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A selective area chemical vapour deposition technique has been used to fabricate continuous and patterned epitaxial CrO2 thin films on (100)-oriented TiO2 substrates. Precessional magnetization dynamics were stimulated both electrically and optically, and probed by means of time-resolved Kerr microscopy and vector network analyser ferromagnetic resonance techniques. The dependence of the precession frequency and the effective damping parameter upon the static applied magnetic field were investigated. All films exhibited a large in-plane uniaxial anisotropy. The effective damping parameter was found to exhibit strong field dependence in the vicinity of the hard axis saturation field. However, continuous and patterned films were found to possess generally similar dynamic properties, confirming the suitability of the deposition technique for fabrication of future spintronic devices. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy has been used to perform optically detected, phase-resolved spin–orbit torque ferromagnetic resonance (SOT-FMR) measurements on a microscale CoFeB ellipse at the center of a Pt Hall cross subject to RF and DC current. Time-resolved polar Kerr images revealed localized dynamics with large amplitude at the center and weaker amplitude at the edges. Therefore, field swept SOT-FMR spectra were acquired from the so-called center mode to probe the SOTs active at the center of the ellipse, thus minimizing non-uniform edge contributions. When the magnetic field was applied at 30° from the hard axis of the ellipse and a DC current was applied, a marked asymmetry was observed in the amplitude and linewidth of the FMR peaks as the applied field was reversed. Both absorptive and dispersive parts of the spectra were in good agreement with a macrospin calculation. The damping parameter (α) and the Slonczewski torque parameter were determined to be 0.025 and (6.75 ± 0.75) × 10−7 Oe A−1 cm2, respectively. The hard axis SOT-FMR linewidth was found to be almost independent of the DC current value, suggesting that the SOT has a minimal influence in the hard axis configuration and that thermal effects were insignificant. This study paves the way for spatially resolved measurements of SOT probed using localized modes of microscale devices that go beyond the spatially averaged capability of electrical measurement techniques. [ABSTRACT FROM AUTHOR]

Time-resolved scanning Kerr microscopy (TRSKM) has been used to image precessional magnetization dynamics excited by a DC current within a nano-contact (NC) spin Hall nano-oscillator (SHNO). Injection of a radio frequency (RF) current was used to phase lock the SHNO to TRSKM. The out of plane magnetization was detected by means of the polar magneto optical Kerr effect (MOKE). However, longitudinal MOKE images were dominated by an artifact arising from the edges of the Au NCs. Time resolved imaging revealed the simultaneous excitation of a non-linear "bullet" mode at the centre of the device, once the DC current exceeded a threshold value, and ferromagnetic resonance (FMR) induced by the RF current. However, the FMR response observed for sub-critical DC current values exhibits an amplitude minimum at the centre, which is attributed to spreading of the RF spin current due to the reactance of the device structure. This FMR response can be subtracted to yield images of the bullet mode. As the DC current is increased above threshold, the bullet mode appears to increase in size, suggesting increased translational motion. The reduced spatial overlap of the bullet and FMR modes, and this putative translational motion, may impede the injection locking and contribute to the reduced locking range observed within NC-SHNO devices. This illustrates a more general need to control the geometry of an injection-locked oscillator so that the autonomous dynamics of the oscillator exhibit strong spatial overlap with those resulting from the injected signal. [ABSTRACT FROM AUTHOR]

Precessional dynamics of a Co50Fe50(0.7)/Ni90Fe10(5)/Dy(1)/Ru(3) (thicknesses in nm) thin film have been explored by low temperature time-resolved magneto-optical Kerr effect and phase-resolved x-ray ferromagnetic resonance measurements. As the temperature was decreased from 300 to 140 K, the magnetic damping was found to increase rapidly while the resonance field was strongly reduced. Static x-ray magnetic circular dichroism measurements revealed increasing ferromagnetic order of the Dy moment antiparallel to that of Co50Fe50/Ni90Fe10. Increased coupling of the Dy orbital moment to the precessing spin magnetization leads to significantly increased damping and gyromagnetic ratio of the film while leaving its magnetic anisotropy effectively unchanged. [ABSTRACT FROM AUTHOR]

Phase-resolved x-ray ferromagnetic resonance (XFMR) has been measured in fluorescence yield, extending the application of XFMR to opaque samples on opaque substrates. Magnetization dynamics were excited in a Co50Fe50(0.7)/Ni90Fe10(5) bilayer by means of a continuous wave microwave excitation, while x-ray magnetic circular dichroism (XMCD) spectra were measured stroboscopically at different points in the precession cycle. By tuning the x-ray energy to the L3 edges of Ni and Fe, the dependence of the real and imaginary components of the element specific magnetic susceptibility on the strength of an externally applied static bias field was determined. First results from measurements on a Co50Fe50(0.7)/Ni90Fe10(5)/Dy(1) sample confirm that enhanced damping results from the addition of the Dy cap. [ABSTRACT FROM AUTHOR]

Element-specific phase-resolved x-ray ferromagnetic resonance (FMR) was used to study spin pumping within Co50Fe50(3)/Cu(6)/Ni80Fe20(5) (thicknesses in nanometers) spin valve structures with large areas, so that edge effects typical of nanopillars used in standard magnetotransport experiments could be neglected. The phase of precession of the Co50Fe50 fixed layer was recorded as FMR was induced in the Ni80Fe20 free layer. The field dependence of the fixed layer phase contains a clear signature of spin transfer torque (STT) coupling due to spin pumping. Fitting the phase delay yields the spin-mixing conductance, the quantity that controls all spin transfer phenomena. The STT coupling is destroyed by insertion of Ta into the middle of the Cu layer. [ABSTRACT FROM AUTHOR]

Despite recent progress in spin-current research, the detection of spin current has mostly remained indirect. By synchronizing a microwave waveform with synchrotron x-ray pulses, we use the ferromagnetic resonance of the Py (Ni81Fe19) layer in a Py/Cu/Cu75Mn25/Cu/Co multilayer to pump a pure ac spin current into the Cu75Mn25 and Co layers, and then directly probe the spin current within the Cu75Mn25 layer and the spin dynamics of the Co layer by x-ray magnetic circular dichroism. This element-resolved pump-probe measurement unambiguously identifies the ac spin current in the Cu75Mn25 layer. [ABSTRACT FROM AUTHOR]