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In this paper we investigate temperature and pressure effects on the properties of a positive pulsed streamer plasma. We use a corona plasma setup in which we vary the temperature between 303 and 773K at atmospheric pressure and the pressure between 37.9 and 100 kPa at room temperature to achieve the same neutral gas density and compare electrical and optical (ICCD imaging) measurements carried out in both experiments. From the measurements we found that the dissipated plasma energy and the average streamer propagation velocity are both higher for the temperature experiments at the same neutral gas densities as in the pressure experiments. This suggests the existence of a specific temperature effect. A possible explanation for this effect is a higher streamer conductivity at high temperatures, as was previously found in the literature. [ABSTRACT FROM AUTHOR]

Gas-cleaning techniques using nonthermal plasma are slowly introduced into industry nowadays. In this paper, we present a novel power modulator for the efficient generation of large-volume corona plasma. No expensive high-voltage components are required. Switching is done at an intermediate voltage level of 1 kV with standard thyristors. Detailed investigations on the modulator and a wire-plate corona reactor will be presented. In a systematic way, modulator parameters have been varied. Furthermore, reactor parameters, such as the number of electrodes and the electrode-plate distance, have been varied systematically. The yield of 0 radicals was determined from the measured ozone concentrations at the exhaust of the reactor. [ABSTRACT FROM AUTHOR]

To supply combustion engines or gasturbines with fuel gas obtained from biomass gasification, it is necessary to clean the fuel gas. Also the production of chemicals by processes such as Fisher-Tropsch requires a high gas quality. Especially heavy aromatic hydrocarbons (“tars”) must be removed. In this work, we give an overview of our investigations on tar removal by pulsed corona discharges as an alternative approach to catalytic or thermal tar cracking. Experimental results (at a gas temperature of 200°C) are reported for the removal of various model tar components in synthetic fuel gas. In order to identify the major reaction pathways, experiments were also done on tars in individual fuel gas components. The results show that tar removal by pulsed corona processing is possible. The process for tar removal is mainly via oxidation. Also termination reactions by CO play an important role. [ABSTRACT FROM AUTHOR]

Although removal of NOx by (pulsed) corona discharges has been thoroughly investigated for high concentrations of NOx in flue gas, removal of low levels in ambient air proves to be a difficult task. (Sub) ppm NOx levels exist in traffic tunnels due to accumulation of exhaust gases. The application of pulsed corona technology for purification of traffic tunnel air is studied during a series of lab and field experiments. An industrial pilot scale wire-cylinder type corona reactor has been utilized. Lab tests have been carried out using a diesel generator as NOx source. NOx conversion levels have been determined by applying two Recordum Airpointers (chemiluminescence-based detection). The detector appeared to be cross-sensitive for HNO3 and high levels of O3. NOx removal rates of 60-80% were obtained for inlet levels of 2-10 ppm. The SIE value of 10 ppm NOx removal is 7 J l-1. The corona discharges produce ppm level NOx at high energy densities. This intrinsic NOx production limits removal of inlet levels due to equilibrium between production and oxidation. [ABSTRACT FROM AUTHOR]

The oxidative degradation of two volatile organic compounds, i.e. toluene (fossil fuel based VOC) and limonene (biogenic VOC), has been studied. A hybrid pulsed power corona reactor with adjustable energy density has been utilized for degradation of ppm level target compounds in large air flows. The observed oxidation product range features an energy density-dependent spectrum of oxygen-functional hydrocarbons, which has been qualitatively discussed on the basis of literature studies. Typically, observed stable oxidation products for both target compounds are the biocompatible carboxylic acids acetic and formic acid. Measured degradation G-values are 23 nmol J-1 at 74% conversion of 70 ppm toluene and 181 nmol J-1 at 81% conversion of 10 ppm limonene [ABSTRACT FROM AUTHOR]

In this article we discuss a 10 kW high-voltage pulse generator for producing corona-induced plasma. The generator mainly consists of a three-step resonant charging circuit switched by thyristors, a transmission line transformer, and a triggered spark-gap switch. Voltage pulses of 30-100 kV with a rise time of about 20 ns, a pulse duration of 50-250 ns, pulse repetition rate of 1-900 pulses per second, energy of up to 12 J/pulse, and an average power of up to 10 kW have been achieved with a total energy transfer efficiency of about 80%-90%. At each frequency, the deviation of the energy per pulse is around 1.0%. Moreover, the generator has been tested for more than 100 h for both industrial demonstrations and laboratory investigations at an average output power of 1-10 kW. © 2001 American Institute of Physics. [ABSTRACT FROM AUTHOR]

Although pulsed corona technology for air purification is widely investigated by the lab experiments, large-scale application has yet to be proven. Industrial systems require large flow handling and thus, high corona power. An autonomous semi-industrial scale pilot wire-cylinder type corona reactor has been constructed for air purification demonstrations. The reactor is powered by a 10-kW spark gap-based pulsed power supply, capable of generating 60-kV 100-ns wide pulses with 1-kHz repetition rate. The pulses are optionally superimposed on a 0–30-kV dc bias to enable electrostatic precipitation. The system has been successfully applied during several field and lab experiments. Conversion data as a function of energy density are presented for NOx, NH3, H2S, toluene, limonene, and fine dust removal. The system proves feasibility of large-scale air purification by pulsed corona. [ABSTRACT FROM AUTHOR]

The Blumlein generator has been one of the most popular pulsed-power circuits. The pulse forming lines are charged simultaneously, and then discharged via a single switch, such as a spark gap. The generator can be used for single pulse or at a high repletion rate. However, for large pulsed power generation, one critical issue for such a single-switch based circuit topology is related to large switching currents. In this article, we propose a novel Blumlein circuit topology based on multiple switches. The pulsed forming lines are charged in parallel and then are synchronously commutated via multiple switches. No special synchronization trigger circuit is needed for the proposed circuit topology; this robust circuit topology is simple and very reliable. A prototype multiple-switch Blumlein generator with two spark-gap switches has been experimentally evaluated with both resistive and corona plasma loads. In terms of the switching currents, it is observed that the two switches can be synchronized within 2–3 ns. The energy conversion efficiencies are 82% and 76.8% for a matched resistive load and a plasma reactor, respectively. [ABSTRACT FROM AUTHOR]