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Exceedingly strong aeolian dust activity has occurred in inland Asia. Comparisons of the late Cenozoic sedimentation rates between aeolian and fluvial‐lacustrine sequences around the northern Tibetan Plateau suggest that aeolian process has played an important role in the erosion, weathering and deposition of sediment. However, recognizing dust as an important source in fluvial‐lacustrine sequences is a vital but difficult task. Here, clay‐sized mineral and elemental records of regional silicate weathering histories are revisited during the period of Asian dust expansion at ~9–8 Ma. The aeolian dust input from the Tianshan‐Altay Orogens into the Jiuquan Basin is identified using the Th/Sc ratio while that from the Qilian Shan into the Xining Basin is identified based on inconsistent fine‐grained silicate weathering proxies. Our study suggests that the use of appropriate dust provenance tracers and recognition of wind transport‐induced changes in dust grain size and chemistry can provide useful aeolian dust discrimination approaches. [ABSTRACT FROM AUTHOR]

The arid interior of Asia is the largest source of dust deposited in the North Pacific Ocean, and some dust is even transported to Greenland. Investigating the provenance history of Asian dust can provide strong constraints on the evolution of topography and climate in the Asian interior. Eolian dust Nd isotopic records preserved in North Pacific Ocean sediments since ∼40 Ma provide a spatially integrated first-order constraint on the provenance changes of Asian dust. However, a lack of similarly long dust Nd isotopic records from Asian dust source areas, namely, the northern Tibetan Plateau and the Central Asian Orogenic Belt, has hindered a full understanding of Asian dust provenance changes linked to the Cenozoic evolution of tectonics, climate and topography in inland Asia. Here, we have constructed the first fine-grained and whole-rock Nd isotopic records from sediments deposited on the northern Tibetan Plateau since ∼52 Ma. The results indicate two major changes, a gradual increase in ε Nd (0) values between ∼42 Ma and ∼25 Ma and a general decrease since ∼25 Ma, which were probably caused by the incremental northward growth of the Tibetan Plateau. Further mass balance estimates based on comparisons between the Nd isotopic characteristics of dust from the northern Tibetan Plateau and the North Pacific Ocean indicate that a rapid increase in the contribution of the Central Asian Orogenic Belt to Asian dust at ∼25 Ma can be closely linked to rapid exhumation caused by tectonic uplift and aridification in inland Asia. Our provenance analyses, together with the onset of eolian sediment in central and eastern Asia, suggest that a modern-like regime promoting Asian dust emissions and transport might have been in place since the late Oligocene. [ABSTRACT FROM AUTHOR]

The Qaidam Basin, located on the northeastern Tibetan Plateau and containing Cenozoic sediments with a maximum thickness of ~ 12,000 m, is an ideal place to study the phased uplift of the NE Tibetan Plateau and regional climate change. The estimation of the paleosalinity of sedimentary environments not only helps to evaluate the evolution of lakes in this region but offers insights into contemporaneous climate change. We present detailed geochemical and mineralogical investigations from the lacustrine interval of the Hongliugou section in the northern Qaidam Basin to reconstruct salinity fluctuations in the paleolake during the late Eocene era (~ 42.0–35.5 Ma). The clay mineral assemblages mainly contain smectite, illite, chlorite, kaolinite and irregular illite/smectite mixed layers. Clay boron-derived paleosalinity estimates (equivalent boron content, Couch's paleosalimeter and B/Ga ratios) along with other proxies sensitive to salinity changes (e.g., Rb/K ratios and ostracod assemblages) collectively indicate an overall brackish sedimentary environment with a higher-salinity period at approximately 40.0–39.2 Ma. This higher-salinity period indicates a more arid environment and is probably related to global cooling. However, the global cooling in late Eocene cannot explain the overall stable long-term salinity pattern, implying that other factors exist. We propose that the migration of the Yiliping depression depocenter in the northern Qaidam and increased orographic rainfall induced by late Eocene tectonic activity at the northern margin of the basin might have partly offset the increase in salinity driven by global cooling. [ABSTRACT FROM AUTHOR]

[Display omitted] The Indo-Pacific warm pool (IPWP) is crucial for regional and global climates. However, the development of the IPWP and its effect on the regional climate during the Cenozoic remain unclear. Here, using a compilation of sea surface temperature (SST) records (mainly since the middle Miocene) and multimodel paleoclimate simulations, our results indicated that the extent, intensity and warmest temperature position of the IPWP changed markedly during the Cenozoic. Specifically, its extent decreased, its intensity weakened, and its warmest temperature position shifted from the Indian to western Pacific Ocean over time. The atmospheric CO 2 dominated its extent and intensity, while paleogeography, by restricting the distribution of the Indian Ocean and the width of the tropical seaways, controlled the shift in its warmest temperature position. In particular, the eastward shift to the western Pacific Ocean from the middle to late Miocene inferred from compiled SST records likely resulted from the constriction of tropical seaways. Furthermore, by changing the atmospheric thermal structure and atmospheric circulation, the reduced extent and intensity of the IPWP decreased the annual precipitation in the western Indian Ocean, eastern Asia and Australia, while the shift in the warmest temperature position from the Indian to western Pacific Ocean promoted aridification in Australia. Qualitative model-data agreements are obtained for both the IPWP SST and regional climate. From the perspective of past warm climates with high concentrations of atmospheric CO 2 , the expansion and strengthening of the IPWP will occur in a warmer future and favor excessive precipitation in eastern Asia and Australia. [ABSTRACT FROM AUTHOR]

Graphical abstract Highlights • Detailed 15.3–1.8 Ma clay elemental geochemistry records for the northeastern Qaidam Basin are presented. • Long-term and persistent weakening of the chemical weathering intensity has occurred since the Middle Miocene. • Global cooling-related drying played a key role in the chemical weathering intensity. • Miocene uplift of the northern Tibetan Plateau might exert some influence on the weakened chemical weathering intensity at 12–8 Ma. Abstract Cenozoic basin sediments around the Tibetan Plateau are valuable archives that can be used to reveal long-term interactions among tectonics, climate and weathering. However, the reconstruction of silicate weathering histories in this tectonically active region is consistently hindered by the presence of frequently embedded conglomerate and sandstone in the long sedimentary sequences. Here, we present detailed geochemical compositions of the clay components of the sediments in the Huaitoutala section (ca. 15.3–1.8 Ma) of the northeastern Qaidam Basin to reconstruct the chemical weathering history of the catchment since the Middle Miocene. Major element ratio proxies reveal evidence of four stages of change: from ca. 15.3 to 12.6 Ma, in which the clay components are characterized by relatively high Chemical Index of Alteration (CIA) values (75–88, average = 81) but low mobile/immobile oxide ratios (e.g., K 2 O/Al 2 O 3 , Na 2 O/Al 2 O 3 and CaO/Al 2 O 3), thus indicating the occurrence of intense chemical weathering conditions; from ca. 12.6 to 6.6 Ma, in which decreasing CIA values, together with increasing mobile/immobile oxide ratios, suggesting that a long-term decrease in silicate weathering intensity occurred in the source area; from 6.6 to 2.6 Ma, in which the clay components in the sediments exhibit persistently low CIA values (66–81, average = 76.8) and high oxide ratios, which are indicative of mild to moderate chemical weathering; and since 2.6 Ma, in which the CIA values (64–80, average = 75.5) have continued to decrease with increasing oxide ratios, thus reflecting mild chemical weathering conditions. The geochemical proxy records demonstrate that the intensity of chemical weathering has continually decreased and that the Qaidam Basin has experienced continuous aridification since ca. 12.6 Ma. We suggest that Middle-Miocene global cooling-related drying has exerted a significant influence on the trend of decreasing chemical weathering intensity since ca. 12.6 Ma. In addition, the Late Cenozoic rapid uplift and exhumation of the NE Tibetan Plateau could have limited the time that the silicate rocks were exposed in the weathering profile prior to the deposition, which may have led to their weakened intensity of chemical weathering. [ABSTRACT FROM AUTHOR]

[Display omitted] • Paleoecological and paleohydrological changes in the Qaidam Basin occurred during the EOT. • Changes in CPI, ACL, Paq and L/H, indicating bacterial, algal and aquatic plants shrink , and terrestrial plants flourish. • δ2H 31 values were increased by 18.1‰, indicating a decrease in water vapor content and an increasingly arid climate. The Eocene/Oligocene transition (EOT) at ∼34 Ma has been considered the most prominent climatic cooling event in the Cenozoic Era. However, few organic biomarker studies have attempted to reconstruct relevant terrestrial ecological and hydrological responses to an age characterized by drastic temperature changes. This research aims to reconstruct the paleoecological and paleohydrological evolution of the Qaidam Basin (QB) on the northeastern Tibetan Plateau (NE TP) between 40.2 and 29.9 Ma, based on analyses of n -alkane chain length distributions as well as compound-specific hydrogen isotopic compositions (δ2H alk). Research showed the presence of a sequence of pronounced ecological and hydrological variations at 35.0–33.1 Ma, including: 1) a significantly decreased input of bacteria, algae and aquatic plants, allied with a markedly increased input of terrestrial plants, reflected in a significant increase in carbon preference index (CPI) and the average chain length (ACL) ratio, as well as an abrupt decline in the relative ratio of mid- to long-chain length homologue (Paq) values and the ratio of low- to high- molecular-weight n -alkanes (L/H); and 2) drier climatic conditions, reflected in an 18.1‰ increase in δ2H 31 values, as well as more positive hydrogen isotopic precipitation values (δ2H p). These features demonstrate significant paleoecological and paleohydrological changes in the QB in response to the drier and cooler climate during the EOT. [ABSTRACT FROM AUTHOR]

Qaidam Basin is a tectonically controlled Mesozoic–Cenozoic depression on the northern margin of the Tibetan Plateau. A 938.5 m-long core was drilled in the Qahansilatu sub-basin in the western Qaidam Basin, with an average core recovery of 95%. It revealed alternating salt layers and carbonate clay layers. Samples were collected at 10–40 cm intervals for mineralogical analysis by XRD and chemical analysis by ICP-OES. The lower 538.5 m sediments are composed of halite, gypsum, anhydrite, gaylussite, calcite, aragonite, ankerite, dolomite, and an unnamed mineral (Mg0.92Ca0.08CO3·3H2O), with trace eugsterite. The mother brines could be Na-type, Na–Ca-type, Na–Ca–(Mg)-type, Ca–(Na)-type, Ca–(Mg)–(Na)-type, and trace Ca–Mg–(Na). Reflux and bacterial activity could be suitable for the formation of dolomite. Deep burial diagenesis could have played an active role in the formation of ankerite and anhydrate. The continuous presence of halite suggested the paleo-lake water was highly brackish or saline, with high evaporation since 2.77 Ma. Salt layers in the lower 538.5 m-long sediments were present from 2221 ka to 2052 ka, corresponding to Pleistocene salt formation in the Qaidam Basin. As hydrated carbonate minerals, both gaylussite and the unnamed mineral are deposited under high precipitation rates with microbial activity. Gaylussite was deposited from Na–Ca-enriched solutions with molar ratios of Na/Ca more than 2 from 691 m (2226 ka) to 413.6 m (1222 ka). The un-named mineral (Mg0.92Ca0.08CO3·3H2O) was found from 523.4 m (1728 ka) to 724.2 m (2308 ka). Anhydrite could be transformed from gypsum under deep burial from 657.42 m (2052 ka) to 867 m (2556 ka). Alternating salt and clay layers in the lower part of the core recorded arid and relatively wet climatic oscillations and the evolution of brine. As a tectonic sub-basin, tectonic activities could change the local climate during episodes of uplift and subsidence. The dominant minerals in the Chahansilatu sub-basin are similar to those of the other sub-basins in the western Qaidam Basin, but have asynchronous evolutionary stages of brine. [ABSTRACT FROM AUTHOR]