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We present a novel airborne imaging differential optical absorption spectroscopy (DOAS) instrument: the Ultraviolet Visible Hyperspectral Imaging Spectrometer (UVHIS), which is developed for trace gas monitoring and pollution mapping. Within a broad spectral range of 200 to 500 nm and operating in three channels, the spectral resolution of UVHIS is better than 0.5 nm. The optical design of each channel comprises a fore-optics with a field of view (FOV) of 40 ∘ , an Offner imaging spectrometer and a charge-coupled device (CCD) array detector of 1032×1072 pixels. A first demonstration flight using UVHIS was conducted on 23 June 2018, above an area of approximately 600 km2 in Feicheng, China, with a spatial resolution of about 25m×22 m. Measurements of nadir backscattered solar radiation of channel 3 are used to retrieve tropospheric vertical column densities (VCDs) of NO2 with a mean total error of 3.0×1015 moleccm-2. The UVHIS instrument clearly detected several emission plumes transporting from south to north, with a peak value of 3×1016 moleccm-2 in the dominant one. The UVHIS NO2 vertical columns are consistent with the ground-based mobile DOAS observations, with a correlation coefficient of 0.65 for all co-located measurements, a correlation coefficient of 0.86 for the co-located measurements that only circled the steel factory and a slight underestimation for the polluted observations. This study demonstrates the capability of UVHIS for NO2 local emission and transmission monitoring. [ABSTRACT FROM AUTHOR]

We present a novel airborne imaging differential optical absorption spectroscopy (DOAS) instrument: Ultraviolet Visible Hyperspectral Imaging Spectrometer (UVHIS), which is developed for trace gas monitoring and pollution mapping. Within a broad spectral range from 200 to 500 nm, operated in three channels, the spectral resolution of UVHIS is better than 0.5 nm. The optical design of each channel comprises a fore-optics with a field of view (FOV) of 40°, an Offner imaging spectrometer, and a charge-coupled device (CCD) array detector of 1032 × 1072 pixels. A first demonstration flight using UVHIS was undertaken on 23 June 2018, above an approximate 600 km2 area in Feicheng, China, with a spatial resolution of about 25 × 22 m2. Measurements of nadir backscattered solar radiation of channel 3 are used to retrieve vertical column densities (VCDs) of NO2 with a mean fitting error of 2.6 × 1015 molec cm−2. The UVHIS instrument clearly detected several emission plumes transporting from south to north, with a peak value of 3 × 1016 molec cm−2 in the dominant one. UVHIS NO2 vertical columns are well correlated with ground-based mobile DOAS observations, with a correlation coefficient of 0.65 for all co-located measurements, and a slight underestimation for polluted observations. This study demonstrates the capability of UVHIS for NO2 local emission and transmission monitoring. [ABSTRACT FROM AUTHOR]

The Environmental Trace Gases Monitoring Instrument (EMI) is a high-spectral-resolution payload onboard the latest pathfinder mission GaoFen-5, designed specifically for the monitoring of global atmospheric trace gas compositions and trends. This study describes a comparative analysis of the tropospheric nitrogen dioxide (NO2) columns over the North China Plain (NCP) from November 2018 to April 2019 based on EMI products. Validation of satellite products based on a cross-correlation analysis with data from four ground-based multi-axis differential optical absorption spectroscopy sites provided good correlation coefficients (r) ranging from 0.78 to 0.88. The distribution and monthly averaged tropospheric NO2 columns revealed high pollution exposure levels during winter (November–January) and a decrease from February onward in the NCP. Moreover, a typical pollution event was analyzed in detail in combination with wind field statistics. The results indicated that variations of NO2 concentrations in Beijing and Tianjin were highly correlated with the wind direction from 22.5–45.0 degrees west of south, especially during times of high NO2 amounts. These findings highlight that the EMI payload on the GaoFen-5 (GF-5) satellite is useful for remote sensing of regional and global NO2 detection. [ABSTRACT FROM AUTHOR]