Search

Metamorphic InAs/In0.15Ga0.85As and InAs/In0.31Ga0.69As quantum dot (QD) arrays are known to be photosensitive in the telecommunication ranges at 1.3 and 1.55 μm, respectively; however, for photonic applications of these nanostructures, the effect of levels related to defects still needs in-depth investigation. We have focused on the influence of electron traps of defects on photocurrent (PC) in the plane of the QD array, studying by PC and deep level thermally stimulated current spectroscopy together with HRTEM and theoretical modeling. In the structures, a rich spectrum of electron trap levels of point defects EL6 (Ec − 0.37 eV), EL7 (0.29–0.30 eV), EL8 (0.27 eV), EL9/M2 (0.22–0.23 eV), EL10/M1 (0.16 eV), M0 (∼0.11 eV) and three extended defects ED1/EL3 (0.52–0.54), ED2/EL4 (0.47–0.48 eV), ED3/EL5 (0.42–0.43 eV) has been identified. Among them, new defect levels undiscovered earlier in InAs/InGaAs nanostructures has been detected, in particular, EL8 and M0. The found electron traps are shown to affect a time-dependent PC at low temperatures. Besides a long-term kinetics due to trap charging, a prolonged PC decrement versus time is measured under constant illumination. The decrement is interpreted to be related to a Coulomb screening of the conductivity channel by the electrons captured in the QD interface traps. The decrement is well fitted by allometric exponents, which means many types of traps involved in electron capturing. This study provides new findings into the mechanism of in-plane PC of QD arrays, showing a crucial importance of growth-related defects on photoresponsivity at low temperatures. [ABSTRACT FROM AUTHOR]

Metamorphic InAs/InGaAs quantum dot (QD) structures have been successfully used in optoelectronics as light-emitting and sensing devices. Previous optical and photoelectrical studies showed many benefits such as the shift of the operating range in the infrared and the possibility of engineering their properties via the control of strain. However, photovoltage (PV) kinetic properties of metamorphic QD structures have not been studied yet. PV kinetics in the vertical metamorphic InAs/In0.15Ga0.85As QD and wetting layer (WL) structures compared with conventional pseudomorphic InAs/GaAs QD ones are investigated. A red-shift of the photoresponse from metamorphic QDs in comparison with pseudomorphic QDs was observed, while the PV magnitudes remain similar. Moreover, time-dependent PV measurements reveal faster increase and decay rates in both the metamorphic samples. At the same time, all the structures reveal a non-monotonous kinetics. This kinetics is explained by an unwanted PV component generated in the interface of n+-GaAs buffer to the semi-insulating GaAs substrate, causing a signal opposite to the main PV generated at the top layers of structure. We believe the findings on faster carrier kinetics in metamorphic QDs can be helpful for the development of novel efficient optoelectronic devices. Specifically, the design of metamorphic QD structure is proposed to be improved by: (i) minimizing strain-related defects, (ii) keeping such interface defects far from QDs, (iii) utilizing n+-GaAs substrates. [ABSTRACT FROM AUTHOR]