Adults 50 years of age and older who engage in regular physical activity have lower rates of hypertension, cardiovascular disease, stroke, obesity, diabetes, and depression;1,2 moreover, they are able to maintain an independent lifestyle and enhanced quality of life.3,4 Nevertheless, almost two-thirds of older adults do not meet the United States national guidelines of 150 minutes of moderate physical activity a week.5 Moreover, physical activity trends continue to decline with age regardless of initial physical activity levels.6 Older adults have unique psychological, social, physical, and environmental influences compared to their younger counterparts. They have more chronic health conditions,6 a lack of knowledge or limited interest about physical activity and health,7 declining personal and community support systems, decreased social networks, increased perceptions of environmental barriers, and limited income.8–10 In light of these differences, it is imprudent to assume that effective strategies that increase physical activity in younger adults can readily be applied to older adults and achieve similar outcomes. Considering the explosive growth of the 60+ adult demographic in the United States—the fastest growing segment of the population6—a better understanding of strategies to maintain physical activity later in life is needed. Several studies have reported on predictors of physical activity initiation (defined here as the beginning of physical activity adoption up to 6 months) in older adults. Motivators for physical activity initiation in this population include physical and psychological well-being,11 maintenance of independent lifestyles,12 and social connections and enjoyment.13 Unfortunately, participation rates in physical activity following initiation drop precipitously. Martin et al14 and Cooper et al15 report an average 50% drop in adherence to physical activity at 6–7 month follow-up. However, longer term achievement of physical activity is needed to maintain the health benefits of exercise.3 Older adults who initiate physical activity may discontinue participation due to changes in physical condition (eg, joint pain, cardiac changes),10,14,15 environmental barriers (eg, safety, lack of transportation),11 and psychosocial issues (eg, lack of a partner, low confidence in physical activity abilities).10 Few studies have investigated how predictors for initiation of physical activity confer long-term achievement of physical activity. Additionally, most short-term and long-term physical activity behavior change studies focus on specific interventions with little discussion about the underlying strategies and constructs that they seek to target.16 Further investigation is needed to identify specific theoretical components that may provide better support for sustained physical activity behaviors in older adults. Self-Determination (SDT)17 and Social-Cognitive (SCT)18 theories support the development of positive self-regulatory factors in individuals. Conceptually, these theories explain both initiation and maintenance of healthy behaviors. Central to SDT are constructs of autonomy, competence, and relatedness. Interventions supporting these basic psychological needs “foster the most volitional and high quality forms of motivation and engagement for activities, including enhanced performance and persistence…”.17(p.60) Central to SCT are self-efficacy beliefs, which are “the foundation of human motivation and action.”18(p.144) Previous accomplishments, relatedness, verbal persuasion, vicarious experience, and physiological arousal constructs are the primary supports for self-efficacy.18 SDT and SCT constructs primarily have targeted physical activity initiation19–23 and important limitations prevent understanding of the theoretical components for long-term physical activity maintenance. First, most studies are short-term (< 6 months), so long-term behaviors cannot be inferred. Second, most long-term studies (≥ 6 months) employ an intervention that is carried on throughout the length of trial, with evaluation of outcome measures performed immediately after intervention conclusion. This limits translation of the effects of intervening components on true behavior adoption and change. Lastly, few studies address the explicit relationship between intervening components and theoretical constructs (and changes in these components/constructs) and long-term behavior change in older adults. Intervening components often are not operationalized adequately, implemented, or they are delivered in “packaged interventions” so their individual efficacies cannot be ascertained. Further investigation is needed to identify SDT and SCT related intervening components and constructs that can be translated into interventions to support long-term achievement of physical activity in older adults. Unique to this investigation is our focus on theoretical constructs with conceptual links reported in a previous randomized controlled trial.24 In this study, the provision of social support, goal setting, and mental imagery were part of a peer-based intervention that resulted in long-term effects on physical activity behavior with older adults. Interventions employing goal setting and social support (eg, social contact between coaches and participants) have shown consistently positive results in physical activity initiation in older adults.14,19,20,25 Guided imagery also has been shown to impact exercise intentions, affect, and motives in randomized controlled trials.26–29 Together, social support, goal setting, and guided mental imagery are a unique and practical set of strategies that have potential to impact physical activity behavior in older adults. The objective of the current study was to identify intervening components and theoretical constructs from a 4-month behavioral intervention that may influence achievement of physical activity (at 18 months) among older adults. We used a mixed-methods approach including qualitative analysis of interview data and quantitative analysis of psychosocial and behavioral outcome data. This is an expansive and creative form of investigation that incorporates multiple approaches (such as inductive and deductive methods) in answering research questions.