

International audience; We propose to use a femtosecond direct laser writing technique to realize dielectric optical elements from photo-resist materials for the generation of structured light from purely geometrical phase transformations. This is illustrated by the fabrication and characterization of spin-to-orbital optical angular momentum couplers generating optical vortices of topological charge from 1 to 20. In addition, the technique is scalable and allows obtaining microscopic to macroscopic flat optics. These results thus demonstrate that direct 3D photopolymerization technology qualifies for the realization of spin-controlled geometric phase optical elements.

International audience; We propose a topological beam-shaping strategy of terahertz (THz) beams using geometric phase elements made of space-variant birefringent slabs. Quasi-monochromatic THz vortex beams are produced and characterized both in amplitude and phase from the reconstructed real-time two-dimensional imaging of the electric field. Nonseparable superpositions of such vortex beams are also obtained and characterized by two-dimensional polarimetric analysis. These results emphasize the versatility of the spin-orbit electromagnetic toolbox to prepare on-demand structured light endowed with polarization-controlled orbital angular momentum content in the THz domain, which should find many uses in future THz technologies.

International audience; We propose the development of a high contrast imaging technique enabling the simultaneous and selective nulling of several light sources. This is done by realizing a reconfigurable multiple vortex phase mask made of a liquid crystal thin film on which local topological features can be addressed electro optically. The method is illustrated by reporting on a triple star optical vortex coronagraphy laboratory demonstration, which can be easily extended to higher multiplicity. These results allow considering the direct observation and analysis of worlds with multiple suns and more complex extrasolar planetary systems.

International audience; We explore the spin-orbit nature of the optical torque exerted on chiral liquid-crystal microspheres exhibiting circular Bragg reflection. Experimental investigation relies on the direct optomechanical observation of spinning liquid-crystal droplets immersed in water and held in a circularly polarized laser levitator. More generally, we anticipate that the total angular momentum transfer per photon may depart from the commonly assumed spin-only ±2¯ h contribution, when the topological features of the illuminated microsphere are taken into account.

International audience; We report on a self-induced strategy to achieve high-contrast optical imaging, without the need for any man-made optical masks, which relies on the self-induced spin-to-orbital angular momentum conversion phenomenon. This is experimentally demonstrated by realizing a laboratory demonstration of self-eclipsing of a light source following the generation of a self-adapted vectorial optical vortex transmission mask. The proposed concept, namely the realization of an alignment-free optical vortex corona-graph, may inspire the development of future generations of smart astronomical imaging instruments.

The generation of a left-handed torque that acts in the opposite direction to light's natural spin angular momentum is reported. The effect is achieved by sending circularly polarized light into an azimuthally patterned birefringent glass disk. Optical forces and torques are two mechanical degrees of freedom available to manipulate matter, and form the basis of optical tweezing strategies1,2. In contrast to the Keplerian intuition that objects should be pushed downstream an incident photon flux, the concept of ‘negative’ optical forces has recently been described3,4 and has triggered many developments5,6,7,8,9,10,11,12,13,14. Here, we report on the counterintuitive angular analogue of negative optical forces by demonstrating that circularly polarized Gaussian light beams give rise to torque with opposite sign to that of the incident optical angular momentum. Such a ‘left-handed’ mechanical effect is demonstrated by the use of an inhomogeneous and anisotropic transparent macroscopic medium. Practical difficulties associated with the direct observation of optically induced spinning of a macroscopic object are circumvented via the rotational Doppler effect15,16. These results shed light on spin–orbit optomechanics and equip the left-handed optomechanical toolbox with angular features.

International audience; Here, we report on the experimental demonstration that highly efficient self-induced spin-orbit optical vortex generation can be achieved by using standard liquid crystal materials and surface treatment agents. This is done by revisiting the recent attempt by Zolot’ko and coworkers to produce self-induced liquid crystal vortex plates using the dc electric field [I. A. Budagovsky, S. A. Shvetsov, and A. S. Zolot’ko, Mol. Cryst. Liq. Cryst. 637, 47 (2016)] that remains, so far, limited to moderate efficiencies. The phenomenon is the result of the self-back-action of light arising from the spontaneous creation of a liquid crystal topological defect. These results demonstrate photo-electric interface activation as a candidate towards the development of a self-adapted spinorbit photonic toolbox, thus enabling agile management of the orbital angular momentum of light.

International audience; We propose a novel class of refractive optical elements by wrinkling the conical surface of a usual (conical) axicon, which leads to geometrical singularities (cusps). Such wrinkled axicons have been fabricated at the micron scale by using three-dimensional femtosecond-laser photopolymerization technique and we report on their experimental and numerical characterization. The beam shaping capabilities of these structures are discussed for both intensity and phase, which includes topological beam shaping that results from azimuthally modulated optical spin-orbit interaction.

Interaction between the polarization and spatial degrees of freedom of a light field has become a powerful tool to tailor the amplitude and phase of light beams. This usually implies the use of space-variant photonic elements involving sophisticated fabrication technologies. Here we report on the optical spin–orbit engineering of the intensity, phase, and polarization structure of Bessel light beams using a homogeneous birefringent axicon. Various kinds of spatially modulated free-space light fields are predicted depending on the nature of the incident light field impinging on the birefringent axicon. In particular, we present the generation of bottle beam arrays, hollow beams with periodic modulation of the core size, and hollow needle beams with periodic modulation of the orbital angular momentum. An experimental attempt is also reported. The proposed structured light fields may find applications in long-distance optical manipulation endowed with self-healing features, periodic atomic waveguides, contactless handling of high aspect ratio micro-objects, and optical shearing of matter.

Controlling the angular spectrum content of light fields is a basic beam shaping strategy implying the control of the wavevector distribution. Here we propose a novel class of refractive optical elements generated by folding the conical surface of a usual (conical) axicon. In particular, we explore folding processes where the continuous deformation of the circular cross-section of an axicon lead to the appearance of geometrical singularities (cusps). This is illustrated considering two prototypical families derived from hypocycloidal and epicycloidal geometries. Such topological axicons have been fabricated at the micron scale by using photopolymerization technique and characterized both experimentally and theoretically.

In 1931, French astronomer Bernard Lyot suggested that placing a beam stop in the center of the Fourier plane of a telescope allows observing faint objects nearby on-axis bright sources. This opened a new chapter in astronomical imaging called coronagraphy. Since then various techniques have been proposed and implemented experimentally. In particular, it was shown that pure phase masks, instead of amplitude ones, is an efficient way to reject on-axis light. Since one decade, there is a growing interest in spiraling phase (optical vortex) masks that may create of a nodal area at the exit pupil plane of the telescope outside which on-axis light is rejected. Such optical vortex coronagraphy implies the development of singular phase masks endowed with well defined topological properties. To this aim, nowadays nanofabrication tools are a prime choice, which includes liquid crystal photo-alignment technology. Here we show that spontaneously occurring liquid crystal topological defects offer a smart alternative to optical vortex phase masks. Our first experimental smart coronagraphy observations will be presented and discussed.

International audience; We report on a soft route toward optical vortex coronagraphy based on self-engineered electrically tunable vortex masks made of liquid crystal topological defects. These results suggest that a nature-assisted technological approach to the fabrication of complex phase masks could be useful in optical imaging whenever optical phase singularities are at play.

International audience; We report on the experimental realization of flat mirrors enabling the broadband generation of optical vortices upon reflection. The effect is based on the geometric Berry phase associated with the circular Bragg reflection phenomenon from chiral uniaxial media. We show the reflective optical vortex generation from both diffractive and nondiffractive paraxial light beams using spatially patterned chiral liquid crystal films. The intrinsic spectrally broadband character of spin-orbit generation of optical phase singularities is demonstrated over the full visible domain. Our results do not rely on any birefringent retardation requirement and, consequently, foster the development of a novel generation of robust optical elements for spin-orbit photonic technologies.

International audience; Tailoring the spatial degree of freedom of light is an essential step towards the realization of advanced optical manipulation tools. A topical challenge consists of device miniaturization for improved performance and enhanced functionality at the micron scale. We demonstrate a novel approach that combines the additive three-dimensional (3D) structuring capability of laser polymerization and the subtractive subwavelength resolution patterning of focused ion beam lithography. As a case in point hybrid (dielectric/metallic) micro-optical elements that deliver a well-defined topological shaping of light are produced. Here we report on hybrid 3D binary spiral zone plates with unit and double topological charge. Their optical performances are compared to corresponding 2D counterparts both numerically and experimentally. Cooperative refractive capabilities without compromising topological beam shaping are shown. Realization of advanced designs where the dielectric architecture itself is endowed with singular properties is also discussed.

International audience; We report on highly reflective spin orbit geometric phase optical elements based on a helicity preserving circular Bragg reflection phenomenon. First, we present a dynamical geometric phase experiment using a flat chiral Bragg mirror. Then, we show that shaping such a geometric phase allows the efficient spin orbit tailoring of light fields without the need to fulfill any condition on birefringent phase retardation, in contrast to the case of transmission spin orbit optical elements. This is illustrated by optical vortex generation from chiral liquid crystal droplets in the Bragg regime that unveils spin orbit consequences of the droplet's curvature. Our results thus introduce a novel class of geometric phase elements " Bragg Berry " optical elements.

Advances of the growing field of micro-optical elements and components created via direct laser writing (DLW) are overviewed. The basic principles and the most recent developments in three-dimensional (3D) DLW in polymers enable creation of miniaturized and integrated optical devices. The employed technique based on femtosecond laser pulses provides efficient and reliable structuring with up to ∼100 nm feature definition as well as less than 10 nm surface roughness required for optical/photonic applications. Research into the structuring by ultrashort laser pulses has seen immense growth over the past decade due to its unique material processing features involving linear and nonlinear photophysical and photochemical mechanisms. This enables nanostructuring of pure organic, hybrid organic–inorganic, as well as hydrogel or elastomer materials via avalanche-induced cross-linking, thus without the usage of any photosensitizers. This approach empowers manufacturing of the low optical losses and high damage threshold, as well as biocompatible elements. Examples of various micro-optical elements are provided with focus on refractive index measurement and engineering for a particular optical function along with unique performance of the miniature devices.

International audience; Interaction between the polarization and spatial degrees of freedom of a light field has become a powerful tool to tailor the amplitude and phase of light beams. This usually implies the use of space-variant photonic elements involving sophisticated fabrication technologies. Here we report on the optical spin orbit engineering of the intensity, phase, and polarization structure of Bessel light beams using a homogeneous birefringent axicon. Various kinds of spatially modulated free-space light fields are predicted depending on the nature of the incident light field impinging on the birefringent axicon. In particular, we present the generation of bottle beam arrays, hollow beams with periodic modulation of the core size, and hollow needle beams with periodic modulation of the orbital angular momentum. An experimental attempt is also reported. The proposed structured light fields may find applications in long-distance optical manipulation endowed with self-healing features, periodic atomic waveguides, contactless handling of high aspect ratio micro-objects, and optical shearing of matter.

International audience; We report on the conversion of an infrared vector beam into terahertz vortex beams using a 110-cut ZnTe cubic crystal. First, we provide a theoretical analysis demonstrating how an infrared vector beam with the azimuthal order can be transformed into a terahertz beam endowed with an orbital angular moment content that consists of optical vortices with topological charge ±2. Experimentally, quasi-monochromatic terahertz vortex beams with topological charges +2 and −2 are produced and characterized both in amplitude and phase using real-time two-dimensional imaging of the terahertz electric field. These results enrich the terahertz vortex beam toolbox via the transfer of topological information from infrared to tera-hertz domains.

International audience; The high sensitivity of liquid crystals to external fields, especially electromagnetic fields, confer to them fascinating properties. In the case of light fields, their large optical nonlinearities over a broad spectrum have great application potential for all-optical devices. The linear optical properties of liquid crystals, such as their high refractive index, birefringence and transparency, are also of great practical interest in optofluidics, which combines the use of optical tools in microfluidic environments. A representative example is the laser micromanipulation of liquid crystalline systems using optical tweezing techniques. Liquid crystal droplets represent a class of systems that can be easily prepared and manipulated by light, with or without a nonlinear light-matter coupling. Here we review different aspects of quasi-statics and dynamical optical angular manipulation of liquid crystal droplets trapped in laser tweezers. In particular, we discuss to the influence of the phase (nematic, cholesteric or smectic), the bulk ordering symmetry, the droplet size, the polarization state and power of the trapping light, together with the prominent role of light-matter angular momentum exchanges and optical orientational nonlinearities.

International audience; Orbital angular momentum carrying light beams are usedfor optical trapping and manipulation. This emerging trend provides new challenges involving device miniaturization for improved performance and enhanced functionality at the microscale. Here we discus a new fabrication method based on combining the additive 3D structuring capability laser photopolymerization and the substractive sub-wavelength resolution patterning of focused ion beam lithography to produce micro-optical elements capable of compound functionality. As a case in point of this approach binary spiral zone pattern based high numerical aperture micro-lenses capable of generating topological charge carrying tightly focused vortex beams in a single wavefront transformation step are presented. The devices were modelled using finite-difference time-domain simulations, and the theoretical predictions were verified by optically characterizing the propagation properties of light transmitted through the fabricated structures. The resulting devices had focal lengths close to the predicted values of f = 18 µm and f = 13 µm as well as topological charge ℓ dependent vortex focal spot sizes of ~ 1:3 µm and ~ 2:0 µm for ℓ = 1 and ℓ = 2 respectively.

International audience; We report on structured light-induced femtosecond direct laser writing (DLW) under tight focusing in non-commercial silver-containing zinc phosphate glass, which leads to original patterns of fluorescent silver clusters. These fluorescence topologies show unique features of frustrated diffusion of charged species, giving rise to distorted silver cluster spatial distributions. Fluorescence and second harmonic generation correlative microscopy demonstrate the realization of structured light-induced direct laser poling, resulting from a laser-induced permanent and stable electric field buried inside the modified glass. Thus, structured light-induced DLW remarkably enables both linear and nonlinear patterning. This work highlights the interest of optical phase engineering to obtain nontrivial beam profiles and subsequent photo-induced patterns that cannot be reached under Gaussian beam irradiation.

Focused ion beam (FIB) milling with a 10 nm resolution is used to directly write metallic metasurfaces and micro-optical elements capable to create structured light fields. Surface density of fabricated nano-features, their edge steepness as well as ion implantation extension around the cut line depend on the ion beam intensity profile. The FIB beam intensity cross section was evaluated using atomic force microscopy (AFM) scans of milled line arrays on a thin Pt film. Approximation of two Gaussian intensity distributions describes the actual beam profile composed of central high intensity part and peripheral wings. FIB fabrication reaching aspect ratio of 10 in gold film is demonstrated.

Optically induced reorientation dynamics in a nematic liquid crystal is investigated for circularly polarized laser beams with spot sizes smaller than the sample thickness. Various dynamical regimes, such as periodic, quasi-periodic, intermittent, self-organized and possibly chaotic regimes are observed. The role finite beam size is identified and a qualitative interpretation based on the spatial walk-off of the ordinary and extraordinary beams arising from double refraction phenomenon is proposed.

International audience; A quasi-modal version of the recently introduced Laguerre-Gaussian modal q-plates [Rafayelyan and Brasselet, Opt. Lett. 42, 1966–1969 (2017)] is proposed and implemented using femtosecond direct laser writing of space-variant nanogratings in the bulk of silica glass. The corresponding design consists of linear azimuthal modulation of the optical axis orientation and polynomial radial modulation of the retardance profile. Experimental demonstration is made for Laguerre-Gaussian modes with azimuthal indices l =(1, 2, 3) and radial index p = 0. Such quasi-modal q-plates overcome previous limitations regarding the robustness of modality against the handedness of the incident circular polarization state.

International audience; We propose space-variant uniaxial flat optical elements designed to generate pure Laguerre–Gaussian modes with arbitrary azimuthal and radial indices l and p from an incident Gaussian beam. This is done via the combined use of the dynamic and the geometric phases. Optimal design protocol for the mode conversion efficiency is derived, and the corresponding characteristics are given for −6≤l≤6 and 0≤p≤5. The obtained “modal q-plates” may find many applications whenever the radial degree of freedom of a light field is at play.

We report that the shape and size of fluorescent patterns can be controlled by the focused laser intensity distribution, which depends on irradiation conditions as well as on the spin and orbital angular momenta being carried by light, inducing the formation of silver cluster patterns in a silver-containing zinc phosphate glass. In particular, we demonstrate that sub-diffraction-limited inner structures of fluorescent patterns can be generated by direct laser writing (DLW) with tightly focused femtosecond laser vortex beams as Laguerre-Gauss modes (LG0l) with linear and left-handed circular polarizations. We believe this technique, further combined with dual-color DLW, can be useful and powerful for developing structured light enabled nanostructures.