Search

A segmented-scintillator-based implantation detector was developed to study the energy distribution of beta-delayed neutrons emitted from exotic isotopes. The detector comprises a 34 $\times$ 34 YSO scintillator coupled to an 8 $\times$ 8 Position-Sensitive Photo-Multiplier Tube (PSPMT) via a tapered light guide. The detector was used at RIBF, RIKEN, for time-of-flight-based neutron spectroscopy measurement in the $^{78}$Ni region. The detector provides the position and timing resolution necessary for ion-beta correlations and ToF measurements. The detector provides a high $\sim$ 80 $\%$ beta-detection efficiency and a sub-nanosecond timing resolution. This contribution discusses the details of the design, operation, implementation, and analysis developed to obtain neutron time-of-flight spectrum and the analysis methods in the context of neutron-rich nuclei in the $^{78}$Ni region.

Single-step Coulomb excitation of $^{46,48,49,50}$Ti is presented. A complete set of $E2$ matrix elements for the quintuplet of states in $^{49}$Ti, centered on the $2^+$ core excitation, was measured for the first time. A total of nine $E2$ matrix elements are reported, four of which were previously unknown. $^{49}_{22}$Ti$_{27}$ shows a $20\%$ quenching in electric quadrupole transition strength as compared to its semi-magic $^{50}_{22}$Ti$_{28}$ neighbour. This $20\%$ quenching, while empirically unprecedented, can be explained with a remarkably simple two-state mixing model, which is also consistent with other ground-state properties such as the magnetic dipole moment and electric quadrupole moment. A connection to nucleon transfer data and the quenching of single-particle strength is also demonstrated. The simplicity of the $^{49}$Ti-$^{50}$Ti pair (i.e., approximate single-$j$ $0f_{7/2}$ valence space and isolation of yrast states from non-yrast states) provides a unique opportunity to disentangle otherwise competing effects in the ground-state properties of atomic nuclei, the emergence of collectivity, and the role of proton-neutron interactions., Comment: 8 pages, 5 figures, accepted in Physics Letters B

$^{65}$Zn is a common calibration source, moreover used as a radioactive tracer in medical and biological studies. In many cases, $\gamma$-spectroscopy is a preferred method of $^{65}$Zn standardization, which relies directly on the branching ratio of $J \pi (^{65}\text{Zn} ) = 5/2^- \rightarrow J \pi (^{65}\text{Cu}) = 5/2^- $ via electron capture (EC*). We measure the relative intensity of this branch to that proceeding directly to the ground state (EC$^0$) using a novel coincidence technique, finding $I_{\text{EC}^0}/I_{\text{EC*}} = 0.9684 \pm 0.0018$. Re-evaluating the decay scheme of $^{65}$Zn by adopting the commonly evaluated branching ratio of $I_{\beta^+}= 1.4271(7)\%$ we obtain $I_{\text{EC*}} = (50.08 \pm 0.06)\%$, and $I_\text{EC^0} = (48.50 \pm 0.06) \%$. The associated 1115 keV gamma intensity agrees with the previously reported NNDC value, and is now accessible with a factor of ~2 increase in precision. Our re-evaluation removes reliance on the deduction of this gamma intensity from numerous measurements, some of which disagree and depend directly on total activity determination. The KDK experimental technique provides a new avenue for verification or updates to the decay scheme of $^{65}$Zn, and is applicable to other isotopes., Comment: Uses similar methodology to the 40K measurement by the KDK Collaboration (Stukel et al PRL 2023, arXiv:2211.10319; Hariasz et al PRC 2023, arXiv:2211.10343), as such there may be some similarity in figures and text

This whitepaper presents the research priorities decided on by attendees of the 2022 Town Meeting for Fundamental Symmetries, Neutrons and Neutrinos, which took place December 13-15, 2022 in Chapel Hill, NC, as part of the Nuclear Science Advisory Committee (NSAC) 2023 Long Range Planning process. A total of 275 scientists registered for the meeting. The whitepaper makes a number of explicit recommendations and justifies them in detail.

Excited-state spectroscopy from the first Facility for Rare Isotope Beams (FRIB) experiment is reported. A 24(2)-$\mu$s isomer was observed with the FRIB Decay Station initiator (FDSi) through a cascade of 224- and 401-keV $\gamma$ rays in coincidence with $^{32}\textrm{Na}$ nuclei. This is the only known microsecond isomer ($1{\text{ }\mu\text{s}}\leq T_{1/2} < 1\text{ ms}$) in the region. This nucleus is at the heart of the $N=20$ island of shape inversion and is at the crossroads of spherical shell-model, deformed shell-model, and ab initio theories. It can be represented as the coupling of a proton hole and neutron particle to $^{32}\textrm{Mg}$, $^{32}\textrm{Mg}+\pi^{-1} + \nu^{+1}$. This odd-odd coupling and isomer formation provides a sensitive measure of the underlying shape degrees of freedom of $^{32}\textrm{Mg}$, where the onset of spherical-to-deformed shape inversion begins with a low-lying deformed $2^+$ state at 885 keV and a low-lying shape-coexisting $0_2^+$ state at 1058 keV. We suggest two possible explanations for the 625-keV isomer in $^{32}$Na: a $6^-$ spherical shape isomer that decays by $E2$ or a $0^+$ deformed spin isomer that decays by $M2$. The present results and calculations are most consistent with the latter, indicating that the low-lying states are dominated by deformation., Comment: 7 pages, 5 figures, accepted by Physical Review Letters

This white paper was submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting in preparation for the next NSAC Long Range Plan. We advocate to support current and future theoretical and experimental searches for physics beyond the Standard Model using nuclear $\beta$ decay., Comment: 12 pages, 2 figures, White paper submitted to the 2022 Fundamental Symmetries, Neutrons, and Neutrinos (FSNN) Town Hall Meeting at the University of North Carolina Chapel Hill

Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissile fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS/TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2010, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states., Comment: Submitted to European Physical Journal A

Potassium-40 is a widespread isotope whose radioactivity impacts estimated geological ages spanning billions of years, nuclear structure theory, and subatomic rare-event searches - including those for dark matter and neutrinoless double-beta decay. The decays of this long-lived isotope must be precisely known for its use as a geochronometer, and to account for its presence in low-background experiments. There are several known decay modes for $^{40}$K, but a predicted electron-capture decay directly to the ground state of argon-40 has never been observed, while theoretical predictions span an order of magnitude. The KDK Collaboration reports on the first observation of this rare decay, obtained using a novel combination of a low-threshold X-ray detector surrounded by a tonne-scale, high-efficiency $\gamma$-ray tagger at Oak Ridge National Laboratory. A blinded analysis reveals a distinctly nonzero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_{\text{EC}^*}$) of $I_{\text{EC}^0} / I_{\text{EC}^*}=0.0095\stackrel{\text{stat}}{\pm}0.0022\stackrel{\text{sys}}{\pm}0.0010$ (68% CL), with the null hypothesis rejected at 4$\sigma$ [Stukel et al., DOI:10.1103/PhysRevLett.131.052503]. This unambiguous signal yields a branching ratio of $I_{\text{EC}^0}=0.098\%\stackrel{\text{stat}}{\pm}0.023\%\stackrel{\text{sys}}{\pm}0.010$, roughly half of the commonly used prediction. This first observation of a third-forbidden unique electron capture improves understanding of low-energy backgrounds in dark-matter searches and has implications for nuclear-structure calculations. A shell-model based theoretical estimate for the $0\nu\beta\beta$ decay half-life of calcium-48 is increased by a factor of $7^{+3}_{-2}$. Our nonzero measurement shifts geochronological ages by up to a percent; implications are illustrated for Earth and solar system chronologies., Comment: This is a companion submission to Stukel et al (KDK collaboration) "Rare $^{40}$K decay with implications for fundamental physics and geochronology" [arXiv:2211.10319; DOI: 10.1103/PhysRevLett.131.052503]. As such, both texts share some figures and portions of text. This version updates the text following its review and production process

Potassium-40 is a widespread, naturally occurring isotope whose radioactivity impacts subatomic rare-event searches, nuclear structure theory, and estimated geological ages. A predicted electron-capture decay directly to the ground state of argon-40 has never been observed. The KDK (potassium decay) collaboration reports strong evidence of this rare decay mode. A blinded analysis reveals a non-zero ratio of intensities of ground-state electron-captures ($I_{\text{EC}^0}$) over excited-state ones ($I_\text{EC*}$) of $ I_{\text{EC}^0} / I_\text{EC*} = 0.0095 \stackrel{\text{stat}}{\pm} 0.0022 \stackrel{\text{sys}}{\pm} 0.0010 $ (68% C.L.), with the null hypothesis rejected at 4$\sigma$. In terms of branching ratio, this signal yields $I_{\text{EC}^0} = 0.098\% \stackrel{\text{stat}}{\pm} 0.023\% \stackrel{\text{sys}}{\pm} 0.010\% $, roughly half of the commonly used prediction, with consequences for various fields [L. Hariasz et al., companion paper, DOI: 10.1103/PhysRevC.108.014327]., Comment: This is a companion paper to Hariasz et al (KDK collaboration) "Evidence for ground-state electron capture of ${}^{40}$K" [arXiv:2211.10343; DOI: 10.1103/PhysRevC.108.014327]. As such, both texts share some figures and portions of text. This version includes the journal DOI

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html., Comment: 96 pages, IAEA CRP report, preliminary version

Potassium-40 ($^{40}$K) is a long-lived, naturally occurring radioactive isotope. The decay products are prominent backgrounds for many rare event searches, including those involving NaI-based scintillators. $^{40}$K also plays a role in geochronological dating techniques. The branching ratio of the electron capture directly to the ground state of argon-40 has never been measured, which can cause difficulty in interpreting certain results or can lead to lack of precision depending on the field and analysis technique. The KDK (Potassium (K) Decay (DK)) collaboration is measuring this decay. A composite method has a silicon drift detector with an enriched, thermally deposited $^{40}$K source inside the Modular Total Absorption Spectrometer. This setup has been characterized in terms of energy calibration, gamma tagging efficiency, live time and false negatives and positives. A complementary, homogeneous, method is also discussed; it employs a KSr$_2$I$_5$:Eu scintillator as source and detector., Comment: 20 pages, 24 figures, Submitted to NIM A

The $^{15}$O($\alpha$,$\gamma$)$^{19}$Ne reaction is responsible for breakout from the hot CNO cycle in Type I x-ray bursts. Understanding the properties of resonances between $E_x = 4$ and 5 MeV in $^{19}$Ne is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2$^-$ and 7/2$^-$, respectively. Gamma-ray transitions from these states were studied using triton-$\gamma$-$\gamma$ coincidences from the $^{19}$F($^{3}$He,$t\gamma$)$^{19}$Ne reaction measured with GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the $J^\pi$ values are actually 7/2$^-$ and 9/2$^-$, respectively. These assignments are consistent with the values in the $^{19}$F mirror nucleus and in contrast to previously accepted assignments.

Detection of nuclear-decay $\gamma$ rays provides a sensitive thermometer of nova nucleosynthesis. The most intense $\gamma$-ray flux is thought to be annihilation radiation from the $\beta^+$ decay of $^{18}$F, which is destroyed prior to decay by the $^{18}$F($p$,$\alpha$)$^{15}$O reaction. Estimates of $^{18}$F production had been uncertain, however, because key near-threshold levels in the compound nucleus, $^{19}$Ne, had yet to be identified. This Letter reports the first measurement of the $^{19}$F($^{3}$He,$t\gamma$)$^{19}$Ne reaction, in which the placement of two long-sought 3/2$^+$ levels is suggested via triton-$\gamma$-$\gamma$ coincidences. The precise determination of their resonance energies reduces the upper limit of the rate by a factor of $1.5-17$ at nova temperatures and reduces the average uncertainty on the nova detection probability by a factor of 2.1., Comment: 6 pages, 4 figures

Many choices are available in order to evaluate large radioactive decay networks. %multi-particle decay data. There are many parameters that influence the calculated $\beta$-decay delayed single and multi-neutron emission branching fractions. We describe assumptions about the decay model, background, and other parameters and their influence on $\beta$-decay delayed multi-neutron emission analysis. An analysis technique, the ORNL BRIKEN analysis procedure, for determining $\beta$-delayed multi-neutron branching ratios in $\beta$-neutron precursors produced by means of heavy-ion fragmentation is presented. The technique is based on estimating the initial activities of zero, one, and two neutrons occurring in coincidence with an ion-implant and $\beta$ trigger. The technique allows one to extract $\beta$-delayed multi-neutron decay branching ratios measured with the hybrid \textsuperscript{3}He BRIKEN neutron counter. As an example, two analyses of the $\beta$-neutron emitter \textsuperscript{77}Cu based on different {\it a priori} assumptions are presented along with comparisons to literature values., Comment: 21 pages, 10 figures

Potassium-40 (${}^{40}$K) is a background in many rare-event searches and may well play a role in interpreting results from the DAMA dark-matter search. The electron-capture decay of ${}^{40}$K to the ground state of ${}^{40}$Ar has never been measured and contributes an unknown amount of background. The KDK (potassium decay) collaboration will measure this branching ratio using a ${}^{40}$K source, an X-ray detector, and the Modular Total Absorption Spectrometer at Oak Ridge National Laboratory., Comment: TAUP 2017 - XV International Conference on Topics in Astroparticle and Underground Physics