Search

We directly measure the electronic structure of twisted graphene/MoS2 van der Waals heterostructures, in which both graphene and MoS2 are monolayers. We use cathode lens microscopy and microprobe angle-resolved photoemission spectroscopy measurements to image the surface, determine twist angle, and map the electronic structure of these artificial heterostructures. For monolayer graphene on monolayer MoS2, the resulting band structure reveals the absence of hybridization between the graphene and MoS2 electronic states. Further, the graphene-derived electronic structure in the heterostructures remains intact, irrespective of the twist angle between the two materials. In contrast, however, the electronic structure associated with the MoS2 layer is found to be twist-angle dependent; in particular, the relative difference in the energy of the valence band maximum at {\Gamma} and K of the MoS2 layer varies from approximately 0 to 0.2 eV. Our results suggest that monolayer MoS2 within the heterostructure becomes predominantly an indirect bandgap system for all twist angles except in the proximity of 30 degrees. This result enables potential bandgap engineering in van der Waals heterostructures comprised of monolayer structures., Comment: 20 pages including supplementary materials

We report ARPES and a set of in situ STM measurements on a narrow-terrace-width vicinal Cu(111) crystal surface, Cu(775), whose vicinal cut lies close to the transition between terrace and step modulation. These measurements show sharp zone-folding (or Umklapp) features with a periodicity in k||, indicating that the predominant reference plane is that of Cu(775), i.e. that the surface is predominately step-modulated. Our measurements also show variation in Umklapp intensity with photon energy, which is consistent with prior ARPES experiments on other vicinal Cu(111) surfaces and in agreement with our designation of the state as being step modulated. The measurements also show a weak terrace-modulated state, which, based on several characteristics, we attribute to the presence of terrace widths larger than the ideal terrace width. By measuring the intensity ratio of the two distinct surface-state modulations from PE and the terrace-width distribution from STM, we derive a value for the terrace width, at which the surface-state switches between the two modulations., Comment: 13 pages, 5 figures

Using low-temperature scanning tunneling microscopy, we demonstrate an unambiguous 1-D system that surprisingly undergoes a CDW instability on a metallic substrate. Our ability to directly and quantitatively measure the structural distortion of this system provides an accurate reference for comparison with first principles theory. In comparison to previously proposed physical mechanisms, we attribute this particular 1-D CDW instability to a ferromagnetic state. We show that though the linear arrayed dimers are not electronically isolated, they are magnetically independent, and hence can potentially serve as a binary spin-memory system., Comment: Includes Supplementary Information