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Long-time-series, high-resolution datasets of the column-averaged dry-air mole fraction of carbon dioxide (XCO 2 ) have great practical importance for mitigating the greenhouse effect, assessing carbon emissions and implementing a low-carbon cycle. However, the mainstream XCO 2 datasets obtained from satellite observations have coarse spatial resolutions and are inadequate for supporting research applications with different precision requirements. Here, we developed a new spatial machine learning model by fusing spatial information with CatBoost, called SCatBoost, to fill the above gap based on existing global land-mapped 1° XCO 2 data (GLM-XCO 2 ). The 1-km-spatial-resolution dataset containing XCO 2 values in China from 2012 to 2019 reconstructed by SCatBoost has stronger and more stable predictive power (confirmed with a cross-validation (R 2  = 0.88 and RSME = 0.20 ppm)) than other traditional models. According to the estimated dataset, the overall national XCO 2 showed an increasing trend, with the annual mean concentration rising from 392.65 ppm to 410.36 ppm. In addition, the spatial distribution of XCO 2 concentrations in China reflects significantly higher concentrations in the eastern coastal areas than in the western inland areas. The contributions of this study can be summarized as follows: (1) It proposes SCatBoost, integrating the advantages of machine learning methods and spatial characteristics with a high prediction accuracy; (2) It presents a dataset of fine-scale and high resolution XCO 2 over China from 2012 to 2019 by the model of SCatBoost; (3) Based on the generated data, we identify the spatiotemporal trends of XCO 2 in the scale of nation and city agglomeration. These long-term and high resolution XCO 2 data help understand the spatiotemporal variations in XCO 2 , thereby improving policy decisions and planning about carbon reduction., Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper., (Copyright © 2023 Elsevier Inc. All rights reserved.)