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Active control of chirality in artificial media such as metamaterials is fundamental in many scientific areas, ranging from research into fundamental optical phenomena to the investigation of novel materials, spectroscopy, and imaging. Precise control of the light polarization states has great importance for light‐matter interaction in chemistry and biology, as media with diverse chiral properties react differently to the incoming polarization of light. In this work an active double layer metamaterial device based on vertically stacked ring resonators is realized by integrating electrostatically tunable graphene as an active element. The device is characterized with a THz time domain spectroscopic system demonstrating an all‐electrical control of circular dichroism and optical activity at ≈2 THz, reporting a tunable ellipticity of 0.55–0.98 and >20° rotation of the plane polarization, respectively, by modifying the conductivity of graphene. Further integration with a narrow frequency quantum cascade laser emitting at ≈1.9 THz, in a crossed polarizer experimental arrangement, realizes an active amplitude modulator, hence highlighting the versatility of this approach. These results represent an important milestone for the investigation of novel concepts in optics and in several applications in the THz range, such as wireless communications and spectroscopy. [ABSTRACT FROM AUTHOR]

Photonic engineering of the terahertz emission from a quantum cascade laser (QCL) is fundamental for the exploitation of this unique source in a myriad of applications where it can be implemented, such as spectroscopy, imaging, and sensing. Active control of the frequency, power, polarization, and beam profile has been achieved through a variety of approaches. In particular, the active control of the emitted frequency, which is difficult to determine a priori, has been achieved through the integration of a photonic structure and/or by using external cavity arrangements. In this work, an external cavity arrangement, which implements a metamaterial/graphene optoelectronic mirror as an external feedback element, is proposed and demonstrated. The reflectivity and dispersion properties of the external active mirror were tuned via electrostatically gating graphene. It was possible to electronically reproduce the mode-switch occurring in a QCL emitting ∼2.8 THz by mechanically changing the external cavity length formed by an Au mirror. The external cavity arrangement was investigated and described in the framework of the self-mixing theory. These results open a way for the all-electronic engineering of the QCL emission by the use of a fast reconfigurable external mirror. This approach can uniquely address both power and frequency control, with ∼100 MHz reconfiguration speeds, using an integrated external element. Furthermore, the metamaterial/graphene mirror's strong dispersive properties might be implemented for the active mode locking of THz QCLs. Finally, this approach offers a unique opportunity to study the laser dynamics and mode competition in THz QCLs in the self-mixing feedback regime. [ABSTRACT FROM AUTHOR]

A terahertz (THz) imaging scheme based on the effect of self-mixing in a 2.9 THz quantum cascade (QC) amplifier has been demonstrated. By coupling an antireflective-coated silicon lens to the facet of a QC laser, with no external optical feedback, the laser mirror losses are enhanced to fully suppress lasing action, creating a THz QC amplifier. The addition of reflection from an external target to the amplifier creates enough optical feedback to initiate lasing action and the resulting emission enhances photon-assisted transport, which in turn reduces the voltage across the device. At the peak gain point, the maximum photon density coupled back leads to a prominent self-mixing effect in the QC amplifier, leading to a high sensitivity, with a signal to noise ratio up to 55 dB, along with a fast data acquisition speed of 20 000 points per second. [ABSTRACT FROM AUTHOR]

We present the realization of a quantum cascade laser emitting at around 2.85 THz, based on a hybrid plasmonic waveguide with a low refractive index dielectric cladding. This hybrid waveguide design allows the performance of a double-metal waveguide to be retained, while improving the emission far-field. A set of lasers based on the same active region material were fabricated with different metal layer thicknesses. A detailed characterization of the performance of these lasers revealed that there is an optimal trade-off that yields the best far-field emission and the maximum temperature of operation. By exploiting the pure plasmonic mode of these waveguides, the standard operation conditions of a double-metal quantum cascade laser were retrieved, such that the maximum operating temperature of these devices is not affected by the process. These results pave the way to realizing a class of integrated devices working in the terahertz range which could be further exploited to fabricate terahertz on-chip circuitry. [ABSTRACT FROM AUTHOR]

Terahertz (THz) spectroscopy and imaging have been heralded for some time as potentially revolutionary techniques for biomedical applications. Label-free detection of molecules and recognition of molecular events are often mentioned as the most exciting possibilities. A crucial practical goal, however, is the ability to perform such measurements on tiny amounts of biological fluids or even on individual organic structures. Living cells, for instance, have diameters at most of some tens of micrometers, i.e. at least λ/10 even for few-THz radiation. Furthermore, all analyses relevant for a biological perspective must be performed in a water environment, which presents a strong absorption across the whole THz spectral range, severely limiting the penetration of the electromagnetic field. Here, it is shown how both issues can be overcome with a lab-on-a-chip approach based on a microfluidic platform coupled to a plasmonic antenna. Using a quantum cascade laser as THz illumination source, liquid volumes down to the picoliter range are probed, and direct operation on individual 10-µm diameter microparticles flowing in water is shown. The present demonstration opens the way to the development of THz biosensing of individual living cells and small probe volumes. [ABSTRACT FROM AUTHOR]

The integration of quantum cascade lasers with devices capable of efficiently manipulating terahertz light represents a fundamental step for many different applications. Split-ring resonators, subwavelength metamaterial elements exhibiting broad resonances that are easily tuned lithographically, represent the ideal route to achieve such optical control of the incident light. We have realized a design based on the interplay between metallic split rings and the electronic properties of a graphene monolayer integrated into a single device. By acting on the doping level of graphene, an active modulation of the optical intensity was achieved in the frequency range between 2.2 and 3.1 THz, with a maximum modulation depth of 18%. [ABSTRACT FROM AUTHOR]