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A recent experimental campaign performed at the LOHENGRIN spectrometer at ILL aimed at measuring the independent fission yield of 136Cs in the 239Pu(nth,f) reaction. This nuclide can have an important contribution to the total dose rate coming from spent light water reactor UOX and MOX fuels. Moreover, its impact is of first order on the uncertainty of the total dose rate calculated in specific areas of Nuclear Power Plants within accidental conditions. One of the most important sources of uncertainty is its independent fission yield. Therefore, a new measurement of its independent yield along with a rigorous uncertainty analysis was performed. Due to its low independent yield, a new measurement technique has been applied. Ions recoiling from neutron-irradiated 239Pu target were collected by implantation into an Al foil placed inside a vacuum chamber. This foil was then transferred to a low γ-ray background setup located at nearby laboratory (LPSC). The procedure was then repeated for different LOHENGRIN settings. Compared to the JEFF-3.1.1 library, a decrease of the fission yield of 136Cs with a reduced uncertainty is obtained.

The VElocity foR Direct particle Identification spectrometer (VERDI) is a 2E-2v fission spectrometer that allows the measurement of the total mass distribution of secondary fission fragments with a resolving power of 1-2 u. It consists of two time-of-flight (ToF) arms, with one Micro Channel Plate (MCP) detector and up to 32 Silicon PIPS (Passive Implanted Planar Silicon) detectors per arm. The MCPs provide the start timing signals and the PIPS detectors provide both the energy and the stopping ToF signals. In real conditions, the PIPS signals are affected by the formation of plasma from the interaction between the heavy ions and the detector material. The plasma contributes to a reduction in signal amplitude, resulting in a Pulse Height Defect (PHD), and introduces a signal delay, known as Plasma Delay Time (PDT). An experiment to characterize the PDT and PHD was performed at the LOHENGRIN recoil separator of the Institut Laue Langevin (ILL). Characteristic fission fragments from the 239Pu(n,f) reaction were separated based on their A/Q and E/Q ratios, allowing the measurement of a wide range of energies from 21 to 110 MeV and masses between 80 and 149 u. Six PIPS detectors were characterized to study their individual responses to the PDT and PHD effects. The signals were recorded in a digital acquisition system to completely exploit the offline analysis capabilities. Achieved combined timing and energy resolutions for fission fragments varied between 72(2) ps and 100(4) ps and 1.4% - 2% (FWHM), respectively. Preliminary PHD and PDT data are presented from the masses A=85, 95, 130 and 143. The PHD trends are strongly correlated with both the ion energy and mass. The PDT, on the other hand, shows a strong variation as a function of the ion kinetic energy but a smaller dependence on the ion mass.

Despite the numerous theoretical and experimental works published very recently, the way in which fission fragments acquire their angular momentum is still an open question. This angular momentum generation mechanism is important not only for improving our understanding of the fission process, but also for nuclear energy applications, since the angular momentum of fission fragments strongly impact the prompt gamma spectra and consequently the decay heat in a reactor. In this context, within the framework of a collaboration between the ‘Laboratoire de Physique Subatomique et Corpusculaire’ (LPSC, France), the ‘Institut Laue Langevin’ (ILL, France) and the CEA-Cadarache (France), an experimental program was developed on the LO-HENGRIN mass-spectrometer with the aim of measuring isomeric ratio of some fission products for different thermal-neutron-induced fission reactions. This paper will be focused on the results obtained for the spherical nucleus 132Sn following thermal-neutron-induced fission of both 235U and 241Pu targets. To further challenge the angular momentum generation models, 132Sn isomeric ratio (IR) was measured as a function of 132Sn fission product kinetic energy (KE). The angular momentum was determined by combining our experimental data with the calculations performed with the FIFRELIN Monte Carlo code. A clear angular momentum decrease with KE was observed for both reactions. Lastly, we investigate the dependence of the 132Sn angular momentum with the incident neutron energy, from thermal region up to 5 MeV (below the second-chance fission). For that, the four free available parameters in FIFRELIN are selected in order to reproduce the average prompt neutron multiplicity. In this way, the angular momentum is deduced for each neutron energy. These results are discussed in terms of the impact of the available intrinsic excitation energy at scission on the spin generation mechanism.

During an experimental campaign performed at the LOHENGRIN recoil spectrometer of the Institut Laue-Langevin (ILL), a kinetic energy dependence of 132Sn fission product isomeric ratio (IR) has been measured by inducing thermal fission of 241Pu. The IRs are deduced using gamma ray spectrometry in coincidence with the ionisation chamber. To interpret these data, we use the FIFRELIN Monte-Carlo code to simulate the de-excitation of the fission fragments. Combining the IRs with the FIFRELIN calculations, the angular momentum distribution with kinetic energy of the doubly magic nucleus of 132Sn was deduced. This will be compared with the angular momentum distribution obtained for the reaction 235U(nth,f) for 132Sn.

Delayed-neutron (DN) data is essential in inherent reactor safety and reactor control since it is needed for the estimation of the reactivity. Nowadays, discrepancies among the data in various international databases (JEFF, ENDF, JENDL) are large and bring excessive conservatism in the safety margins. The ALDEN (Average Lifetime of DElayed Neutrons) experiment, built in a collaboration between CEA and CNRS, aimed at re-measuring the DN data associated with several fissioning systems (average delayed-neutron yield and kinetic parameters). The first experimental campaign consisted in the integral measurement of the DN activity after the irradiation of an 235U target. It took place under the cold neutron flux of ILL (Institut Laue-Langevin) at the beginning of September 2018, in the PF1b experimental zone (doi:10.1016/j.nima.2006.03.020). The data analysis gave an average DN yield of 1.631E-02(2) DN/fiss and a mean precursors’ half-life of 8.93(9) s. The results are consistent with the literature, but they are affected by one third of the uncertainty.

The recently published article [1] claims to reach quantitative conclusions from a collaborative experiment dedicated to the study of the 7Be(n,α)α reaction. The Authors of this Comment who were collaborators in the experi-ment categorically reject the conclusions therein.

The evolution of the deformation across the Y isotopic chain, in the vicinity of N = 60 boundary, has been studied using gamma spectroscopy methods. The nuclei of interest have been produced by neutron induced fission of 235U and 241Pu targets, during two experimental campaigns named EXILL and FIPPS at the Institute Laue-Langevin in Grenoble. The emitted gamma rays have been collected by HPGe and LaBr3 detectors providing the identification of the high-spin levels in the 94Y and 96Y isotopes up to 6 MeV excitation energy, as well as information about the half-lives of the in-band states in the 98Y nucleus. The obtained results shed new light on the onset of deformation in the neutron-rich Y isotopes and, in general, in the A ≈ 100 region.

Radiative capture reactions on rare targets and prompt spectroscopy of neutron-rich nuclei produced in the neutron-capture induced-fission of 235U and 241Pu have been performed at the Institut Laue-Langevin (ILL). The high efficiency germanium (Ge) EXOGAM array has been used, complemented with Ge detectors from GASP and the ILL. LaBr3 detectors from the FATIMA collaboration have also been coupled to EXOGAM to measure lifetimes of lowlying excited states. The measured characteristics indicate very good performances of the overall setup. Some recent results will be discussed.

FIPPS is the new nuclear physics instrument of ILL for the spectroscopy of nuclei produced in neutron-induced reactions. The performance of the first implementation of the setup will be shown, together with an overview of the first experimental campaign (December 2016-March 2017). Future perspectives and physics opportunities will then be discussed.

The γ-coincidence studies of low-spin structures of 210Bi and 206Tl are presented. The 210Bi nucleus, populated in thermal neutron capture reaction, was investigated using EXILL HPGe array at Institut Laue-Langevin in Grenoble. The experimental results were compared to the shell-model calculations allowing to draw the conclusions on the nature of the low-spin excitations populated below the neutron binding energy in 210Bi (4.6 MeV). It has been found that some levels cannot be described by the valence proton and neutron couplings, but may arise from couplings of valence particles to the 3- octupole phonon of the doubly magic 208Pb core. Moreover, preliminary results of a low-spin structure measurements of 206Tl by the γ-coincidence technique, making use of the 205Tl(n,γ)206Tl reaction at the FIPPS prompt γ-ray spectroscopy facility of ILL are shown. The population of a large number of excited states of 206Tl above the ground state up to the neutron binding energy (at 6.5 MeV), within a few units of spin is expected. The analysis involving double and triple γ-coincidences and γγ-angular correlations will allow to significantly extend the experimental information on the energy and spin-parity of the levels in 206Tl. This will help shedding light on the proton-hole and neutron-hole couplings near the doubly magic core 208Pb.

Nuclei in the neutron-rich region beyond 132Sn have been produced recently by various experiments using fission. Using isomer and β-decay studies nuclear structure data has been collected on the orbital evolution and collectivity in the region with both the increase of proton and neutron numbers. Examples on particular questions related to the g.s. of the A=136 odd-odd 136Sb nucleus and its heavier neighbours are given in the scope of expectations by shell-model theory.

Nuclear fission yields data measurements for thermal neutron induced fission of 241Pu have been carried out at the Institut Laue Langevin (ILL) in Grenoble, using the Lohengrin mass spectrometer. Mass, isotopic and isomeric yields have been extracted for the last measurements. A focus is given in this document to the mass yield results which are obtained for almost the entire heavy peak and most of the light high yields masses, along with the covariance matrix. The mean kinetic energy as a function of the fission product mass has also been extracted from the measurements. The total mean kinetic energy pre and post neutron emission have been assessed and compared to other works showing a rather good agreement.

In recent experiments, the new concept of calorimetric low-temperature detectors (CLTDs) was applied for the first time for the investigation of isotopic yields of fission fragments. Fragments from neutron-induced fission sources were mass-separated by the LOHENGRIN spectrometer at the ILL Grenoble and, after passing silicon nitride membranes used as degraders, detected in a CLTD array. The new detector concept of a thermal detector provides a fundamental advantage over conventional ionization-mediated detectors, in particular for heavier particle masses at low energies. Using fissile targets of 235U, 239Pu and 241Pu, nuclear-charge separation was studied in the mass region 82 ≤ A ≤ 139. For light fragments, the Z resolution matches historically best values with conventional techniques, while for heavier masses substantial improvement was attained. We have gained first LOHENGRIN data on the isotopic yields in the light-mass group of 241Pu. Towards mass-symmetry, known Z-yield data were supplemented in the range A = 110 to 113 for 241Pu and 239Pu. Extended data sets were cumulated for A = 92 and 96 due to a recent request from studies on the reactor anti-neutrino spectrum. Furthermore, considerable progress was achieved to extend isotopic yield measurements up to the heavy-mass region, hardly accessible until now.

Fission yields are essential for nuclear reactor studies (decay heat, fuel inventory…) and constitute also one of the main observables needed to improve our understanding of the fission process. The symmetric mass region is of particular interest due to various intriguing properties of the fission fragments already reported in the literature : inversion of the nuclear charge polarization, large width of the fission fragment kinetic energy distribution, strong change of the prompt neutron multiplicity, etc. Recently, measurements of fission yields and kinetic energy distributions in the symmetric mass region were achieved at the LOHENGRIN mass spectrometer of the Institut Laue-Langevin (ILL). This experimental work is challenging due to the low counting rate and the appearance of contaminant masses, leading to pronounced components in the fission fragment kinetic energy distribution. Despite removing the undesirable contributions, the fission fragment kinetic energy distributions still show two components, indicating that the fission process could be modal. To go further and better characterize these components a comparison between our experimental data and Monte Carlo calculations (FIFRELIN code) simulating the de-excitation of the fission fragments for different fission channels will be presented and discussed.

A large array of Ge detectors installed at ILL, around a 235U target irradiated with cold neutrons, (EXILL) allowed measurement of prompt gamma-ray cascades occurring in fission fragments with an unambiguous determination of fragments. Here we present preliminary results of a systematic comparison between experimental γ-ray intensities and those obtained from the Monte-Carlo simulation code FIFRELIN, which is dedicated to the de-excitation of fission fragments. Major γ-ray intensities in the 142Ba and 92Kr fission products, extracted from EXILL data, were compared to FIFRELIN, as well as to reported values (when available) obtained with EUROGAM2 in the spontaneous fission of 248Cm. The evolution of γ-ray intensities in 92Kr versus the complementary partner in fission (i.e. versus the total number of evaporated neutrons by the fission pair) was then extracted and compared to FIFRELIN.

We have developed a new setup to measure prompt γ-rays from the 235U(nth,f) reaction. The setup consists of two multi-wire proportional counters (MWPCs) to detect the fission fragments, two LaBr3(Ce) scintillators to measure the γ-rays. The highly efficient setup was installed at the PF1B beam line of the Institut Laue Langevin (ILL). We have successfully measured the γ-ray spectrum up to about 20 MeV for the fist time in neutron-induced fission.

The mixing ratio of the main 320-keV, M1 + E2 ground-state γ transition in 210Bi has been more precisely quantified, allowing a significant reduction in the uncertainty of measurements of the neutron-capture cross section to the ground state of 210Bi from 25% to 0.9%. Accurate values for neutron-capture cross sections to both the ground and long-lived 9− isomeric state at 271 keV in 210Bi are of particular importance as Pb-Bi finds increased usage in Accelerator Driven Systems.

The huge neutron fluxes offer the possibility to use research reactors to produce isotopes of interest, which can be investigated afterwards. An example is the half-lives of long-lived isotopes like 129I. A direct usage of reactor neutrons in the astrophysical energy regime is only possible, if the corresponding ions are not at rest in the laboratory frame. The combination of an ion storage ring with a reactor and a neutron guide could open the path to direct measurements of neutron-induced cross sections on short-lived radioactive isotopes in the astrophysically interesting energy regime.