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Across the physics disciplines, the 186Pb nucleus is the only known system, where the two first excited states, together with the ground state, form a triplet of zero-spin states assigned with prolate, oblate and spherical shapes. Here we report on a precision measurement where the properties of collective transitions in 186Pb were determined in a simultaneous in-beam γ-ray and electron spectroscopy experiment employing the recoil-decay tagging technique. The feeding of the 0+2 state and the interband 2+2→2+1 transition have been observed. We also present direct measurement of the energies of the electric monopole transitions from the excited 0+ states to the 0+ ground state. In contrast to the earlier understanding, the obtained reduced transition probability B(E2;2+1→0+2) value of 190(80) W.u., the transitional quadrupole moment |Qt(2+1→0+2)|=7.7(33) eb and intensity balance arguments provide evidence to reassign the 0+2 and 0+3 states with predominantly prolate and oblate shape, respectively. Our work demonstrates a step-up in experimental sensitivity and paves the way for systematic studies of electric monopole transitions in this region. These electric monopole transitions probe the nuclear volume in a unique manner and provide unexploited input for development of the next-generation energy density functional models. peerReviewed

Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-K isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of 2.8(5) ms and an excitation energy $\ge 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of 1.4(3) s and an excitation energy $\ge 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-K states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen–Cooper–Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods–Saxon potential. The most probable candidates for the configurations of K-isomeric states in Md nuclei are proposed. Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-$K$ isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of $2.8(5)$ ms and an excitation energy $\geq 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of $1.4(3)$ s and an excitation energy $\geq 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-$K$ states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen-Cooper-Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods-Saxon potential. The most probable candidates for the configurations of $K$-isomeric states in Md nuclei are proposed.

International audience; Prolate-oblate shape coexistence close to the ground state in the strongly-deformed proton-rich A≈120 nuclei is reported for the first time. One of the four reported bands in 119Cs, built on a 11/2− state at 670 keV, consists of nearly degenerate signature partners, and has properties which unequivocally indicate the strongly-coupled πh11/2[505]11/2− configuration associated with oblate shape. Together with the decoupled πh11/2[541]3/2− band built on the 11/2− prolate state at 110 keV, for which a half-life of T1/2=55(5)μs has been measured, the new bands bring evidence of shape coexistence at low spin in the proton-rich strongly deformed A≈120 nuclei, a phenomenon predicted since long time, but not yet observed. Calculations using the particle-number conserving cranked shell model and two dimensional tilted axis cranking covariant density functional theory support and well reproduce the observed oblate and prolate coexisting low-energy states in 119Cs.

The very neutron-deficient strongly deformed Cs 119 nucleus has been studied using the Ni 58 ( Zn 64 , 3 p ) reaction and the JUROGAM 3 γ -ray detector array coupled to the MARA recoil-mass separator setup. The excitation energies of all observed bands have been determined, spins and parities have been firmly assigned to most of the observed states. The previously known and the newly identified rotational bands have been extended to very high spin and excitation energy. The configurations of the observed bands are discussed using the particle number conserving cranked shell model. The present study establishes the largest set of rotational bands observed in the proton-rich A ≈ 120 mass region.

Using a fusion-evaporation reaction and a gas-filled recoil separator, an isomeric state [T12=83(8)μs] with a most likely spin and parity of 132+ has been identified in Th211. The isomeric state is mainly depopulated via a hindered internal M2 transition [B(M2)=0.0025(5) W.u.], but also a weak α-decay branch of 4(3)% was observed. The present observations fit well to the systematic pattern set by the previously identified states of the same spin and parity in this region of the nuclear chart.

Two new excited bands built on the πh11/2 configuration have been identified in Nd135 in addition to the known πh11/2 band. The energy spectra of the excited bands and the available electromagnetic transition probabilities are in good agreement with theoretical results obtained using quasiparticle-plus-triaxial-rotor model calculations. The properties of the bands identify them as tilted precession bands instead of wobbling bands. Our results give a new insight into the interpretation of the low-lying bands in odd-A mass nuclei, and can stimulate future studies to address the nuclear triaxiality.

The neutron-deficient gold (Z=79) isotopes in the vicinity of the neutron midshell N=104 provide prolific examples of shape coexistence and isomerism at low excitation energy. They can be probed via a number of different experimental techniques. In this study, two new isomeric states with half-lives of 294(7) and 373(9) ns have been observed in the neutron-deficient odd-odd nuclide Au178 (N=99) in an experiment at the RITU gas-filled separator at JYFL, Jyvaskyla. This result was achieved due to the use of a segmented planar germanium detector with a high efficiency at low energies. By applying the recoil-decay tagging technique, they were assigned to decay to two different long-lived α-decaying states in Au178.

Lifetime measurements in $$^{178}$$ 178 Pt with excited states de-exciting through $$\gamma $$ γ -ray transitions and internal electron conversions have been performed. Ionic charges were selected by the in-flight mass separator MARA and measured at the focal plane in coincidence with the $$4_1^+\rightarrow 2_1^+$$ 4 1 + → 2 1 + $$257\,$$ 257 keV $$\gamma $$ γ -ray transition detected using the JUROGAM 3 spectrometer. The resulting charge-state distributions were analysed using the differential decay curve method (DDCM) framework to obtain a lifetime value of 430(20) ps for the $$2_1^+$$ 2 1 + state. This work builds on a method that combines the charge plunger technique with the DDCM analysis. As an alternative analysis, ions were selected in coincidence with the $$^{178}$$ 178 Pt alpha decay ($$E_{\mathrm {alpha}} = 5.458(5)$$ E alpha = 5.458 ( 5 ) MeV) at the focal plane. Lifetime information was obtained by fitting a two-state Bateman equation to the decay curve with the lifetime of individual states defined by a single quadrupole moment. This yielded a lifetime value of 430(50) ps for the $$2_1^+$$ 2 1 + state, and 54(6) ps for the $$4_1^+$$ 4 1 + state. An analysis method based around the Bateman equation will become especially important when using the charge plunger method for the cases where utilising coincidences between prompt $$\gamma $$ γ rays and recoils is not feasible.

Fine structure in the α decay of Th90221, populating excited states in Ra88217, was studied using αγ-coincidence spectroscopy. Two α-decay branches from Th221 have been newly observed, with Eα(keV)[bα(%)]=7951(8)[0.14(3)] and 8247(3)[1.51(12)], together with three previously known branches. Also, two new states in Ra217 were identified at E = 177 and 227 keV. The ground-state configurations of the odd-A, N = 131 transitional isotones above Pb208 are interpreted from their α-decay fine structure systematics and considered in terms of predictions using spherical shell and reflection-asymmetric models.

Experimental signatures of moderately enhanced octupole correlations at high spin in 136 Nd are indicated for the first time. The extracted dipole moments of two negative-parity bands are only two times smaller than those of the lanthanide nuclei with N ≈ 90 which present well-established octupole correlations. Calculations using the cranked quasiparticle random phase approximation and a model of quadrupole-octupole rotations with octupole vibrations reveal the structure of the bands and the enhanced octupole correlations at high spin in 136 Nd .

The odd-Z Md251 nucleus was studied using combined γ-ray and conversion-electron in-beam spectroscopy. Besides the previously observed rotational band based on the [521]1/2− configuration, another rotational structure has been identified using γ-γ coincidences. The use of electron spectroscopy allowed the rotational bands to be observed over a larger rotational frequency range. Using the transition intensities that depend on the gyromagnetic factor, a [514]7/2− single-particle configuration has been inferred for this band, i.e., the ground-state band. A physical background that dominates the electron spectrum with an intensity of ≃60% was well reproduced by simulating a set of unresolved excited bands. Moreover, a detailed analysis of the intensity profile as a function of the angular momentum provided a method for deriving the orbital gyromagnetic factor, namely gK=0.69−0.16+0.19 for the ground-state band. The odd-Z Md249 was studied using γ-ray in-beam spectroscopy. Evidence for octupole correlations resulting from the mixing of the Δl=Δj=3 [521]3/2− and [633]7/2+ Nilsson orbitals were found in both Md249,251. A surprising similarity of the Md251 ground-state band transition energies with those of the excited band of Lr255 has been discussed in terms of identical bands. Skyrme-Hartree-Fock-Bogoliubov calculations were performed to investigate the origin of the similarities between these bands.

High-spin states of the odd–odd $${}^{194}$$ Bi nucleus have been studied by means of nuclear spectroscopy for the first time. Two low-lying rotational bands were observed. The positive-parity band built on a short-lived isomeric state 633 keV above the $$\alpha $$ and $$\beta $$ decaying long-lived (10 $$^-$$ ) state is assigned a $${\pi i_{13/2} \otimes \nu i_{13/2 }^{-1}}$$ configuration, while the other band is attributed to the $${\pi h_{9/2} \otimes \nu i_{13/2 }^{-1}}$$ configuration. Both of these bands are assumed to have oblate shape. Three band-like structures composed predominantly of $$\Delta I = 1$$ transitions were also found. One of the shears band candidates is firmly linked to the lower lying level structures whereas for the other two links to lower-lying structures remain missing.

Rotational structures have been measured using the Jurogam II and GAMMASPHERE arrays at low spin following the Gd155(α,2n)Dy157 and Nd148(C12,5n)Dy155 reactions at 25 and 65 MeV, respectively. We report high-K bands, which are conjectured to be the first candidates of a Kπ=2+γ vibrational band, built on the [505]11/2− neutron orbital, in both odd-ADy155,157 isotopes. The coupling of the first excited K=0+ states or the so-called β vibrational bands at 661 and 676 keV in Dy154 and Dy156 to the [505]11/2− orbital, to produce a Kπ=11/2− band, was not observed in both Dy155 and Dy157, respectively. The implication of these findings on the interpretation of the first excited 0+ states in the core nuclei Dy154 and Dy156 are also discussed.

Evaluated nuclear structure and decay data for all nuclei with mass number A=188 (Lu, Hf, Ta, W, Re, Os, Ir, Pt, Au, Hg, Tl, Pb, Bi, Po) are presented. The experimental data are compiled and evaluated, and best values for level and gamma-ray energies, quantum numbers, lifetimes, gamma-ray intensities, and other nuclear properties are recommended. Inconsistencies and discrepancies that exist in the literature are noted. This work supersedes the earlier evaluation by Balraj Singh (2002Si10), published in Nuclear Data Sheets 95, 387 (2002). The gamma-ray transition probabilities were calculated using the ENSDF analysis program ruler ( www-nds.iaea.org/public/ensdf_pgm/ ). However, the reader should be warned that the program may produce incorrect results when dealing with non-symmetric uncertainties.

The mean lifetimes of the lowest energy 2(+), 8(+) and 9(-) states in Os-166 have been measured using the recoil distance Doppler-shift method in conjunction with a selective recoil-decay tagging t ...

The quenching of the experimental spectroscopic factor for proton emission from the short-lived $d_{3/2}$ isomeric state in $^{151m}$Lu was a long-standing problem. In the present work, proton emission from this isomer has been reinvestigated in an experiment at the Accelerator Laboratory of the University of Jyv\"{a}skyl\"{a}. The proton-decay energy and half-life of this isomer were measured to be 1295(5) keV and 15.4(8) $\mu$s, respectively, in agreement with another recent study. These new experimental data can resolve the discrepancy in the spectroscopic factor calculated using the spherical WKB approximation. Using the R-matrix approach it is found that the proton formation probability indicates no significant hindrance for the proton decay of $^{151m}$Lu., Comment: 6 pages, 5 figures

Decay spectroscopy of No250 has been performed using digital electronics and pulse-shape analysis of the fast nuclear decays for the first time. Previous studies of No250 reported two distinct fission decay lifetimes, related to the direct fission of the ground state and to the decay of an isomeric state but without the possibility to determine if the isomeric state decayed directly via fission or via internal electromagnetic transitions to the ground state. The data obtained in the current experiment allowed the puzzle to finally be resolved, attributing the shorter half-life of t1/2=3.8±0.3μs to the ground state and the longer half-life t1/2=34.9−3.2+3.9μs to the decay of an isomeric state. No250 becomes, thus, one of a very few examples of very heavy nuclei with an isomeric state living considerably longer than its ground state. This phenomenon has important consequences for the nuclear-structure models aiming to determine the borders of the island of stability of superheavy elements.

High-spin states in the N = 128 nucleus 218Th have been investigated following fusion–evaporation reactions, using the recoil-decay tagging technique. Due to the short-lived nature of the ground state of 218Th prompt γ rays have been correlated with the α decay of the daughter nucleus 214Ra. The level scheme representing the decay of excited states has been extended to (16+) with the observation of six previously unreported transitions. The observations are compared with the results of shell model calculations and within the context of the systematics of neighbouring nuclei.

Two new bands have been identified in $^{137}$Nd from a high-statistics JUROGAM II gamma-ray spectroscopy experiment. Constrained density functional theory and particle rotor model calculations are used to assign configurations and investigate the band properties, which are well described and understood. It is demonstrated that these two new bands can be interpreted as chiral partners of previously known three-quasiparticle positive- and negative-parity bands. The newly observed chiral doublet bands in $^{137}$Nd represent an important support to the existence of multiple chiral bands in nuclei. The present results constitute the missing stone in the series of Nd nuclei showing multiple chiral bands, which becomes the most extended sequence of odd–even and even-even nuclei presenting multiple chiral bands in the Segré chart. Two new bands have been identified in $^{137}$Nd from a high-statistics JUROGAM II gamma-ray spectroscopy experiment. Constrained density functional theory and particle rotor model calculations are used to assign configurations and investigate the band properties, which are well described and understood. It is demonstrated that these two new bands can be interpreted as chiral partners of previously known three-quasiparticle positive- and negative-parity bands. The newly observed chiral doublet bands in $^{137}$Nd represent an important support to the existence of multiple chiral bands in nuclei. The present results constitute the missing stone in the series of Nd nuclei showing multiple chiral bands, which becomes the most extended sequence of nuclei presenting multiple chiral bands in the Segr\'e chart.

The extremely neutron-deficient isotopes 177,179Au were studied by means of in-beam ?-ray spectroscopy. Specific tagging techniques, ?-decay tagging in 177Au and isomer tagging in 179Au, were used for these studies. Feeding of positive-parity, nearly spherical states, which are associated with 2d3/2 and 3s1/2 proton-hole configurations, from the 1i13/2 proton-intruder configuration was observed in 177Au. Such a decay path has no precedent in odd-Au isotopes and it is explained by the effect of mixing of wave functions of the initial state. © 2020, 262010 2/0129/17 Science and Technology Facilities Council, STFC European Research Council, ERC: 203481 Academy of Finland: 131665 Agentúra na Podporu V?skumu a V?voja, APVV: APVV-15-0225, The authors express their gratitude to the staff of the Accelerator Laboratory at the University of Jyväskylä for their excellent technical support. This work has been supported by the EU-FP7-IA project ENSAR (No. 262010 ), the Academy of Finland (CoE in Nuclear and Accelerator Based Physics, grant to T.G., Contract No. 131665 ), the European Research Council through the project SHESTRUCT (Grant Agreement No. 203481 ), the UK Science and Technology Facilities Council , the Slovak Research and Development Agency under Contract No. APVV-15-0225 , and the Slovak Grant Agency VEGA (Contract No. 2/0129/17 ).

Excited states in the extremely neutron-deficient nucleus $$^{172}{\mathrm {Pt}}$$172Pt were populated via $$^{96}\mathrm {Ru}(^{78}\mathrm {Kr},2p)$$96Ru(78Kr,2p) and $$^{92}\mathrm {Mo}(^{83}\mathrm {Kr},3n)$$92Mo(83Kr,3n) reactions. The level scheme has been extended up to an excitation energy of $$\approx 5~\hbox {MeV}$$≈5MeV and tentative spin-parity assignments up to $$I^\pi = 18^+$$Iπ=18+. Linear polarization and angular distribution measurements were used to determine the electromagnetic E1 character of the dipole transitions connecting the positive-parity ground-state band with an excited side-band, firmly establishing it as a negative-parity band. The lowest member of this negative-parity structure was firmly assigned spin-parity $$3^-$$3-. In addition, we observed an E3 transition from this $$3^-$$3- state to the ground state, providing direct evidence for octupole collectivity in $$^{172}{\mathrm {Pt}}$$172Pt. Large-scale shell model (LSSM) and total Routhian surface (TRS) calculations have been performed, supporting the interpretation of the $$3^-$$3- state as a collective octupole-vibrational state.

© 2019 American Physical Society. An analysis technique has been developed in order to mitigate energy summing due to sequential short-lived α decays from nuclei implanted into a silicon detector. Using this technique, α-decay spectroscopy of the N=130 isotones Ra218 (Z=88) and Th220 (Z=90) has been performed. The energies of the α particles emitted in the Ra218→Rn214 and Th220→Ra216 ground-state-to-ground-state decays have been measured to be 8381(4) keV and 8818(13) keV, respectively. The half-lives of the ground states of Ra218 and Th220 have been measured to be 25.99(10) μs and 10.4(4) μs, respectively. The half-lives of the ground states of the α-decay daughters, Rn214 and Ra216, have been measured to be 259(3) ns and 161(11) ns, respectively. Fine structure in the α decay of Ra218 has been observed for the first time, populating the 695-keV 21+ state in Rn214. The fine-structure α decay has an α-particle energy of 7715(40) keV and branching ratio bα=0.123(11)%.

CITATION: Majola, S. N. T. et al. 2019. β and γ bands in N=88, 90, and 92 isotones investigated with a five-dimensional collective Hamiltonian based on covariant density functional theory: Vibrations, shape coexistence, and superdeformation. Physical Review C, 100(4). doi:10.1103/PhysRevC.100.044324.

CITATION: Majola, S. N. T., et al. 2019. Spectroscopy of low-spin states in 157Dy : Search for evidence of enhanced octupole correlations. Physical Review C, 100(6):034322, doi:10.1103/PhysRevC.100.034322.

Lifetime measurements of excited states in Hg-178 have been performed using the Rh-103(Kr-78, p2n) reaction at a beam energy of 354 MeV. The recoil-decay tagging (RDT) technique was applied to select the Hg-178 nuclei and associate the prompt gamma rays with the correlated characteristic ground-state alpha decay. Lifetimes of the four lowest yrast states of Hg-178 have been determined using the recoil distance Doppler-shift (RDDS) method. The experimental data are compared to theoretical predictions with focus on shape coexistence. The results confirm the shift of the deformed prolate structures to higher lying states but also indicate their increasing deformation with decreasing neutron number.

In the study of the odd-$Z$, even-$N$ nuclei $^{243}$Es and $^{249}$Md, performed at the University of Jyv\"askyl\"a, the fusion-evaporation reactions $^{197}$Au($^{48}$Ca,2$n$)$^{243}$Es and $^{203}$Tl($^{48}$Ca,2$n$)$^{249}$Md have been used for the first time. Fusion-evaporation residues were selected and detected using the RITU gas-filled separator coupled with the focal-plane spectrometer GREAT. For $^{243}$Es, the recoil decay correlation analysis yielded a half-life of $24 \pm 3$s, and a maximum production cross section of $37 \pm 10$ nb. In the same way, a half-life of $26 \pm 1$ s, an $\alpha$ branching ratio of 75 $\pm$ 5%, and a maximum production cross section of 300 $\pm$ 80 nb were determined for $^{249}$Md. The decay properties of $^{245}$Es, the daughter of $^{249}$Md, were also measured: an $\alpha$ branching ratio of 54 $\pm$ 7% and a half-life of 65 $\pm$ 6 s. Experimental cross sections were compared to the results of calculations performed using the KEWPIE2 statistical fusion-evaporation code.