1. Unveil carbon dioxide recycling potential throughout distributor-type membrane reactor.
- Author
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Sato, Yuya, Moździerz, Marcin, Berent, Katarzyna, Brus, Grzegorz, and Nomura, Mikihiro
- Subjects
MEMBRANE reactors ,CARBON dioxide ,GREEN fuels ,COMPUTATIONAL fluid dynamics ,HYDROGEN production ,CARBON offsetting ,GAS mixtures - Abstract
With the cost of green hydrogen production decreasing year by year, methanation, a carbon dioxide hydrogenation reaction, is becoming a more critical technology for the realization of a carbon-neutral society. Here, we show the procedure of membrane preparation for a distributor-type membrane reactor that simultaneously captures and recycles C O 2 together with experimental tests of the proposed reactor design. To decrease the temperature gradient in the reactor and to improve methane recovery from the inlet gas mixture, a three-dimensional computational fluid dynamics simulation of the reactor was conducted. The numerical results suggest that the distributed feed design results in a uniform distribution of carbon dioxide, preventing localized reactions at the reactor inlet. In addition, it reduces the temperature rise in the reactor by up to about 300 K compared to the case where the carbon dioxide and hydrogen gas mixture is fed from a single inlet. The effect of the feed C O 2 concentration on reactivity is also discussed. Simulation results show that the membrane reactor with inlet concentration of about 15 %, such as those emitted from industrial boilers, is capable of recovering methane at concentrations about 1.5 times higher in comparison to 100 % C O 2 concentration at the inlet in a classical reactor. [Display omitted] • The distributor-type reactor advances C O 2 capture and recycling, aiding carbon neutrality. • The proposed reactor design lowers temperature rises by 300 K, enhancing efficiency. • Reactor achieves 1.5 times higher methane recovery, improving C O 2 recycling. [ABSTRACT FROM AUTHOR]
- Published
- 2024
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