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Spin-orbit torques (SOTs) act as efficient drivers for nanoscale magnetic systems, such as in magnetic tunnel junctions, nano-oscillators and racetrack geometries. In particular, in combination with materials exhibiting high Dzyaloshinskii--Moriya interaction, SOTs are considered to result in well-controlled deterministic magnetisation dynamics and are, therefore, used as robust drives to move and create magnetic skyrmions. In contrast to these expectations, we here find unpredictable, transiently chaotic dynamics induced by SOT at an artificial anisotropy-engineered defect in a magnetic racetrack. Based on these controlled conditions, we directly observe the nanoscale dynamics with holography-based, time-resolved x-ray imaging. In concert with micromagnetic simulations, we disclose a regime of violent picosecond fluctuations, including topological instabilities that, remarkably, result in deterministic final configurations. In addition, our images expose previously unseen skyrmion shedding and highlight the potential of transiently chaotic pathways for topological switching. Our approach offers new perspectives for the investigation and application of highly non-linear SOT dynamics in spintronics materials.

In ferromagnetic multilayers, a single laser pulse with a fluence above an optical nucleation threshold can create magnetic skyrmions, which are randomly distributed over the area of the laser spot. However, in order to study the dynamics of skyrmions and for their application in future data technology, a controllable localization of the skyrmion nucleation sites is crucial. Here, it is demonstrated that patterned reflective masks behind a thin magnetic film can be designed to locally tailor the optical excitation amplitudes reached, leading to spatially controlled skyrmion nucleation on the nanometer scale. Using x-ray microscopy, the influence of nanopatterned back-side aluminum masks on the optical excitation is studied in two sample geometries with varying layer sequence of substrate and magnetic Co/Pt multilayer. Surprisingly, the masks' effect on suppressing or enhancing skymion nucleation reverses when changing this sequence. Moreover, optical near-field enhancements additionally affect the spatial arrangement of the nucleated skyrmions. Simulations of the spatial modulation of the laser excitation, and the following heat transfer across the interfaces in the two sample geometries are employed to explain these observations. The results demonstrate a reliable approach to add nanometer-scale spatial control to optically induced magnetization processes on ultrafast timescales.

Experimental investigations of ultrafast magnetization dynamics increasingly employ resonant magnetic spectroscopy in the ultraviolet spectral range. Besides allowing to disentangle the element-specific transient response of functional magnetic systems, these techniques also promise to access attosecond to few-femtosecond dynamics of spin excitations. Here, we report on a systematic study of transient magnetic circular dichroism (MCD) on the transition metals Fe, Co and Ni as well as on a FeNi and GdFe alloy and reveal a delayed onset between the electronic and magnetic response. Supported by \textit{ab-initio} calculations, we attribute our observation to a transient energy shift of the absorption and MCD spectra at the corresponding elemental resonances due to non-equilibrium changes of electron occupations., Comment: 8 figures