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Ionic conductive elastomers (ICEs) are emerging stretchable and ionic conductive materials that are solvent-free and thus demonstrate excellent thermal stability. Three-dimensional (3D) printing that creates complex 3D structures in free forms is considered as an ideal approach to manufacture sophisticated ICE-based devices. However, the current technologies constrain 3D printed ICE structures in a single material, which greatly limits functionality and performance of ICE-based devices and machines. Here, we report a digital light processing (DLP)-based multimaterial 3D printing capability to seemly integrate ultraviolet-curable ICE (UV-ICE) with nonconductive materials to create ionic flexible electronic devices in 3D forms with enhanced performance. This unique capability allows us to readily manufacture various 3D flexible electronic devices. To demonstrate this, we printed UV-ICE circuits into polymer substrates with different mechanical properties to create resistive strain and force sensors; we printed flexible capacitive sensors with high sensitivity (2 kPa

Stretchable strain sensor detects a wide range of strain variation and is therefore a key component in various applications. Unlike traditional ones made of elastomers doped with conductive components or fabricated with liquid conductors, ionically conductive hydrogel-based strain sensors remain conductive under large deformations and are biocompatible. However, dehydration is a challenging issue for the latter. Researchers have developed hydrogel-elastomer-based strain sensors where an elastomer matrix encapsulates a hydrogel circuit to prevent its dehydration. However, the reported multi-step approaches are generally time-consuming. Our group recently reported a multimaterial 3D printing approach that enables fast fabrication of such sensors, yet requires a self-built digital-light-processing-based multimaterial 3D printer. Here, we report a simple projection lithography method to fabricate hydrogel-elastomer-based stretchable strain sensors within 5 minutes. This method only requires a UV projector/lamp with photomasks; the chemicals are commercially available; the protocols for preparing the polymer precursors are friendly to users without chemistry background. Moreover, the manufacturing flexibility allows users to readily pattern the sensor circuit and attach the sensor to a 3D printed soft pneumatic actuator to enable strain sensing on the latter. The proposed approach paves a simple and versatile way to fabricate hydrogel-elastomer-based stretchable strain sensors and flexible electronic devices.

Conventional robots have shown good positioning accuracy and reliability in multiple environments. However, the robots’ lack of flexibility makes them unsuitable for application in certain areas. Thus, a soft robotic system should be considered due to its adaptivity and flexibility. This paper proposes a novel shape memory alloy (SMA)-actuated multiple degrees of freedom (DOF) soft robot, which theoretically supports a maximum of nine-DOF movement and good positioning accuracy. A motion test and positioning evaluation are conducted for the proposed multi-DOF soft robot. The structural design, control method, and analysis of the kinematics and the coordinate system are also given.

4D printing is an emerging fabrication technology that enables 3D printed structures to change configuration over "time" in response to an environmental stimulus. Compared with other soft active materials used for 4D printing, shape-memory polymers (SMPs) have higher stiffness, and are compatible with various 3D printing technologies. Among them, ultraviolet (UV)-curable SMPs are compatible with Digital Light Processing (DLP)-based 3D printing to fabricate SMP-based structures with complex geometry and high-resolution. However, UV-curable SMPs have limitations in terms of mechanical performance, which significantly constrains their application ranges. Here, a mechanically robust and UV-curable SMP system is reported, which is highly deformable, fatigue resistant, and compatible with DLP-based 3D printing, to fabricate high-resolution (up to 2 µm), highly complex 3D structures that exhibit large shape change (up to 1240%) upon heating. More importantly, the developed SMP system exhibits excellent fatigue resistance and can be repeatedly loaded more than 10 000 times. The development of the mechanically robust and UV-curable SMPs significantly improves the mechanical performance of the SMP-based 4D printing structures, which allows them to be applied to engineering applications such as aerospace, smart furniture, and soft robots.