Search

Mass measurements of $^{31-33}$Na and $^{31-35}$Mg using the TITAN MR-TOF-MS at TRIUMF's ISAC facility are presented, with the uncertainty of the $^{33}$Na mass reduced by over two orders of magnitude. The excellent performance of the MR-TOF-MS has also allowed the discovery of a millisecond isomer in $^{32}$Na. The precision obtained shows that the binding energy of the normally closed N = 20 neutron shell reaches a minimum for $^{32}$Mg but increases significantly for $^{31}$Na, hinting at the possibility of enhanced shell strength toward the unbound $^{28}$O. We compare the results with new ab initio predictions that raise intriguing questions of nuclear structure beyond the dripline.

Studies aiming to determine the astrophysical origins of nuclei produced by the rapid neutron capture process ($r$ process) rely on nuclear properties as inputs for simulations. The solar abundances can be used as a benchmark for such calculations, with the $r$-process rare-earth peak (REP) around mass number ($A$) 164 being of special interest due to its presently unknown origin. With the advancement of rare isotope beam production over the last decade and improvement in experimental sensitivities, many of these REP nuclides have become accessible for measurement. Masses are one of the most critical inputs as they impact multiple nuclear properties, namely the neutron-separation energies, neutron capture rates, $\beta$-decay rates, and $\beta$-delayed neutron emission probabilities. In this work, we report masses of 20 neutron-rich nuclides (along the Ba, La, Ce, Pr, Nd, Pm, Gd, Dy and Ho isotopic chains) produced at the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) facility at Argonne National Laboratory. The masses were measured with the Canadian Penning trap (CPT) mass spectrometer using the Phase-Imaging Ion-Cyclotron-Resonance (PI-ICR) technique. We then use these new masses along with previously published CPT masses to inform predictions for a Markov Chain Monte Carlo (MCMC) procedure aiming to identify the astrophysical conditions consistent with both solar data and mass measurements. We show that the MCMC responds to this updated mass information, producing refined results for both mass predictions and REP abundances., Comment: 11 pages, 8 figures

Precise mass measurements of the ground and isomeric states of the odd-odd $^{108, 110, 112, 114, 116}$Rh were performed using the Canadian Penning Trap at Argonne National Laboratory, showing good agreement with recent JYFLTRAP measurements. A new possible isomeric state of $^{114}$Rh was also observed. These isotopes are part of the longest odd-odd chain of identical ground-state spin-parity assignment of 1$^+$, spanning $^{104-118}$Rh, despite being in a region of deformation. Realistic phenomenological mean-field calculations using ``universal'' Wood-Saxon Hamiltonian were performed, which explained this phenomenon for the first time. In addition, multi-quasiparticle blocking calculations were performed to study the configuration of low-lying states in the odd-odd Rh nuclei, elucidating anomalous isomeric yield ratio observed for $^{114}$Rh.

Atomic masses are a foundational quantity in our understanding of nuclear structure, astrophysics and fundamental symmetries. The long-standing goal of creating a predictive global model for the binding energy of a nucleus remains a significant challenge, however, and prompts the need for precise measurements of atomic masses to serve as anchor points for model developments. We present precise mass measurements of neutron-rich Ru and Pd isotopes performed at the Californium Rare Isotope Breeder Upgrade facility at Argonne National Laboratory using the Canadian Penning Trap mass spectrometer. The masses of $^{108}$Ru, $^{110}$Ru and $^{116}$Pd were measured to a relative mass precision $\delta m/m \approx 10^{-8}$ via the phase-imaging ion-cyclotron-resonance technique, and represent an improvement of approximately an order of magnitude over previous measurements. These mass data were used in conjunction with the physically interpretable machine learning (PIML) model, which uses a mixture density neural network to model mass excesses via a mixture of Gaussian distributions. The effects of our new mass data on a Bayesian-updating of a PIML model are presented., Comment: 6 pages, 4 figures

The Canadian Penning Trap mass spectrometer (CPT) has conducted precision mass measurements of neutron-rich nuclides from the CAlifornium Rare Isotope Breeder Upgrade (CARIBU) of the Argonne Tandem Linac Accelerator System (ATLAS) facility at Argonne National Laboratory using the Phase-Imaging Ion-Cyclotron-Resonance (PIICR) technique for over half a decade. Here we discuss the CPT system, and methods to improve accuracy and precision in mass measurement using PI-ICR including some optimization techniques and recently studied systematic effects., Comment: 19 pages, 9 figures

These proceedings summarize the program and discussions of the ``Workshop on Xenon Detector $0\nu\beta\beta$ Searches: Steps Towards the Kilotonne Scale'' held on October 25-27 2023 at SLAC National Accelerator Laboratory. This workshop brought together experts from the communities of neutrinoless double-beta decay and dark matter detection, to discuss paths forward for the realization of monolithic experiments with xenon approaching the kilotonne scale., Comment: 7 pages, 2 figures. Proceedings

We report precision mass measurements of $^{133}$Sb, $^{133g,m}$Te, and $^{133g,m}$I, produced at CARIBU at Argonne National Laboratory's ATLAS facility and measured using the Canadian Penning Trap mass spectrometer. These masses clarify an anomaly in the $^{133}$Te $\beta$-decay. The masses reported in the 2020 Atomic Mass Evaluation (M. Wang et al., 2021) produce $Q_{\beta^-}(^{133}$Te)=2920(6) keV; however, the highest-lying $^{133}$I level populated in this decay is observed at $E_i=2935.83(15)$ keV, resulting in an anomalous $Q_{\beta^{-}}^{i}=-16(6)$~keV. Our new measurements give $Q_{\beta^-}(^{133}\text{Te})=2934.8(11)$ keV, a factor of five more precise, yielding $Q{_\beta^i}=-1.0(12)$~keV, a 3$\sigma$ shift from the previous results. This resolves this anomaly, but indicates further anomalies in our understanding of the structure of this isotope., Comment: 5 pages, 3 figures

The Beta-decay Paul Trap is an open-geometry, linear trap used to measure the decays of $^8$Li and $^8$B to search for a tensor contribution to the weak interaction. In the latest $^8$Li measurement of Burkey et al. (2022), $\beta$ scattering was the dominant experimental systematic uncertainty. The Beta-decay Paul Trap Mk IV reduces the prevalence of $\beta$ scattering by a factor of 4 through a redesigned electrode geometry and the use of glassy carbon and graphite as electrode materials. The trap has been constructed and successfully commissioned with $^8$Li in a new data campaign that collected 2.6 million triple coincidence events, an increase in statistics by 30% with 4 times less $\beta$ scattering compared to the previous $^8$Li data set., Comment: 17 pages, 7 figures

We report on the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program "Nuclear Isomers in the Era of FRIB". We outline the many ways isomers influence and contribute to nuclear science and technology, especially in the four FRIB pillars: properties of rare isotopes, nuclear astrophysics, fundamental symmetries, and applications for the nation and society. We conclude with a resolution stating our recommendation that the nuclear physics community actively pursue isomer research. A white paper is forthcoming., Comment: 4 pages including references

This whitepaper presents the research priorities decided on by attendees of the 2022 Town Meeting for Fundamental Symmetries, Neutrons and Neutrinos, which took place December 13-15, 2022 in Chapel Hill, NC, as part of the Nuclear Science Advisory Committee (NSAC) 2023 Long Range Planning process. A total of 275 scientists registered for the meeting. The whitepaper makes a number of explicit recommendations and justifies them in detail.

A new \textsuperscript{3}He-driven IGISOL production station and mass separator have been designed to produce neutron-deficient low-mass isotopes at the Cyclotron Institute for the TAMUTRAP facility. The LSTAR design has a mass resolution $M/\Delta M\geq 3, 000$ to reject contaminants with $\gt95\%$ efficiency., Comment: Proceeding for EMIS 2022

This white paper was submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting in preparation for the next NSAC Long Range Plan. We advocate to support current and future theoretical and experimental searches for physics beyond the Standard Model using nuclear $\beta$ decay., Comment: 12 pages, 2 figures, White paper submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting at the University of North Carolina Chapel Hill

We report here on the recent upgrade of the TwinSol radioactive nuclear beam (RNB) facility at the University of Notre Dame. The new TriSol system includes a magnetic dipole to provide a second beamline and a third solenoid which acts to reduce the size of the radioactive beam on target., Comment: submitted to Nuclear Instruments and Methods A

The electroweak interaction in the Standard Model (SM) is described by a pure vector-axial-vector structure, though any Lorentz-invariant component could contribute. In this work, we present the most precise measurement of tensor currents in the low-energy regime by examining the $\beta$-$\bar{\nu}$ correlation of trapped $^{8}$Li ions with the Beta-decay Paul Trap. We find $a_{\beta\nu} = -0.3325 \pm 0.0013_{stat} \pm 0.0019_{syst}$ at $1\sigma$ for the case of coupling to right-handed neutrinos $(C_T=-C_T')$, which is consistent with the SM prediction., Comment: 6 pages, 3 figures, 1 table

Isobaric quintets provide the best test of the isobaric multiplet mass equation (IMME) and can uniquely identify higher order corrections suggestive of isospin symmetry breaking effects in the nuclear Hamiltonian. The Generalized IMME (GIMME) is a novel microscopic interaction theory that predicts an extension to the quadratic form of the IMME. Only the $A=20, 32$ $T=2$ quintets have the exotic $T_z = -2$ member ground state mass determined to high-precision by Penning trap mass spectrometry. In this work, we establish $A=36$ as the third high-precision $T=2$ isobaric quintet with the $T_z = -2$ member ground state mass measured by Penning trap mass spectrometry and provide the first test of the predictive power of the GIMME. A radioactive beam of neutron-deficient $^{36}$Ca was produced by projectile fragmentation at the National Superconducting Cyclotron Laboratory. The beam was thermalized and the mass of $^{36}$Ca$^+$ and $^{36}$Ca$^{2+}$ measured by the Time of Flight - Ion Cyclotron Resonance method in the LEBIT 9.4 T Penning trap. We measure the mass excess of $^{36}$Ca to be ME$ = -6483.6(56)$ keV, an improvement in precision by a factor of 6 over the literature value. The new datum is considered together with evaluated nuclear data on the $A=36$, $T=2$ quintet. We find agreement with the quadratic form of the IMME given by isospin symmetry, but only coarse qualitative agreement with predictions of the GIMME. A total of three isobaric quintets have their most exotic members measured by Penning trap mass spectrometry. The GIMME predictions in the $T = 2$ quintet appear to break down for $A = 32$ and greater.

The Isobaric Multiplet Mass Equation (IMME) has been successful at predicting the masses of isobaric analogue states in the same multiplet, while its coefficients are known to follow trends as functions of mass number. The Atomic Mass Evaluation 2016 [Chin. Phys. C 41, 030003 (2017)] $^{44}$V mass value results in an negative $c$ coefficient for the IMME quadratic term. The $b$ and $c$ coefficients can provide constraints for construction of the isospin-nonconserving (INC) Hamiltonians for the $pf$ shell. The excitation energy of the $0^+, T=2$ level in $^{44}$V is currently unknown and can be used to constrain the $^{44}$Cr mass. The aim of the experiment was to perform high-precision mass measurements to resolve the difference between $^{44}$V isomeric and ground states, to test the IMME, and to provide ingredients for identifying the $0^+$, $T=2$ state in $^{44}$V. High-precision Penning trap mass spectrometry was performed at LEBIT, to measure the cyclotron frequency ratios of [$^{44g,m}$VO]$^+$ versus [$^{32}$SCO]$^+$, a reference mass, to extract both the isomeric and ground state masses of $^{44}$V. The mass excess of the ground and isomeric states in $^{44}$V were measured to be $-23\ 804.9(80)$ keV/$\text{c}^2$ and $-23\ 537.0(55)$ keV/$\text{c}^2$. This yielded a new proton separation energy of $S_p$ = 1\ 773(10) keV. The new mass values of $^{44}$V have been used to deduce the IMME $b$ and $c$ coefficients of the lowest $2^+$ and $6^+$ triplets in $A=44$. The $2^+$ $c$ coefficient is verified with the IMME trend and agrees with the shell-model predictions using charge-dependent Hamiltonians. The mirror energy differences were determined between $^{44}$V and $^{44}$Sc, in line with isospin-symmetry. The new value of the proton separation energy determined will be important for the determination of the $0^+$, $T=2$ state in $^{44}$V and for prediction of the mass of $^{44}$Cr., Comment: 9 pages, 5 figures

The JYFLTRAP double Penning trap at the Ion Guide Isotope Separator On-Line (IGISOL) facility has been used to measure the atomic masses of 13 neutron-rich rare-earth isotopes. Eight of the nuclides, $^{161}$Pm, $^{163}$Sm, $^{164,165}$Eu, $^{167}$Gd, and $^{165,167,168}$Tb, were measured for the first time. The systematics of the mass surface has been studied via one- and two-neutron separation energies as well as neutron pairing-gap and shell-gap energies. The proton-neutron pairing strength has also been investigated. The impact of the new mass values on the astrophysical rapid neutron capture process has been studied. The calculated abundance distribution results in a better agreement with the solar abundance pattern near the top of the rare-earth abundance peak at around $A\approx165$., Comment: 15 pages, 17 figures

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context., Comment: 132 pages, 18 figures, submitted to Journal of Physics G

The rare-earth peak in the $r$-process abundance pattern depends sensitively on both the astrophysical conditions and subtle changes in nuclear structure in the region. This work takes an important step elucidating the nuclear structure and reducing the uncertainties in $r$-process calculations via precise atomic mass measurements at the JYFLTRAP double Penning trap. $^{158}$Nd, $^{160}$Pm, $^{162}$Sm, and $^{164-166}$Gd have been measured for the first time and the precisions for $^{156}$Nd, $^{158}$Pm, $^{162,163}$Eu, $^{163}$Gd, and $^{164}$Tb have been improved considerably. Nuclear structure has been probed via two-neutron separation energies $S_{2n}$ and neutron pairing energy metrics $D_n$. The data do not support the existence of a subshell closure at $N=100$. Neutron pairing has been found to be weaker than predicted by theoretical mass models. The impact on the calculated $r$-process abundances has been studied. Substantial changes resulting in a smoother abundance distribution and a better agreement with the solar $r$-process abundances are observed., Comment: 8 pages, 4 figures, accepted for publication in Physical Review Letters

The region near Z=28, N=40 is a subject of great interest for nuclear structure studies due to spectroscopic signatures in $^{68}$Ni suggesting a subshell closure at N=40. Trends in nuclear masses and their derivatives provide a complementary approach to shell structure investigations via separation energies. Penning trap mass spectrometry has provided precise measurements for a number of nuclei in this region, however a complete picture of the mass surfaces has so far been limited by the large uncertainty remaining for nuclei with N > 40 along the iron and cobalt chains. Here we present the first Penning trap measurements of $^{68,69}$Co, performed at the Low-Energy Beam and Ion Trap facility at the National Superconducting Cyclotron Laboratory. In addition, we perform ab initio calculations of ground state and two-neutron separation energies of cobalt isotopes with the valence-space in-medium similarity renormalization group approach based on a particular set of two- and three-nucleon forces which predict saturation in infinite matter. We discuss the importance of these measurements and calculations for understanding the evolution of nuclear structure near $^{68}$Ni., Comment: 7 pages, 6 figures

A direct $Q_{EC}$-value measurement of the superallowed $\beta^+$ emitter $^{22}$Mg was performed using TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). The direct ground-state to ground-state atomic mass difference between $^{22}$Mg and $^{22}$Na was determined to be $Q_{EC}=4781.40(22)$~keV, representing the most precise single measurement of this quantity to date. In a continued push towards calculating superallowed isospin-symmetry-breaking (ISB) corrections from first principles, ab-initio shell-model calculations of the $A=22$ IMME are also presented for the first time using the valence-space in-medium similarity renormalization group formalism. With particular starting two- and three-nucleon forces, this approach demonstrates a level of agreement with the experimental data that suggests reliable ab-initio calculations of superallowed ISB corrections are now possible.

If the mass excess of neutron-deficient nuclei and their neutron-rich mirror partners are both known, it can be shown that deviations of the Isobaric Mass Multiplet Equation (IMME) in the form of a cubic term can be probed. Such a cubic term was probed by using the atomic mass of neutron-rich magnesium isotopes measured using the TITAN Penning trap and the recently measured proton-separation energies of $^{29}$Cl and $^{30}$Ar. The atomic mass of $^{27}$Mg was found to be within 1.6$\sigma$ of the value stated in the Atomic Mass Evaluation. The atomic masses of $^{28,29}$Mg were measured to be both within 1$\sigma$, while being 8 and 34 times more precise, respectively. Using the $^{29}$Mg mass excess and previous measurements of $^{29}$Cl we uncovered a cubic coefficient of $d$ = 28(7) keV, which is the largest known cubic coefficient of the IMME. This departure, however, could also be caused by experimental data with unknown systematic errors. Hence there is a need to confirm the mass excess of $^{28}$S and the one-neutron separation energy of $^{29}$Cl, which have both come from a single measurement. Finally, our results were compared to ab initio calculations from the valence-space in-medium similarity renormalization group, resulting in a good agreement., Comment: 7 pages, 3 figures

We report the mass measurement of $^{56}$Cu, using the LEBIT 9.4T Penning trap mass spectrometer at the National Superconducting Cyclotron Laboratory at Michigan State University. The mass of $^{56}$Cu is critical for constraining the reaction rates of the $^{55}$Ni(p,$\gamma$)$^{56}$Cu(p,$\gamma$)$^{57}$Zn($\beta^+$)$^{57}$Cu bypass around the $^{56}$Ni waiting point. Previous recommended mass excess values have disagreed by several hundred keV. Our new value, ME=$-38 626.7(6.4)$ keV, is a factor of 30 more precise than the suggested value from the 2012 atomic mass evaluation [Chin. Phys. C {\bf{36}}, 1603 (2012)], and more than a factor of 12 more precise than values calculated using local mass extrapolations, while agreeing with the newest 2016 atomic mass evaluation value [Chin. Phys. C {\bf{41}}, 030003 (2017)]. The new experimental average was used to calculate the astrophysical $^{55}$Ni(p,$\gamma$) and $^{57}$Zn($\gamma$,p) reaction rates and perform reaction network calculations of the rp-process. These show that the rp-process flow redirects around the $^{56}$Ni waiting point through the $^{55}$Ni(p,$\gamma$) route, allowing it to proceed to higher masses more quickly and resulting in a reduction in ashes around this waiting point and an enhancement to higher-mass ashes., Comment: 6 pages, 5 figures

We present the results of precision mass measurements of neutron-rich cadmium isotopes. These nuclei approach the $N=82$ closed neutron shell and are important to nuclear structure as they lie near doubly-magic $^{132}$Sn on the chart of nuclides. Of particular note is the clear identification of the ground state mass in $^{127}$Cd along with the isomeric state. We show that the ground state identified in a previous mass measurement which dominates the mass value in the Atomic Mass Evaluation is an isomeric state. In addition to $^{127/m}$Cd, we present other cadmium masses measured ($^{125/m}$Cd and $^{126}$Cd) in a recent TITAN experiment at TRIUMF. Finally, we compare our measurements to new \emph{ab initio} shell-model calculations and comment on the state of the field in the $N=82$ region., Comment: 8 Pages with citations, 3 Figures, 2 Tables

We report on the mass measurements of several neutron-rich $\mathrm{Rb}$ and $\mathrm{Sr}$ isotopes in the $A \approx 100$ region with the TITAN Penning-trap mass spectrometer. Using highly charged ions in the charge state $q=10+$, the masses of $^{98,99}\mathrm{Rb}$ and $^{98-100}\mathrm{Sr}$ have been determined with a precision of $6 - 12\ \mathrm{keV}$, making their uncertainty negligible for r-process nucleosynthesis network calculations. The mass of $^{101}\mathrm{Sr}$ has been determined directly for the first time with a precision eight times higher than the previous indirect measurement and a deviation of $3\sigma$ when compared to the Atomic Mass Evaluation. We also confirm the mass of $^{100}\mathrm{Rb}$ from a previous measurement. Furthermore, our data indicates the existance of a low-lying isomer with $80\ \mathrm{keV}$ excitation energy in $^{98}\mathrm{Rb}$. We show that our updated mass values lead to minor changes in the r-process by calculating fractional abundances in the $A\approx 100$ region of the nuclear chart., Comment: 8 pages, 5 figures

We report the first direct measurement of the $^{14}\text{O}$ superallowed Fermi $\beta$-decay $Q_{EC}$-value, the last of the so-called "traditional nine" superallowed Fermi $\beta$-decays to be measured with Penning trap mass spectrometry. $^{14}$O, along with the other low-$Z$ superallowed $\beta$-emitter, $^{10}$C, is crucial for setting limits on the existence of possible scalar currents. The new ground state $Q_{EC}$ value, 5144.364(25) keV, when combined with the energy of the $0^+$ daughter state, $E_x(0^+)=2312.798(11)$~keV [Nucl. Phys. A {\bf{523}}, 1 (1991)], provides a new determination of the superallowed $\beta$-decay $Q_{EC}$ value, $Q_{EC}(\text{sa}) = 2831.566(28)$ keV, with an order of magnitude improvement in precision, and a similar improvement to the calculated statistical rate function $f$. This is used to calculate an improved $\mathcal{F}t$-value of 3073.8(2.8) s., Comment: 5 pages, 5 figures

Using the Penning trap mass spectrometer TITAN, we performed the first direct mass measurements of 20,21Mg, isotopes that are the most proton-rich members of the A = 20 and A = 21 isospin multiplets. These measurements were possible through the use of a unique ion-guide laser ion source, a development that suppressed isobaric contamination by six orders of magnitude. Compared to the latest atomic mass evaluation, we find that the mass of 21Mg is in good agreement but that the mass of 20Mg deviates by 3{\sigma}. These measurements reduce the uncertainties in the masses of 20,21Mg by 15 and 22 times, respectively, resulting in a significant departure from the expected behavior of the isobaric multiplet mass equation in both the A = 20 and A = 21 multiplets. This presents a challenge to shell model calculations using either the isospin non-conserving USDA/B Hamiltonians or isospin non-conserving interactions based on chiral two- and three-nucleon forces., Comment: 5 pages, 2 figures

A new technique has been developed at TRIUMF's TITAN facility to perform in-trap decay spectroscopy. The aim of this technique is to eventually measure weak electron capture branching ratios (ECBRs) and by this to consequently determine GT matrix elements of $\beta\beta$ decaying nuclei. These branching ratios provide important input to the theoretical description of these decays. The feasibility and power of the technique is demonstrated by measuring the ECBR of $^{124}$Cs., Comment: 9 pages, 9 figures

Recent high-precision mass measurements of $^{9}$Li and $^{9}$Be, performed with the TITAN Penning trap at the TRIUMF ISAC facility, are analyzed in light of state-of-the-art shell model calculations. We find an explanation for the anomalous Isobaric Mass Multiplet Equation (IMME) behaviour for the two $A$ = 9 quartets. The presence of a cubic $d$ = 6.3(17) keV term for the $J^{\pi}$ = 3/2$^{-}$ quartet and the vanishing cubic term for the excited $J^{\pi}$ = 1/2$^{-}$ multiplet depend upon the presence of a nearby $T$ = 1/2 state in $^{9}$B and $^{9}$Be that induces isospin mixing. This is contrary to previous hypotheses involving purely Coulomb and charge-dependent effects. $T$ = 1/2 states have been observed near the calculated energy, above the $T$ = 3/2 state. However an experimental confirmation of their $J^{\pi}$ is needed., Comment: 5 pages, 2 figures

The use of highly charged ions increases the precision and resolving power, in particular for short-lived species produced at on-line radio-isotope beam facilities, achievable with Penning trap mass spectrometers. This increase in resolving power provides a new and unique access to resolving low-lying long-lived ($T_{1/2} > 50$ ms) nuclear isomers. Recently, the $111.19(22)$ keV (determined from $\gamma$-ray spectroscopy) isomeric state in $^{78}$Rb has been resolved from the ground state, in a charge state of $q=8+$ with the TITAN Penning trap at the TRIUMF-ISAC facility. The excitation energy of the isomer was measured to be $108.7(6.4)$ keV above the ground state. The extracted masses for both the ground and isomeric states, and their difference, agree with the AME2003 and Nuclear Data Sheet values. This proof of principle measurement demonstrates the feasibility of using Penning trap mass spectrometers coupled to charge breeders to study nuclear isomers and opens a new route for isomer searches., Comment: 8 pages, 6 figures

We present Penning-trap mass measurements of neutron-rich 44,47-50K and 49,50Ca isotopes carried out at the TITAN facility at TRIUMF-ISAC. The 44K mass measurement was performed with a charge-bred 4+ ion utilizing the TITAN EBIT, and agrees with the literature. The mass excesses obtained for 47K and 49,50Ca are more precise and agree with the values published in the 2003 Atomic Mass Evaluation (AME'03). The 48,49,50K mass excesses are more precise than the AME'03 values by more than one order of magnitude. For 48,49K, we find deviations by 7 sigma and 10 sigma, respectively. The new 49K mass excess lowers significantly the two-neutron separation energy at the neutron number N=30 compared with the separation energy calculated from the AME'03 mass-excess values, and thus, increases the N=28 neutron-shell gap energy at Z=19 by approximately 1 MeV., Comment: 6 pages, 5 figures, accepted for PRC

TITAN (TRIUMF's Ion Traps for Atomic and Nuclear science) is an online facility designed to carry out high-precision mass measurements on singly and highly charged radioactive ions. The TITAN Penning trap has been built and optimized in order to perform such measurements with an accuracy in the sub ppb-range. A detailed characterization of the TITAN Penning trap is presented and a new compensation method is derived and demonstrated, verifying the performance in the range of sub-ppb., Comment: 33 pages, 16 figures

Penning trap mass measurements of short-lived nuclides have been performed for the first time with highly-charged ions (HCI), using the TITAN facility at TRIUMF. Compared to singly-charged ions, this provides an improvement in experimental precision that scales with the charge state q. Neutron-deficient Rb-isotopes have been charge bred in an electron beam ion trap to q = 8 - 12+ prior to injection into the Penning trap. In combination with the Ramsey excitation scheme, this unique setup creating low energy, highly-charged ions at a radioactive beam facility opens the door to unrivalled precision with gains of 1-2 orders of magnitude. The method is particularly suited for short-lived nuclides such as the superallowed {\beta} emitter 74Rb (T1/2 = 65 ms). The determination of its atomic mass and an improved QEC-value are presented., Comment: 5 pages, 3 figures

We present a description of the Radio Frequency Quadrupole (RFQ) ion trap built as part of the TITAN facility. It consists of a gas-filled, segmented, linear Paul trap and is the first stage of the TITAN setup with the purpose of cooling and bunching radioactive ion beams delivered from ISAC-TRIUMF. This is the first such device to be driven digitally, i.e., using a high voltage ($V_{pp} = \rm{400 \, V}$), wide bandwidth ($0.2 < f < 1.2 \, \rm{MHz}$) square-wave as compared to the typical sinusoidal wave form. Results from the commissioning of the device as well as systematic studies with stable and radioactive ions are presented including efficiency measurements with stable $^{133}$Cs and radioactive $^{124, 126}$Cs. A novel and unique mode of operation of this device is also demonstrated where the cooled ion bunches are extracted in reverse mode, i.e., in the same direction as previously injected., Comment: 34 pages, 17 figures

The first direct mass-measurement of $^{6}$He has been performed with the TITAN Penning trap mass spectrometer at the ISAC facility. In addition, the mass of $^{8}$He was determined with improved precision over our previous measurement. The obtained masses are $m$($^{6}$He) = 6.018 885 883(57) u and $m$($^{8}$He) = 8.033 934 44(11) u. The $^{6}$He value shows a deviation from the literature of 4$\sigma$. With these new mass values and the previously measured atomic isotope shifts we obtain charge radii of 2.060(8) fm and 1.959(16) fm for $^{6}$He and $^{8}$He respectively. We present a detailed comparison to nuclear theory for $^6$He, including new hyperspherical harmonics results. A correlation plot of the point-proton radius with the two-neutron separation energy demonstrates clearly the importance of three-nucleon forces., Comment: 4 pages, 2 figures

In this letter, we report a new mass for $^{11}$Li using the trapping experiment TITAN at TRIUMF's ISAC facility. This is by far the shortest-lived nuclide, $t_{1/2} = 8.8 \rm{ms}$, for which a mass measurement has ever been performed with a Penning trap. Combined with our mass measurements of $^{8,9}$Li we derive a new two-neutron separation energy of 369.15(65) keV: a factor of seven more precise than the best previous value. This new value is a critical ingredient for the determination of the halo charge radius from isotope-shift measurements. We also report results from state-of-the-art atomic-physics calculations using the new mass and extract a new charge radius for $^{11}$Li. This result is a remarkable confluence of nuclear and atomic physics., Comment: Formatted for submission to PRL