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North Africa, the Middle East, and Europe (NAMEE domain) host a variety of suspended particles characterized by different optical and microphysical properties. In the current study, we investigate the importance of the lidar ratio (LR) on Cloud-Aerosol Lidar with Orthogonal Polarization–Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIOP-CALIPSO) aerosol retrievals towards assessing aerosols' impact on the Earth-atmosphere radiation budget. A holistic approach has been adopted involving collocated Aerosol Robotic Network (AERONET) observations, Radiative Transfer Model (RTM) simulations, as well as reference radiation measurements acquired using spaceborne (Clouds and the Earth's Radiant Energy System-CERES) and ground-based (Baseline Surface Radiation Network-BSRN) instruments. We are assessing the clear-sky shortwave (SW) direct radiative effects (DREs) on 550 atmospheric scenes, identified within the 2007–2020 period, in which the primary tropospheric aerosol species (dust, marine, polluted continental/smoke, elevated smoke, and clean continental) are probed using CALIPSO. RTM runs have been performed relying on CALIOP retrievals in which the default and the DeLiAn (Depolarization ratio, Lidar ratio, and Ångström exponent)-based aerosol-speciated LRs are considered. The simulated fields from both configurations are compared against those produced when AERONET AODs are applied. Overall, the DeLiAn LRs leads to better results mainly when mineral particles are either solely recorded or coexist with other aerosol species (e.g., sea-salt). In quantitative terms, the errors in DREs are reduced by ~26–27% at the surface (from 5.3 to 3.9 W/m2) and within the atmosphere (from −3.3 to −2.4 W/m2). The improvements become more significant (reaching up to ~35%) for moderate-to-high aerosol loads (AOD ≥ 0.2). [ABSTRACT FROM AUTHOR]

In this study, an assessment of the FORTH radiative transfer model (RTM) surface solar radiation (SSR) as well as its interdecadal changes (Δ(SSR)), namely global dimming and brightening (GDB), is performed during the 35-year period of 1984–2018. Furthermore, a thorough evaluation of SSR and (Δ(SSR)) is conducted against high-quality reference surface measurements from 1193 Global Energy Balance Archive (GEBA) and 66 Baseline Surface Radiation Network (BSRN) stations. For the first time, the FORTH-RTM Δ(SSR) was evaluated over an extended period of 35 years and with a spatial resolution of 0.5° × 0.625°. The RTM uses state-of-the-art input products such as MERRA-2 and ISCCP-H and computes 35-year-long monthly SSR and GDB, which are compared to a comprehensive dataset of reference measurements from GEBA and BSRN. Overall, the FORTH-RTM deseasonalized SSR anomalies correlate satisfactorily with either GEBA (R equal to 0.72) or BSRN (R equal to 0.80). The percentage of agreement between the sign of computed GEBA and FORTH-RTM Δ(SSR) is equal to 63.5% and the corresponding percentage for FORTH-RTM and BSRN is 54.5%. The obtained results indicate that a considerable and statistically significant increase in SSR (Brightening) took place over Europe, Mexico, Brazil, Argentina, Central and NW African areas, and some parts of the tropical oceans from the early 1980s to the late 2010s. On the other hand, during the same 35-year period, a strong and statistically significant decrease in SSR (Dimming) occurred over the western Tropical Pacific, India, Australia, Southern East China, Northern South America, and some parts of oceans. A statistically significant dimming at the 95% confidence level, equal to −0.063 Wm−2 year−1 (or −2.22 Wm−2) from 1984 to 2018 is found over the entire globe, which was more prevalent over oceanic than over continental regions (−0.07 Wm−2 year−1 and −0.03 Wm−2 year−1, statistically significant dimming at the 95% confidence level, respectively) in both hemispheres. Yet, this overall 35-year dimming arose from alternating decadal-scale changes, consisting of dimming during 1984–1989, brightening in the 1990s, turning into dimming over 2000–2009, and brightening during 2010–2018. [ABSTRACT FROM AUTHOR]