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Colossal magnetoresistance (CMR) emerges from intertwined spin and charge degrees of freedom in the form of ferromagnetic clusters also known as trapped magnetic polarons. As a result, CMR is rarely observed in antiferromagnetic materials. Here we use electron spin resonance (ESR) to reveal microscopic evidence for the formation of magnetic polarons in antiferromagnetic Eu$_{5}$In$_{2}$Sb$_{6}$. First, we observe a reduction of the Eu$^{2+}$ ESR linewidth as a function of the applied magnetic field consistent with ferromagnetic clusters that are antiferromagnetically coupled. Additionally, the Eu$^{2+}$ lineshape changes markedly below T' ~ 200 K, a temperature scale that coincides with the onset of CMR. The combination of these two effects provide strong evidence that magnetic polarons grow in size below T' and start influencing the macroscopic properties of the system., 7 pages, 4 figures. Accepted in Phys. Rev. B

CeRhIn5 provides a textbook example of quantum criticality in a heavy fermion system: Pressure suppresses local-moment antiferromagnetic (AFM) order and induces superconductivity in a dome around the associated quantum critical point (QCP) near pc ≈ 23 kbar. Strong magnetic fields also suppress the AFM order at a field-induced QCP at Bc ≈ 50 T. In its vicinity, a nematic phase at B* ≈ 28 T characterized by a large in-plane resistivity anisotropy emerges. Here, we directly investigate the interrelation between these phenomena via magnetoresistivity measurements under high pressure. As pressure increases, the nematic transition shifts to higher fields, until it vanishes just below p. While pressure suppresses magnetic order in zero field as pc is approached, we find magnetism to strengthen under strong magnetic fields due to suppression of the Kondo effect. We reveal a strongly nonmean-field-like phase diagram, much richer than the common local-moment description of CeRhIn would suggest.

Kondo insulators are predicted to undergo an insulator-to-metal transition under applied magnetic field, yet the extremely high fields required to date have prohibited a comprehensive investigation of the nature of this transition. Here we show that Ce3Bi4Pd3 provides an ideal platform for this investigation, owing to the unusually small magnetic field of B ~ 11 T required to overcome its Kondo insulating gap. Above Bc, we find a magnetic field-induced Fermi liquid state whose characteristic energy scale T_FL collapses near Bc in a manner indicative of a magnetic field-tuned quantum critical point. A direct connection is established with the process of Kondo singlet formation, which yields a broad maximum in the magnetic susceptibility as a function of temperature in weak magnetic fields that evolves progressively into a sharper transition at Bc as T -> 0., 10 pages including 10 figures

We present nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements performed on single crystalline \ccag{}, a member of a recently discovered family of heavy fermion materials Ce$_2M$Al$_7$Ge$_4$ ($M$ = Co, Ir, Ni, or Pd). Previous measurements indicated a strong Kondo interaction as well as magnetic order below $T_M = 1.8$ K. Our NMR spectral measurements show that the Knight shift $K$ is proportional to the bulk magnetic susceptibility $\chi$ at high temperatures. A clear Knight shift anomaly ($K \not\propto \chi$) is observed at coherence temperatures $T^* \sim 17.5$ K for $H_0 \parallel \hat{c}$ and 10 K for $H_0 \parallel \hat{a}$ at the ${}^{59}$Co site, and $T^* \sim 12.5$ K at the ${}^{27}$Al(3) site for $H_0 \parallel \hat{a}$ characteristic of the heavy fermion nature of this compound. At high temperatures the ${}^{59}$Co NMR spin-lattice relaxation rate $T_1^{-1}$ is dominated by spin fluctuations of the 4$f$ local moments with a weak metallic background. The spin fluctuations probed by ${}^{59}$Co NMR are anisotropic and larger in the basal plane than in the $c$ direction. Furthermore, we find $(T_1TK)^{-1} \propto T^{-1/2}$ at the ${}^{59}$Co site as expected for a Kondo system for $T > T^*$ and $T> T_K$. ${}^{59}$Co NQR \slrr{} measurements at low temperatures indicate slowing down of spin fluctuations above the magnetic ordering temperature $T_M \sim 1.8$ K. A weak ferromagnetic character of fluctuations around $\mathbf{q}=0$ is evidenced by an increase of $\chi T$ versus $T$ above the magnetic ordering temperature. We also find good agreement between the observed and calculated electric field gradients at all observed sites.

The effects of uniaxial compressive stress on the normal state $^{17}$O nuclear magnetic resonance properties of the unconventional superconductor Sr$_{2}$RuO$_{4}$ are reported. The paramagnetic shifts of both planar and apical oxygen sites show pronounced anomalies near the nominal $\mathbf{a}$-axis strain $\varepsilon_{aa}\equiv\varepsilon_v$, that maximizes the superconducting transition temperature, $T_{c}$. The spin susceptibility weakly increases on lowering the temperature below $T$$\simeq$10 K, consistent with an enhanced density of states associated with passing the Fermi energy through a van Hove singularity. Although such a Lifshitz transition occurs in the $\gamma$ band, formed by the Ru $d_{xy}$ states hybridized with in-plane O $p_{\pi}$ orbitals, the large Hund's coupling renormalizes the uniform spin susceptibilty, which, in turn, affects the hyperfine fields of all nuclei. We estimate this \textquotedblleft Stoner\textquotedblright\ renormalization, $S,$ by combining the data with first-principles calculations and conclude that this is an important part of the strain effect, with implications for superconductivity., Comment: 15 pages, 9+6 figures, 0+1 table

CeCo(In0.990Hg0.010)(5) is a charge doped variant of the d-wave CoCoIn5 superconductor with coexistent antiferromagnetic and superconducting transitions occurring at T-N = 3.4 and T-c = 1.4 K, respectively. We use neutron diffraction and spectroscopy to show that the magnetic resonant fluctuations present in the parent superconducting phase are replaced by collinear c-axis magnetic order with three-dimensional Ising critical fluctuations. No low-energy transverse spin fluctuations are observable in this doping-induced antiferromagnetic phase and the dynamic resonant spectral weight predominately shifts to the elastic channel. Static (tau > 0.2 ns) collinear Ising order is proximate to superconductivity in CeCoIn5 and is stabilized through hole doping with Hg.

SmB6 is a candidate topological Kondo insulator that displays surface conduction at low temperatures. Here, we perform torque magnetization measurements as a means to detect de Haas-van Alphen (dHvA) oscillations in SmB6 crystals grown by aluminum flux. We find that dHvA oscillations occur in single crystals containing embedded aluminum, originating from the flux used to synthesize SmB6. Measurements on a sample with multiple, unconnected aluminum inclusions show that aluminum crystallizes in a preferred orientation within the SmB6 cubic lattice. The presence of aluminum is confirmed through bulk susceptibility measurements, but does not show a signature in transport measurements.

We present nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements performed on single crystalline \ccag{}, a member of a recently discovered family of heavy fermion materials Ce$_2M$Al$_7$Ge$_4$ ($M$ = Co, Ir, Ni, or Pd). Previous measurements indicated a strong Kondo interaction as well as magnetic order below $T_M = 1.8$ K. Our NMR spectral measurements show that the Knight shift $K$ is proportional to the bulk magnetic susceptibility $��$ at high temperatures. A clear Knight shift anomaly ($K \not\propto ��$) is observed at coherence temperatures $T^* \sim 17.5$ K for $H_0 \parallel \hat{c}$ and 10 K for $H_0 \parallel \hat{a}$ at the ${}^{59}$Co site, and $T^* \sim 12.5$ K at the ${}^{27}$Al(3) site for $H_0 \parallel \hat{a}$ characteristic of the heavy fermion nature of this compound. At high temperatures the ${}^{59}$Co NMR spin-lattice relaxation rate $T_1^{-1}$ is dominated by spin fluctuations of the 4$f$ local moments with a weak metallic background. The spin fluctuations probed by ${}^{59}$Co NMR are anisotropic and larger in the basal plane than in the $c$ direction. Furthermore, we find $(T_1TK)^{-1} \propto T^{-1/2}$ at the ${}^{59}$Co site as expected for a Kondo system for $T > T^*$ and $T> T_K$. ${}^{59}$Co NQR \slrr{} measurements at low temperatures indicate slowing down of spin fluctuations above the magnetic ordering temperature $T_M \sim 1.8$ K. A weak ferromagnetic character of fluctuations around $\mathbf{q}=0$ is evidenced by an increase of $��T$ versus $T$ above the magnetic ordering temperature. We also find good agreement between the observed and calculated electric field gradients at all observed sites.

Quantum critical points (QCPs) are widely accepted as a source of a diverse set of collective quantum phases of matter. A central question is how the order parameters of phases near a QCP interact and determine the fundamental character of the critical dynamics which drive the quantum critical behavior. One of the most interesting proposals for the quantum critical behavior that occurs in correlated electron systems is that the behavior may arise from local, as opposed to long wavelength, critical fluctuations of the order parameter. The local criticality is believed to give rise to energy over temperature ($E/T$) scaling of the dynamic susceptibility with a fractional exponent near the quantum critical point (QCP). Here we show that $E/T$ scaling is indeed observed for CeCu$_{6-x}$Ag$_x$ but on closer inspection, the fluctuations can be separated into two components, implying that multiple order parameters play an important role in the unconventional critical behavior. Additionally, when the fluctuations corresponding to the magnetically ordered side of the phase diagram are separated, they are found to be three dimensional and to obey the scaling behavior expected for long wavelength fluctuations near an itinerant antiferromagnetic QCP., 12 pages, 11 figures

Applied pressure drives the heavy-fermion antiferromagnet CeRhIn$_{5}$ towards a quantum critical point that becomes hidden by a dome of unconventional superconductivity. Magnetic fields suppress this superconducting dome, unveiling the quantum phase transition of local character. Here, we show that $5\%$ magnetic substitution at the Ce site in CeRhIn$_{5}$, either by Nd or Gd, induces a zero-field magnetic instability inside the superconducting state. This magnetic state not only should have a different ordering vector than the high-field local-moment magnetic state, but it also competes with the latter, suggesting that a spin-density-wave phase is stabilized in zero field by Nd and Gd impurities - similarly to the case of Ce$_{0.95}$Nd$_{0.05}$CoIn$_{5}$. Supported by model calculations, we attribute this spin-density wave instability to a magnetic-impurity driven condensation of the spin excitons that form inside the unconventional superconducting state.

© 2015 IOP Publishing Ltd. Electric resistivity, specific heat, magnetic susceptibility, and inelastic neutron scattering experiments were performed on a single crystal of the heavy fermion compound Ce(Ni0.935Pd0.065)2Ge2in order to study the spin fluctuations near an antiferromagnetic (AF) quantum critical point (QCP). The resistivity and the specific heat coefficient for T ≤ 1K exhibit the power law behavior expected for a 3D itinerant AF QCP (ρ(T) ∼ T3/2and γ(T) ∼ γ0- bT1/2). However, for 2 ≤ T ≤ 10 K, the susceptibility and specific heat vary as logT and the resistivity varies linearly with temperature. Furthermore, despite the fact that the resistivity and specific heat exhibit the non-Fermi liquid behavior expected at a QCP, the correlation length, correlation time, and staggered susceptibility of the spin fluctuations remain finite at low temperature. We suggest that these deviations from the divergent behavior expected for a QCP may result from alloy disorder.

The easily tuned balance among competing interactions in Kondo-lattice metals allows access to a zero-temperature, continuous transition between magnetically ordered and disordered phases, a quantum-critical point (QCP). Indeed, these highly correlated electron materials are prototypes for discovering and exploring quantum-critical states. Theoretical models proposed to account for the strange thermodynamic and electrical transport properties that emerge around the QCP of a Kondo lattice assume the presence of an indefinitely large number of itinerant charge carriers. Here, we report a systematic transport and thermodynamic investigation of the Kondo-lattice system CeNi$_{2-��}$As$_2$ ($��$$\thickapprox$0.28) as its antiferromagnetic order is tuned by pressure and magnetic field to zero-temperature boundaries. These experiments show that the very small but finite carrier density of $\sim$0.032 $e^-$/f.u. in CeNi$_{2-��}$As$_2$ leads to unexpected transport signatures of quantum criticality and the delayed development of a fully coherent Kondo lattice state with decreasing temperature. The small carrier density and associated semi-metallicity of this Kondo-lattice material favor an unconventional, local-moment type of quantum criticality and raise the specter of Nozi��res exhaustion idea that an insufficient number of conduction-electron spins to separately screen local moments requires collective Kondo screening., 15+7 pages, 4+5 figures in Proc. Natl. Acad. Sci. USA (2015)

We report the phase diagram of the doping series U_2Pt_xRh_(1-x)C_2, studied through measurements of resistivity, specific heat and magnetic susceptibility. The Neel temperature of U_2RhC_2 of ~ 22 K is suppressed with increasing Pt content, reaching zero temperature close to x=0.7, where we observed signatures of increased quantum fluctuations. In addition, evidence is presented that the antiferromagnetic state undergoes a spin-reorientation transition upon application of an applied magnetic field. This transition shows non-monotonic behaviour as a function of x, peaking at around x=0.3. Superconductivity is observed for x>=0.9, with T_c increasing with increasing x. The reduction in T_c and increase in residual resistivity with decreasing Pt content is inconsistent with the extension of the Abrikosov-Gor'kov theory to unconventional superconductivity., 7 pages, 9 figures

Nuclear magnetic resonance (NMR) measurements on the $^{195}$Pt nucleus in an aligned powder of the moderately heavy-fermion material U2PtC2 are consistent with spin-triplet pairing in its superconducting state. Across the superconducting transition temperature and to much lower temperatures, the NMR Knight shift is temperature independent for field both parallel and perpendicular to the tetragonal c-axis, expected for triplet equal-spin pairing superconductivity. The NMR spin-lattice relaxation rate 1/T$_1$, in the normal state, exhibits characteristics of ferromagnetic fluctuations, compatible with an enhanced Wilson ratio. In the superconducting state, 1/T$_1$ follows a power law with temperature without a coherence peak giving additional support that U$_2$PtC$_2$ is an unconventional superconductor. Bulk measurements of the AC-susceptibility and resistivity indicate that the upper critical field exceeds the Pauli limiting field for spin-singlet pairing and is near the orbital limiting field, an additional indication for spin-triplet pairing.

We report the pressure response of charge-density-wave (CDW) and ferromagnetic (FM) phases of the rare-earth intermetallic SmNiC2 up to 5.5 GPa. The CDW transition temperature (T_{CDW}), which is reflected as a sharp inflection in the electrical resistivity, is almost independent of pressure up to 2.18 GPa but is strongly enhanced at higher pressures, increasing from 155.7 K at 2.2 GPa to 279.3 K at 5.5 GPa. Commensurate with the sharp increase in T_{CDW}, the first-order FM phase transition, which decreases with applied pressure, bifurcates into the upper (T_{M1}) and lower (T_c) phase transitions and the lower transition changes its nature to second order above 2.18 GPa. Enhancement both in the residual resistivity and the Fermi-liquid T^2 coefficient A near 3.8 GPa suggests abundant magnetic quantum fluctuations that arise from the possible presence of a FM quantum critical point., 5 pages, 5 figures

We have carried out a comprehensive study of the UCo1-xFexGe series across the entire range of compositions 0, 7 pages, 7 figures

We report extensive measurements on a new compound (Yb0.24Sn0.76)Ru that crystallizes in the cubic CsCl structure. Valence band photoemission and L3 x-ray absorption show no divalent component in the 4f configuration of Yb. Inelastic neutron scattering (INS) indicates that the eight-fold degenerate J-multiplet of Yb3+ is split by the crystalline electric field (CEF) into a {\Gamma}7 doublet ground state and a {\Gamma}8 quartet at an excitation energy 20 meV. The magnetic susceptibility can be fit very well by this CEF scheme under the assumption that a {\Gamma}6 excited state resides at 32 meV; however, the {\Gamma}8/{\Gamma}6 transition expected at 12 meV was not observed in the INS. The resistivity follows a Bloch- Gr\"uneisen law shunted by a parallel resistor, as is typical of systems subject to phonon scattering with no apparent magnetic scattering. All of these properties can be understood as representing simple local moment behavior of the trivalent Yb ion. At 1 K, there is a peak in specific heat that is too broad to represent a magnetic phase transition, consistent with absence of magnetic reflections in neutron diffraction. On the other hand, this peak also is too narrow to represent the Kondo effect in the {\Gamma}7 ground state doublet. On the basis of the field-dependence of the specific heat, we argue that antiferromagnetic shortrange order (possibly co-existing with Kondo physics) occurs at low temperatures. The long-range magnetic order is suppressed because the Yb site occupancy is below the percolation threshold for this disordered compound.

We investigated the effect of electron and hole doping on the high-field low-temperature superconducting state in CeCoIn5by measuring specific heat of CeCo (In1-xMx) 5 with M=Sn, Cd, and Hg and x up to 0.33% at temperatures down to 0.1 K and fields up to 14 T. Although both Cd and Hg doping (hole doping) suppresses the zero-field Tcmonotonically, Hc2increases with small amounts of doping and has a maximum around x=0.2% (M=Cd). On the other hand, with Sn doping (electron doping) both zero-field Tcand Hc2decrease monotonically. The critical temperature for the high-field low-temperature superconducting state correlates with Hc2and Tc, which we interpret in support of the superconducting origin of this state. © 2010 The American Physical Society.

We report results of $^{59}$Co nuclear magnetic resonance measurements on a single crystal of superconducting PuCoGa5 in its normal state. The nuclear spin-lattice relaxation rates and the Knight shifts as a function of temperature reveal an anisotropy of spin fluctuations with finite wave vector q. By comparison with the isostructural members, we conclude that antiferromagnetic XY-type anisotropy of spin fluctuations plays an important role in mediating superconductivity in these heavy fermion materials., Published in Phys. Rev. Lett

We investigated the effect of electron and hole doping on the high-field low-temperature superconducting state in CeCoIn$_5$ by measuring specific heat of CeCo(In$_{\rm 1-x}$M$_{\rm x}$)$_5$ with M=Sn, Cd and Hg and $x$ up to 0.33% at temperatures down to 0.1\,K and fields up to 14\,T. Although both Cd- and Hg-doping (hole-doping) suppresses the zero-field $T_c$ monotonically, $H_{c2}$ increases with small amounts of doping and has a maximum around $x$=0.2% (M=Cd). On the other hand, with Sn-doping (electron-doping) both zero-field $T_c$ and $H_{c2}$ decrease monotonically. The critical temperature for the high-field low-temperature superconducting state (so called {\it Q}-state) correlates with $H_{c2}$ and $T_c$, which we interpret in support of the superconducting origin of this state., Phys. Rev. B 82, 220502(R) (2010)

Magnetic susceptibility results for single crystals of the new cubic compounds UT$_2$Al$_{20}$ (T=Mn, V, and Mo) are reported. Magnetization, specific heat, resistivity, and neutron diffraction results for a single crystal and neutron diffraction and inelastic spectra for a powder sample are reported for UMn$_2$Al$_{20}$. For T = V and Mo, temperature independent Pauli paramagnetism is observed. For UMn$_2$Al$_{20}$, a ferromagnetic transition is observed in the magnetic susceptibility at $T_c$ = 20 K. The specific heat anomaly at $T_c$ is very weak while no anomaly in the resistivity is seen at $T_c$. We discuss two possible origins for this behavior of UMn$_2$Al$_{20}$: moderately small moment itinerant ferromagnetism, or induced local moment ferromagnetism., 5 pages, 5 figures, to be published in Phys. rev. B

When subjected to pressure, the prototypical heavy-fermion antiferromagnet CeRhIn5 becomes superconducting, forming a broad dome of superconductivity centered around 2.35 GPa (=P2) with maximal Tc of 2.3 K. Above the superconducting dome, the normal state shows strange metallic behaviours, including a divergence in the specific heat and a sub-T-linear electrical resistivity. The discovery of a field-induced magnetic phase that coexists with superconductivity for a range of pressures P < P2 has been interpreted as evidence for a quantum phase transition, which could explain the non-Fermi liquid behavior observed in the normal state. Here we report electrical resistivity measurements of CeRhIn5 under magnetic field at P2, where the resistivity is sub-T-linear for temperatures above Tc (or T_FL) and a T^2-coefficient A found below T_FL diverges as Hc2 is approached. These results are similar to the field-induced quantum critical compound CeCoIn5 and confirm the presence of a quantum critical point in the pressure-induced superconductor CeRhIn5., 7 pages, 3 figures

We show using neutron diffraction that the magnetic structure of CeRhIn4.85 Hg0.15 is characterized by a commensurate propagation vector (1/2,1/2,1/2). This is different from the magnetic structure in the parent compound CeRhIn5, which orders with an incommensurate propagation vector (1/2,1/2,0.297). The special relation between the commensurate magnetic mode and unconventional superconductivity has been shown previously for this class of heavy fermion superconductors. This work provides further evidence for the ubiquity of this antiferromagnetic mode. © 2009 The American Physical Society.

We report quantum oscillation measurements on CaFe2As2 under strong magnetic fields- recently reported to become superconducting under pressures of as little as a kilobar. The largest observed carrier pocket occupies less than 0.05 % of the paramagnetic Brillouin zone volume- consistent with Fermi surface reconstruction caused by antiferromagnetism. On comparing several alkali earth AFe2As2 antiferromagnets (with A=Ca,Sr and Ba), the dependence of both the Fermi surface cross-sectional area F_alpha and the effective mass m*_alpha of the primary observed pocket on the antiferromagnetic/structural transition temperature T_s is found to be consistent with quasiparticles in a conventional spin-density wave model. These findings suggest that a conventional spin-density wave exists within close proximity to superconductivity in this series of compounds, which may have implications for the microscopic origin of unconventional pair formation., 4 pages with 5 figures

The physical properties of CeM (In1 - xHgx)5(M = Rh, Ir) including specific heat and magnetic susceptibility are reported. Two magnetic phases exist in CeRhIn (In1 - xHgx)5with some evidence of a change from incommensurate magnetic order to a commensurate structure near 10% nominal Hg substitution. In CeIr (In1 - xHgx)5, an antiferromagnetic quantum critical point near x = 3 % (followed by robust long-range antiferromagnetism for x > 5 %) appears to be separated from superconductivity in CeIrIn5. The multitude of magnetic ground states observed in the CeM (In1 - xHgx)5materials is quite sensitive to doping and magnetic fields. © 2007.

The antiferromagnet CaFe$_2$As$_2$ does not become superconducting when subject to ideal hydrostatic pressure conditions, where crystallographic and magnetic states also are well defined. By measuring electrical resistivity and magnetic susceptibility under quasi-hydrostatic pressure, however, we find that a substantial volume fraction of the sample is superconducting in a narrow pressure range where collapsed tetragonal and orthorhombic structures coexist. At higher pressures, the collapsed tetragonal structure is stabilized, with the boundary between this structure and the phase of coexisting structures strongly dependent on pressure history. Fluctuations in magnetic degrees of freedom in the phase of coexisting structures appear to be important for superconductivity., Comment: revised (6 pages, 5 figures) - includes additional experimental results

We report an $^{75}$As NMR study of BaFe$_2$As$_2$ in both single crystals and polycrystal forms. We find that Sn impurities in the single crystal dramatically alter the low energy spin fluctuations and suppress the ordering temperature from 138 K to 85 K. In contrast to Sn-free samples, we find that the temperature dependence of the $^{75}$As NMR spectra and spin lattice relaxation rates reveal a second order phase transition to a state of incommensurate magnetic order., Comment: 4 pages, 4 figures ; extensive and significant changes have been made to the previous version, focusing on the effect of impurities on the intrinsic physics

To elucidate the nature of the single-particle excitations in the undoped parent cuprates, we have performed a detailed study of Ca2CuO2Cl2 using photoemission spectroscopy. The photoemission lineshapes of the lower Hubbard band are found to be well-described by a polaron model. By comparing the lineshape and temperature dependence of the lower Hubbard band with additional O 2p and Ca 3p states, we conclude that the dominant broadening mechanism arises from the interaction between the photohole and the lattice. The strength of this interaction was observed to be strongly anisotropic and may have important implications for the momentum dependence of the first doped hole states.

We present specific heat and susceptibility data on Sm(La,Sr)CuO4 in magnetic fields up to 9 T and temperatures down to 100 mK. We find a broad peak in specific heat which is insensitive to magnetic field at a temperature of 1.5 K with a value of 2.65 J/mol K. The magnetic susceptibility at 5 T continues to increase down to 2 K, the lowest temperature measured. The data suggest that the Sm spin system may be an ideal realization of the frustrated Heisenberg antiferromagnet on the square lattice., 2 pages, 2 figures, submitted to ICM

We measured specific heat and resistivity of heavy fermion CeCoIn5 at and above the superconducting critical field with field in [001] (Hc2 = 5 T) and [100] directions (Hc2 = 12 T), and at temperatures down to 50 mK. At the critical fields the data show Non Fermi Liquid (NFL) behavior down to the lowest temperatures. With increasing field the data exhibit crossover from NFL to Fermi liquid behavior at the lowest temperatures. Analysis of the scaling properties of the specific heat, and comparison of both resistivity and the specific heat with the predictions of a spinfluctuation theory suggest that the NFL behavior is due to incipient antiferromagnetism (AF) in CeCoIn5, with the quantum critical point in the vicinity of Hc2. Below Hc2 the AF phase which competes with the paramagnetic ground state is superseded by the superconducting transition. To separate the quantum critical point HQCP from the superconducting critical field Hc2 we performed a series of Sn-doping and hydrostatic pressure studies. Sn-doping appears not to be able to separate HQCP and Hc2. Preliminary resistivity in magnetic field measurements under hydrostatic pressure indicate that the QCP point moves inside the superconducting phase in the H-P plane with increasing field.

Thermal conductivity of Sr3Ru2O7 was measured down to 40 mK and at magnetic fields through the quantum critical endpoint at H_c = 7.85 T. A peak in the electrical resistivity as a function of field was mimicked by the thermal resistivity. In the limit as T -> 0 K we find that the Wiedemann-Franz law is satisfied to within 5% at all fields, implying that there is no breakdown of the electron despite the destruction of the Fermi liquid state at quantum criticality. A significant change in disorder (from $\rho_0$(H=0T) = 2.1 $\mu\Omega$ cm to 0.5 $\mu\Omega$ cm) does not influence our conclusions. At finite temperatures, the temperature dependence of the Lorenz number is consistent with ferromagnetic fluctuations causing the non-Fermi liquid behavior as one would expect at a metamagnetic quantum critical endpoint., Comment: 4 figures, published in PRL

Low temperature heat transport was used to investigate the ground state of high-purity single crystals of the lightly-doped cuprate YBa$_{2}$Cu$_{3}$O$_{6.33}$. Samples were measured on either side of the superconducting phase boundary, in both zero and applied magnetic field. We report the observation of delocalized fermionic excitations at zero energy in the non-superconducting state, which shows that the ground state of underdoped cuprates is metallic. Its low-energy spectrum appears to be similar to that of the d-wave superconductor, i.e. nodal. The insulating ground state observed in underdoped La$_{2-x}$Sr$_{x}$CuO$_4$ is attributed to the competing spin-density-wave order present in that system., 4 pages, 3 figures; published in Physical Review Letters

We present the results of out-of-plane electrical transport measurements on the heavy fermion superconductor CeCoIn$_{5}$ at temperatures from 40 mK to 400 K and in magnetic field up to 9 T. For $T $ B$_{c2}$ restores Fermi-liquid behavior in $\rho_{c}(T)$ at $T$ less than 130 mK. Analysis of the $T{^2}$ resistivity coefficient's field-dependence suggests that the QCP in CeCoIn$_{5}$ is located \emph{below} the upper critical field, inside the superconducting phase. These data indicate that while high-$T$ c-axis transport of CeCoIn$_{5}$ exhibits features typical for a heavy fermion system, low-$T$ transport is governed both by spin fluctuations associated with the QCP and Kondo interactions that are influenced by the underlying complex electronic structure intrinsic to the anisotropic CeCoIn$_{5}$ crystal structure.

Thermal transport in the T -> 0 limit was measured as a function of doping in high-quality single crystals of the cuprate superconductor YBa_2Cu_3O_y. The residual linear term kappa_0/T is found to decrease as one moves from the overdoped regime towards the Mott insulator region of the phase diagram. The doping dependence of the low-energy quasiparticle gap extracted from kappa_0/T is seen to scale closely with that of the pseudogap, arguing against a non-superconducting origin for the pseudogap. The presence of a linear term for all dopings is evidence against the existence of a quantum phase transition to an order parameter with a complex (ix) component., 2 pages, 2 figures, submitted to M2S-Rio 2003 Proceedings

We present angle resolved photoemission (ARPES) data on Na-doped Ca$_2$CuO$_2$Cl$_2$. We demonstrate that the chemical potential shifts upon doping the system across the insulator to metal transition. The resulting low energy spectra reveal a gap structure which appears to deviate from the canonical $d_{x2-y2} ~ |cos(k_x a)-cos(k_y a)|$ form. To reconcile the measured gap structure with d-wave superconductivity one can understand the data in terms of two gaps, a very small one contributing to the nodal region and a very large one dominating the anti-nodal region. The latter is a result of the electronic structure observed in the undoped antiferromagnetic insulator. Furthermore, the low energy electronic structure of the metallic sample contains a two component structure in the nodal direction, and a change in velocity of the dispersion in the nodal direction at roughly 50 meV. We discuss these results in connection with photoemission data on other cuprate systems., Comment: 10 pages, 12 figures, accepted by PRB; a high quality pdf is available at http://helios.physics.utoronto.ca/~fronning/RonningNaCCOCResub.pdf (2.2MB)

We present an angle resolved photoemission (ARPES) doping dependence study of the n-type cuprate superconductor Nd_2-xCe_xCuO_4, from the half-filled Mott-insulator to the T_c=24K superconductor. In Nd2CuO4, we reveal the charge-transfer band (CTB) for the first time. As electrons are doped into the system, this feature's intensity decreases with the concomitant formation of near-E_F spectral weight. At low doping, the Fermi surface is an electron-pocket (with volume ~ x) centered at (pi,0). Further doping leads to the creation of a new hole-like Fermi surface (volume ~ 1+x) centered at (pi,pi). These findings shed light on the Mott gap, its doping evolution, as well as the anomalous transport properties of the n-type cuprates., Comment: Submitted Phys. Rev. Lett. - Nov. 20, 2001

Using methods made possible by recent advances in photoemission technology, we perform an indepth line-shape analysis of the angle-resolved photoemission spectra of the electron doped (n-type) cuprate superconductor Nd_1.85Ce_0.15CuO_4. Unlike for the p-type materials, we only observe weak mass renormalizations near 50-70 meV. This may be indicative of smaller electron-phonon coupling or due to the masking effects of other interactions that make the electron-phonon coupling harder to detect. This latter scenario may suggest limitations of the spectral function analysis in extracting electronic self-energies when some of the interactions are highly momentum dependent., Comment: 8 pages, 5 figures

The low-energy electronic structure of the trilayer cuprate superconductor Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+\delta}$ near optimal doping is investigated by angle-resolved photoemission spectroscopy. The normal state quasiparticle dispersion and Fermi surface, and the superconducting d-wave gap and coherence peak are observed and compared with those of single and bilayer systems. We find that both the superconducting gap magnitude and the relative coherence-peak intensity scale linearly with $T_c$ for various optimally doped materials. This suggests that the higher $T_c$ of the trilayer system should be attributed to parameters that simultaneously enhance phase stiffness and pairing strength., Comment: 5 pages, 5 figres

We have addressed the possibility of surface ferromagnetism in Sr2RuO4 by investigating its surface electronic states by angle-resolved photoemission spectroscopy (ARPES). By cleaving samples under different conditions and using various photon energies, we have isolated the surface from the bulk states. A comparison with band structure calculations indicates that the ARPES data are most readily explained by a nonmagnetic surface reconstruction., 4 pages, 4 figures, RevTex, submitted to Phys. Rev. B

We report a high-resolution angle-resolved photoemission spectroscopic (ARPES) study of the electron-doped (n-type) cuprate superconductor Nd_1.85Ce_0.15CuO_4. We observe regions along the Fermi surface where the near-E_F intensity is suppressed and the spectral features are broad in a manner reminiscent of the high-energy ``pseudogap'' in the underdoped p-type (hole doped) cuprates. However, instead of occurring near the (pi, 0) region, as in the p-type materials, this pseudogap falls near the intersection of the underlying Fermi surface with the antiferromagnetic Brillouin zone boundary., Comment: 5 pages, 3 figures, RevTex, submitted Phys. Rev. Lett. December 21, 2000

Based on angle resolved photoemission spectra measured on different systems at different dopings, momenta and photon energies, we show that the anomalously large spectral linewidth in the $(��,0)$ region of optimal doped and underdoped Bi$_2$Sr$_2$CaCu$_2$O$_{8+��}$ has significant contributions from the bilayer splitting, and that the scattering rate in this region is considerably smaller than previously estimated. This new picture of the electronic excitation near $(��,0)$ puts additional experimental constraints on various microscopic theories and data analysis., 5 pages, 4 figures

The low-energy electronic structure of the trilayer cuprate superconductor Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+��}$ near optimal doping is investigated by angle-resolved photoemission spectroscopy. The normal state quasiparticle dispersion and Fermi surface, and the superconducting d-wave gap and coherence peak are observed and compared with those of single and bilayer systems. We find that both the superconducting gap magnitude and the relative coherence-peak intensity scale linearly with $T_c$ for various optimally doped materials. This suggests that the higher $T_c$ of the trilayer system should be attributed to parameters that simultaneously enhance phase stiffness and pairing strength., 5 pages, 5 figres

We investigated the low-energy electronic structure of Sr2RuO4 by angle-resolved photoemission spectroscopy (ARPES) focusing, in particular, on the controversial issues of the Fermi surface (FS) topology and of the extended van Hove singularity (evHs). A detailed study of temperature and photon energy dependence demonstrates the surface-state nature of the electronic band responsible for the evHs, and may suggest the presence of ferromagnetic correlations at the surface. In addition, we detected a replica of the primary FS that indicates a (sqrt2 x sqrt2) surface reconstruction, as confirmed by LEED. In light of these findings, the FS determined by ARPES is consistent with LDA and de Haas-van Alphen (dHvA) results, and it provides additional information on the detailed shape of the alpha, beta and gamma sheets. Also, at this stage, because of the strong sensitivity of the cleaved surface, we could not find any robust signature of the crossover from 2D to 3D Fermi liquid behavior in our ARPES measurements for T, 6 pages, 5 figures, to appear on J. Electron Spectr. Relat. Phenom

We have performed angle resolved photoelectron spectroscopy on the electron doped cuprate superconductor Nd$_{1.85}$Ce$_{0.15}$CuO$_4$. A comparison of the leading edge midpoints between the superconducting and normal states reveals a small, but finite shift of 1.5-2 meV near the ($\pi$,0) position, but no observable shift along the zone diagonal near ($\pi$/2,$\pi$/2). This is interpreted as evidence for an anisotropic superconducting gap in the electron doped materials, which is consistent with the presence of d-wave superconducting order in this cuprate superconductor., Comment: 5 pages, 4 figures, RevTex, to be published in Phys. Rev. Lett

We have investigated the lowest binding-energy electronic structure of the model cuprate Sr_2CuO_2Cl_2 using angle resolved photoemission spectroscopy (ARPES). Our data from about 80 cleavages of Sr_2CuO_2Cl_2 single crystals give a comprehensive, self-consistent picture of the nature of the first electron-removal state in this model undoped CuO_2-plane cuprate. Firstly, we show a strong dependence on the polarization of the excitation light which is understandable in the context of the matrix element governing the photoemission process, which gives a state with the symmetry of a Zhang-Rice singlet. Secondly, the strong, oscillatory dependence of the intensity of the Zhang-Rice singlet on the exciting photon-energy is shown to be consistent with interference effects connected with the periodicity of the crystal structure in the crystallographic c-direction. Thirdly, we measured the dispersion of the first electron-removal states along G->(pi,pi) and G->(pi,0), the latter being controversial in the literature, and have shown that the data are best fitted using an extended t-J-model, and extract the relevant model parameters. An analysis of the spectral weight of the first ionization states for different excitation energies within the approach used by Leung et al. (Phys. Rev. B56, 6320 (1997)) results in a strongly photon-energy dependent ratio between the coherent and incoherent spectral weight. The possible reasons for this observation and its physical implications are discussed., 10 pages, 8 figures

The Fermi surface of the Bi2212 system is systematically studied using a variety of photon energies. In addition to reconciling the conflicting reports on the Fermi surface of this important material, we identify almost perfectly nested Fermi surface segments parallel to the $(1,0)$ or $(0,1)$ direction. This general yet long overlooked feature of the Fermi surface is intriguingly similar to the Fermi surface of the $La_{1.48}Nd_{0.4}Sr_{0.12}CuO_4$ system., PDF file, 5 pages, 3 figures, submitted to Phys. Rev. Lett, need Acrobat Reader 3.0+ to open

The transport of heat and charge in cuprates was measured in undoped and heavily-underdoped single crystal La_{2-x}Sr_xCuO_{4+delta} (LSCO). In underdoped LSCO, the thermal conductivity is found to decrease with increasing magnetic field in the T --> 0 limit, in striking contrast to the increase observed in all superconductors, including cuprates at higher doping. The suppression of superconductivity with magnetic field shows that a novel thermal metal-to-insulator transition occurs upon going from the superconducting state to the field-induced normal state., 2 pages, 2 figures, submitted to M2S-Rio 2003 Proceedings

We report Shubnikov-de Haas oscillation measurements within the high magnetic field (μ0H>39 T) magnetically polarized regime of URu2Si2, made possible using mesoscopic samples prepared by means of focused ion beam lithography. A significant change in the Fermi surface topology relative to the “hidden-order” phase is observed, signaling a transformation into a high magnetic field regime in which 5f-electrons are removed from the Fermi surface. URu2Si2 is therefore a rare example of an actinide compound in which a transformation of 5f-electrons can be directly observed at low temperatures, setting the stage for the unconventional ordering and high magnetic field quantum criticality in this material.